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The quantum mechanics of photon addition and subtraction

Myungshik Kim

Published Jan 1, 2008• 4 citations
Publisher

Abstract

In atomic-scale or quantum physics, an electromagnetic field is composed of photons, optical packets so small that a typical laser pointer with 1mW of power emits billions of them each second. Being able to take away or add a single photon in a light field at will would be useful for accurate engineering of quantum states. Such pure single photons are ideal for carrying and manipulating information in emerging quantum technologies, but generating them still is very challenging. In quantum physics, subtraction or addition of a photon is not a deterministic process. Instead, the probability is proportional to the number of photons originally in the electromagnetic field. This is described by the equation â|n〉 = √ n|n − 1〉 and â†|n〉 = √ n+ 1|n + 1〉, where â and ↠are annihilation and creation operators, respectively, representing the action of subtracting and adding a photon in a field composed of n photons.1 Such single-photon operations were limited to pure theoretical discussions until 2004, when Grangier and coworkers found a simple way to subtract a photon2 from a field. Passing through a beam splitter of high transmittivity, some photons can be split from the initial field. A ‘click’ detected in the photodetector in the reflected channel means one photon has been subtracted from the field: see Figure 1(a). When the initial field is composed of a small number of photons, the effect is dramatic and may even completely change the characteristics of the field. For example, let us take an initial single-mode squeezed state generated by ‘degenerate’ parametric down-conversion, which is an optical nonlinear process that converts a pump photon into two twin photons with half the pump photon energy. (This state is well known for its quantum noise squeezed into one quadrature at the expense of expanded noise in the other quadrature.) In order to visualize the noise properties and characteristics of the squeezed state, a probability-like function, such Figure 1. Setups to subtract (a) and add (b) a single photon from/to a light field. ρin and ρout denote the density operators of the input and output fields; BS is a low-reflectivity beam splitter; PDC is a nonlinear crystal where parametric down-conversion takes place; â and ↠denote on/off photodetectors.

DOI
10.1117/2.1200811.1369

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In atomic-scale or quantum physics, an electromagnetic field is composed of photons, optical packets so small that a typical laser pointer with 1mW of power emits billions of them each second. Being able to take away or add a single photon in a light field at will would be useful for accurate engineering of quantum states. Such pure single photons are ideal for carrying and manipulating information in emerging quantum technologies, but generating them still is very challenging. In quantum physics, subtraction or addition of a photon is not a deterministic process. Instead, the probability is proportional to the number of photons originally in the electromagnetic field. This is described by the equation â|n〉 = √ n|n − 1〉 and â†|n〉 = √ n+ 1|n + 1〉, where â and ↠are annihilation and creation operators, respectively, representing the action of subtracting and adding a photon in a field composed of n photons.1 Such single-photon operations were limited to pure theoretical discussions until 2004, when Grangier and coworkers found a simple way to subtract a photon2 from a field. Passing through a beam splitter of high transmittivity, some photons can be split from the initial field. A ‘click’ detected in the photodetector in the reflected channel means one photon has been subtracted from the field: see Figure 1(a). When the initial field is composed of a small number of photons, the effect is dramatic and may even completely change the characteristics of the field. For example, let us take an initial single-mode squeezed state generated by ‘degenerate’ parametric down-conversion, which is an optical nonlinear process that converts a pump photon into two twin photons with half the pump photon energy. (This state is well known for its quantum noise squeezed into one quadrature at the expense of expanded noise in the other quadrature.) In order to visualize the noise properties and characteristics of the squeezed state, a probability-like function, such Figure 1. Setups to subtract (a) and add (b) a single photon from/to a light field. ρin and ρout denote the density operators of the input and output fields; BS is a low-reflectivity beam splitter; PDC is a nonlinear crystal where parametric down-conversion takes place; â and ↠denote on/off photodetectors.
The non-Gaussian operations effected by adding or subtracting a photon on entangled optical beams emerging from a parametric down-conversion process have been suggested to enhance entanglement. Heralded photon addition or subtraction is, as a matter of fact, at the heart of continuous-variable entanglement distillation. The use of such processes has recently been experimentally demonstrated in the context of the generation of optical coherent-state superpositions or the verification of canonical commutation relations. Here, we carry out a systematic study of the effect of local photon additions and subtractions on a two-mode squeezed vacuum state, showing that the entanglement generally increases with the number of such operations. This is analytically proven when additions or subtractions are restricted to one mode only, while we observe that the highest entanglement is achieved when these operations are equally shared between the two modes. We also note that adding photons typically provides a stronger entanglement enhancement than subtracting photons, while photon subtraction performs better in terms of energy efficiency. Furthermore, we analyze the interplay between entanglement and non-Gaussianity, showing that it is more subtle than previously expected.
Single photons are the smallest excitation states of the elctromagnetic field. They can be experimentally created but there is no apparatus that performs this task with 100% efficiency. Many techniques and theorems of optical quantum information theory use single photons. In order to utilize them for information processing, it is reasonable to know if they had been successfully produced. In other words: One needs heralded single photons. How to achieve this, is the main result of this diploma thesis. The task has been to improve the efficiency of already existing single photon sources. An apparatus had to be found which postprocesses the output of such sources in order to either herald the photons or at least to improve the efficiency. This apparatus is explicitly allowed to use other optical sources, for example coherent states (laser). The situation has been formally represented by the assumption that single photon sources produce a mixture of vacuum and the single photon state. It is known that experimental set-ups also create higher photon contributions. These contributions are considered to be small in corresponding publications. For some cases they even seem to vanish at all. One can distinguish two regimes concerning the techniques which have been used in this work: linear and nonlinear optics. Linear optical tools, for example the beam splitter, do not absorb photons in the ideal case, but it is not easy to implement useful transformations by their means. Absorption and weak coupling are drawbacks which arise mainly in nonlinear optical media. This work shows that the interactions two-photon absorption and cross phase modulation can be used in schemes, which enable the heralding of single photons. Already there are some linear optical quantum gates which manipulate optical states by means of single photons. Photons do not interact with each other directly, in contrast to electrons for example. Therefore quantum gates which act on more than one mode are interesting. The effective interaction of these gates is not quitecomparable to unitary dynamics. Moreover, these gates do not function in each case. Measurements required in auxiliary modes yield different results for each single case and in order to obtain the desired effect the cases have to be selected according to the measurement results. It has been investigated, how such gates perform if they have statistical mixtures as a resource instead of perfect single-photon states. Yet, no improvement of the single-photon contribution has been accomplished by means of these apparatuses. Hereby it has not been disproved that it is possible to achieve this goal using other apparatuses and techniques of linear optics. Yet, it has been shown that an enhancement is possible but then a non-vanishing two-photon contribution is appended. One of the most basic quantum gates is the conditional sign flip. The optical 8 interaction cross phase modulation acts in quite the same way considering only single photons. This effect enables the heralding of single photons in the ideal case. Within this work it has been shown that a Mach-Zehnder interferometer, a cross phase modulating medium and a photo-detector can be employed for this purpose. One could use any source of light as input to the interferometer but a strong coherent state (laser) may be preferred for the purpose of enhancing the interaction. The absorption of two-photon states is another non-linear effect. Astonishingly this effect serves to generate a heralded single-photon state given two imperfect single-photon sources. First the photon adding tool is employed which consists of a beam splitter and a photo-detector. By means of that and the statistical mixtures of two single-photon sources one creates a mixture which contains vacuum, the single-photon state and additionally the two-photon Fock state. This mixture propagates through a Mach-Zehnder interferometer. The interferometer is adjusted such that it is transparent for incoming light. In addition to the interferometer alone a two-photon absorbing medium is placed in one of its arms. For this reason there is a chance that the two-photon contribution entering the interferometer is absorbed within this medium. We cannot exclude this unfortunate case. A detector is placed in one of the two output modes. The interferometer is adjusted such that the single photon state does not leave in the mode in which the detector is placed, but always in the other mode. The detector can only click if the two-photon state propagates through the interferometer and if it is not destroyed in the absorbing medium. If the detector then receives one photon it is obvious that another one must leave in the other mode. The whole phenomenon is very similar to the concept of null measurement. Although not a main result, it has been shown here that the so-called Hong-Ou-Mandel effect can be generalized. It has been proven that the beam splitter transforms Fock states with equal Fock number into superpositions of Fock numbers which are even in each mode. Another effect on special odd Fock states is conjectured.
Photon subtraction is useful to produce nonclassical states of light addressed to applications in photonic quantum technologies. After a very accelerated development, this technique makes possible obtaining either single photons or optical cats on demand. However, it lacks theoretical formulation enabling precise predictions for the produced fields. Based on the representation generated by the two-mode SU(2) coherent states, we introduce a model of entangled light beams leading to the subtraction of photons in one of the modes, conditioned to the detection of any photon in the other mode. We show that photon subtraction does not produce nonclassical fields from classical fields. It is also derived a compact expression for the output field from which the calculation of conditional probabilities is straightforward for any input state. Examples include the analysis of squeezed-vacuum and odd-squeezed states. We also show that injecting optical cats into a beam splitter gives rise to entangled states in the Bell representation.
We have witnessed proliferate growth in theoretical and experimental efforts to understand and control physical systems in a quantum level. In a quantum optics laboratory, Gaussian states, whose phase properties are described by Gaussian probability-like functions, were generated but there was some limitation to use them for various tasks of quantum information processing. There have been suggestions and realisations to engineer the quantum state by subtracting or adding single photons from/to a Gaussian field. It is also possible to test fundamental quantum theories using these techniques. We discuss various issues in subtraction and addition of single photons.
We develop a method to generate nonclassical light with a larger quadrature squeezing than one of the single-mode squeezed vacuum (SMSV) states by subtracting 2,4,6 photons from it. In general, the more photons are subtracted, the more gain of the squeezing (more than 3 dB) is observed in the measurement-induced continuous variable (CV) states of definite parity. However, the two-photon subtraction strategy is practically preferred. It can be implemented with higher success probability, wider squeezing gain width ∼5dB, and less quadrature variance. We demonstrate the mitigating effect of a photon-number resolving (PNR) detector with nonunit quantum efficiency on the output characteristics of the measurement-induced CV states, resulting in their slight decrease compared to ideal measurement of photons in the auxiliary mode. Use of a single photon in addition to the SMSV state at beam splitter (BS) input with subsequent registration of an odd number of photons (say, 3 photons) in auxiliary mode allows the implementation of the measurement-induced even CV state, which is several times brighter than the initial state, has lower quadrature noise, and is generated with greater probability.
The subtraction of a single photon from a multimode quantum field is analyzed as the conditional evolution of an open quantum system. We develop a theory describing different subtraction schemes in a unified approach and we introduce the concept of subtraction modes intrinsic to the process. The matching between the subtraction modes and the modes of the field defines different possible scenarios for the photon subtraction. In particular, our framework identifies: the conditions of pure photon subtraction, the quantum states of the field modes conditioned to the photon subtraction, the mode with the highest fidelity with a single-photon state when the subtraction is performed on multimode squeezed light. We use our theory to analyze the photon subtraction from a highly multimode quantum resource - a train of quantum squeezed or correlated optical pulses. Performing the photon subtraction optimally on various multimode light field has the potential to implement a number of quantum information protocols in a multiplexed and scalable way.