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Quantum entanglement control of electron–phonon systems by light irradiation

Kunio Ishida, Hiroaki Matsueda, Akira Kamada

Published Jan 1, 2022• 5 citations
Publisher

Abstract

We numerically study the dynamics of quantum entanglement between interacting electron-phonon and qubit-spin systems under photoirradiation, employing a model of multiple spins and boson modes. The interplay of the antiferromagnetic exchange and electron-phonon interactions provides us with a phase diagram, wherein each phase is characterized by the ground state property of the electron-phonon system. Light irradiation of the electron-phonon system facilitates the generation of quantum entanglement, according to the spin configuration and the phonon state in the ground state. Analyses using the quantum mutual information and the singular values of the reduced density matrix indicate that the quantum mechanical effect of the irradiated light appears in the state of the material.

DOI
10.1039/d2fd00007e

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We numerically study the dynamics of quantum entanglement between interacting electron-phonon and qubit-spin systems under photoirradiation, employing a model of multiple spins and boson modes. The interplay of the antiferromagnetic exchange and electron-phonon interactions provides us with a phase diagram, wherein each phase is characterized by the ground state property of the electron-phonon system. Light irradiation of the electron-phonon system facilitates the generation of quantum entanglement, according to the spin configuration and the phonon state in the ground state. Analyses using the quantum mutual information and the singular values of the reduced density matrix indicate that the quantum mechanical effect of the irradiated light appears in the state of the material.
The generation of quantum entanglement between phonons in photoirradiated remote electron-phonon systems is numerically studied. Upon excitation by a visible/ultraviolet laser pulse, the entanglement of electrons is immediately generated and that of phonons follows via electron-phonon interactions, i.e., the entanglement generation of phonons is a two-step process. Therefore, it is important to design the temporal properties of incident optical pulses in order to control the entanglement of electrons and/or phonons. These features are revealed by the quantum mutual information and the composite modes derived from the Heisenberg equation of motion. The calculated results also show that the dynamics of the phonon entanglement can be observed by time-resolved spectroscopy on the scattered light.
Herein, the dynamics of excitons coupled with optical phonons in a triangular system is numerically studied. By representing the excitons by quasi-spin states, the similarity between the chiral spin states and the exciton chiral states is discussed. In particular, the optical control of excitons is discussed, where photoirradiation causes the switching of the exciton states on the ultrafast time scale by Raman scattering. A phase diagram is obtained based on the ground-state properties of the system determined by the magnitudes of the exciton-phonon interactions and exciton transfer energy. By varying the frequency and/or intensity of light, a transition between exciton-phonon composite states is induced, which suggests the possibility of the coherent control of the chiral properties of excitonic systems via phonon excitation.
We propose a quantum dynamics simulator for light-irradiated matter. As the coherent control of the quantum states of matter is an intriguing problem in realizing quantum technology, the quantum properties of light-matter complexes have attracted much attention. Theoretical calculations corresponding to individual experimental configurations are required to understand these properties, and simulation methods that flexibly adapt to various experimental configurations are required. In this paper, we propose a quantum dynamics simulation method that encompasses program modules corresponding to light sources, optical components, material systems, and the evaluation of physical properties. We demonstrate the entanglement generation dynamics between two spin-chains via irradiated photons and show that a flexible and expandable quantum dynamics simulator can be constructed.
Competing interactions are often responsible for intriguing phase diagrams in correlated electron systems. Here we analyze the competition of instantaneous short-range Coulomb interaction U with the retarded electron-electron interaction induced by an electron-phonon coupling g as described by the Hubbard-Holstein model. The ground-state phase diagram of this model in the limit of large dimensions at half-filling is established. The study is based on dynamical mean-field theory combined with the numerical renormalization group. Depending on U , g , and the phonon frequency ω 0 , the ground state is antiferromagnetically (AFM) or charge ordered (CO). We find quantum phase transitions from the AFM to CO state to occur when U-λ≃0, where λ characterizes the phonon-induced effective attraction. The transition is continuous for small couplings and large phonon frequencies ω 0 and becomes discontinuous for large couplings and small values of ω 0 . We comment on the possible relevance of this work for Ba 1- x K x BiO 3 .