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arXiv:1002.3059

Quantum electrodynamics of one-photon wave packets

M. Stobińska, G. Alber, Gerd Leuchs

Published Feb 16, 2010• 0 citations
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Abstract

In this contribution we investigate quantum electrodynamical many-mode aspects by exploring the simplest possible situation in this context, namely the interaction of a single atom, modeled by a simple two-level system, with many-mode one-photon quantum states of the electromagnetic field. In particular, we concentrate on the question how the engineering of electromagnetic field modes influences the atom-field interaction. An interesting problem in this context is the engineering of ideal one-photon multi-mode quantum states which may excite a single atom perfectly [M. Stobińska, G. Alber, and G. Leuchs, EPL {\bf 86}, 14007 (2009)]. For purposes of quantum information processing such one-photon multi-mode states are particularly well suited for transmitting quantum information and for storing it in a material memory again.

DOI
10.48550/arxiv.1002.3059

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In this contribution we investigate quantum electrodynamical many-mode aspects by exploring the simplest possible situation in this context, namely the interaction of a single atom, modeled by a simple two-level system, with many-mode one-photon quantum states of the electromagnetic field. In particular, we concentrate on the question how the engineering of electromagnetic field modes influences the atom-field interaction. An interesting problem in this context is the engineering of ideal one-photon multi-mode quantum states which may excite a single atom perfectly [M. Stobińska, G. Alber, and G. Leuchs, EPL {\bf 86}, 14007 (2009)]. For purposes of quantum information processing such one-photon multi-mode states are particularly well suited for transmitting quantum information and for storing it in a material memory again.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.
Usually it is assumed that the stimulated emission appears as a consequence of the Bose—Einstein statistics of photons and that to observe this effect at least two excitations have to be initially present in the atom—field system. That is, both the atom and the electromagnetic field have to be excited. In this paper we show that stimulated emission can appear exclusively as a consequence of quantum interference in a system with just a single excitation. Specifically, we consider a single two-level atom which is initially in its lower energy state and it interacts with a single-photon multi-mode wave packet. We show that for a proper choice of the photon-wave packet the atom can exhibit stimulated emission.
In this Thesis the interaction of an electromagnetic field and matter is studied from various aspects in the general framework of cold atoms. Our subjects cover a wide spectrum of phenomena ranging from semiclassical few-level models to fully quantum mechanical interaction with structured reservoirs leading to non-Markovian open quantum system dynamics. Within closed quantum systems, we propose a selective method to manipulate the motional state of atoms in a time-dependent double-well potential and interpret the method in terms of adiabatic processes. Also, we derive a simple wave-packet model, based on distributions of generalized eigenstates, explaining the finite visibility of interference in overlapping continuous-wave atom lasers. In the context of open quantum systems, we develop an unraveling of non-Markovian dynamics in terms of piecewise deterministic quantum jump processes confined in the Hilbert space of the reduced system - the non-Markovian quantum jump method. As examples, we apply it for simple 2- and 3-level systems interacting with a structured reservoir. Also, in the context of ion-cavity QED we study the entanglement generation based on collective Dicke modes in experimentally realistic conditions including photonic losses and an atomic spontaneous decay.
We introduce a simple model for electromagnetically induced transparency in which all fields are treated quantum mechanically. We study a system of three separated atoms at fixed positions in a one-dimensional multimode optical cavity. The first atom serves as the source for a single spontaneously emitted photon; the photon scatters from a three-level Lambda-configuration atom which interacts with a single-mode field coupling two of the atomic levels; the third atom serves as a detector of the total transmitted field. We find an analytical solution for the quantum dynamics. From the quantum amplitude describing the excitation of the detector atom we extract information that provides exact single-photon analogs to wave delays predicted by semi-classical theories. We also find complementary information in the expectation value of the electric field intensity operator.
Quantum information processing tasks have been implemented in various physical platforms. In this thesis, we consider two specific implementations: Part I presents a detailed study of the interaction of a single atom with a light pulse. Part II examines the case of a quantum controlled-phase gate in circuit quantum electrodynamics in the ultrastrong coupling regime. They are both actively pursued by many research groups. In Part I, we first present the framework for a single two-level atom interacting with the quantized electromagnetic field. The effect of temporal and spectral properties of the pulses on atomic excitation is studied for both Fock state and coherent state pulse. The detailed analysis of atomic excited state population is provided for single photon pulse with various temporal shapes. The work is then extended to a more general case with two spatial-modes and multi-photon pulses. The difference between Fock state and coherent state pulse on atomic excitation is further investigated. We find that at few photon levels, the maximum atomic excitation probability is a monotonic function of photon number for the coherent state pulse, but not for the Fock state pulse. Furthermore, we show that the atomic dynamics can be controlled by the initial relative phase between the two counter-propagating coherent state pulses incident on the atom, which is not the case with two Fock state pulses. The theoretical prediction is then compared with an experiment, where a single trapped 87Rb atom interacts with coherent state pulses engineered in temporal shape of rising exponential and rectangular form. Next, we propose a quantum memory setup based on a single two-level atom in a half cavity with a moving mirror. The efficiency of the quantum storage process is studied analytically and