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Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium (EFTF/IFCS)

High-Stability Rb Optical Clock Based on Pulse-Modulated Broad-Spectrum Comb-Tooth Laser

Xiaolei Guan, Tiantian Shi, Jianxiang Miao, Tian Zhao, Jingbiao Chen

Published Jul 7, 2021• 0 citations
Publisher

Abstract

We have proposed a new scheme to realize the Rb optical clock using a pulse-modulated broad-spectrum multi-frequency laser. By applying a pulse-modulated signal to a 420 nm external cavity diode laser, a broad-spectrum comb-tooth laser with multiple frequency components is generated, which can interact with almost all the Rb atoms with different transverse velocities, so that more Rb atoms in the Rb cell can contribute to the frequency stabilization signal of the clock transition spectral line. The effective atomic number is expected to be improved by a factor of 102- 103, which will significantly improve the signal-to-noise ratio of spectrum, so as to optimize the frequency stability of Rb optical clock. The Rb optical frequency standard with high stability can be widely used in laser physics and precision measurement.

DOI
10.1109/eftf/ifcs52194.2021.9604345

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We have proposed a new scheme to realize the Rb optical clock using a pulse-modulated broad-spectrum multi-frequency laser. By applying a pulse-modulated signal to a 420 nm external cavity diode laser, a broad-spectrum comb-tooth laser with multiple frequency components is generated, which can interact with almost all the Rb atoms with different transverse velocities, so that more Rb atoms in the Rb cell can contribute to the frequency stabilization signal of the clock transition spectral line. The effective atomic number is expected to be improved by a factor of 102- 103, which will significantly improve the signal-to-noise ratio of spectrum, so as to optimize the frequency stability of Rb optical clock. The Rb optical frequency standard with high stability can be widely used in laser physics and precision measurement.
We demonstrated a compact 780 nm rubidium optical clock, which includes an optical frequency standard and an optical frequency comb, with an optical volume of 11.6 liters. Unlike the 778 nm rubidium atomic clocks based on two-photon transition, here, the laser frequency is stabilized to the Rb D2 transition, using modulation transfer spectroscopy. This approach effectively eliminates Doppler background and provides a high signal to noise ratio and high sensitivity. A nearly 300 MHz microwave signal, whose phase exactly tracks that of the optical frequency standard, is generated via the optical frequency comb, yielding a frequency instability of 1.91 E-13 @1 s and 5.29 E-14 @1000 s in the electronic domain. To the best of our knowledge, this is the most precise frequency stabilization result for the first-excited-state transition of alkali metal atoms to date and represents the first optical clock based on this transition. These results offer a promising approach for the development of portable optical clocks.
A compact rubidium optical clock is presented, incorporating an optical frequency standard, a fiber frequency comb, and associated control electronics. Modulation transfer spectroscopy, devoid of Doppler background and characterized by a high signal-to-noise ratio and sensitivity, is employed to lock the laser frequency to the hyperfine transitions of rubidium atomic lines. The clock exhibits a short-term stability of 4.10 × 10-13at a 1-second gate time, and the stability remains below 7.27 × 10-13up to 1000 seconds. These results offer a promising alternative approach for the development of portable optical clocks.
We describe a high-performance, compact optical frequency standard based on a microfabricated Rb vapor cell and a low-noise, external cavity diode laser operating on the Rb two-photon transition at 778 nm. The optical standard achieves an instability of 1.8 × 10 − 13 τ − 1 / 2 for times less than 100 s and a flicker noise floor of 1 × 10 − 14 out to 6000 s. At long integration times, the instability is limited by variations in optical probe power and the ac Stark shift. The retrace was measured to 5.7 × 10 − 13 after 30 h of dormancy. Such a simple, yet high-performance optical standard could be suitable as an accurate realization of the meter or, if coupled with an optical frequency comb, as a compact atomic clock comparable to a hydrogen maser.
The paper presents the realisation of a high-performance vapour-cell atomic frequency standard demonstrator based on laser optical pumping. The development of such devices aims to fully exploit the advantages of using a narrow-band diode laser pump light source instead of the discharge lamps commonly used in Rb gas-cell clocks. These advantages include improved control over the pump light spectrum, higher selectivity of the optical pumping, and increased signal contrast, and thus show the potential for the realisation of Rb atomic clocks with improved short-term frequency stability.
Optical wavelength standards, based on the optical transitions of atoms or molecules, provide ultra-high precision frequency references and are the core technology of next-generation optical clocks. Their stability far exceeds that of the microwave frequency range, laying the foundation for precision metrology and cutting-edge scientific research. The wavelength standard device based on the 5S1/2-5D3/2 hyperfine level two-photon transition of 87Rb atoms exhibits significant advantages such as no Doppler broadening, high signal-to-noise ratio (SNR), and potential for miniaturization and chip integration, showing important application potential in precision measurement fields like rubidium atomic clocks and optical communication. In this paper, an experimental setup for two-photon transition was constructed using an external cavity diode laser (ECDL), achieving stable locking of the 778 nm wavelength by modulating the laser current. The effects of the temperature and length of the atomic vapor cell on the blue fluorescence linewidth, SNR, and frequency stability were systematically studied, further optimizing the system. By using an atomic vapor cell designed at Brewster's angle, optical reflection loss was effectively reduced, compensating for the impact of shortened optical path on frequency stability in miniaturized atomic vapor cells. This provides new research directions and performance enhancement solutions for the miniaturization and chip integration of two-photon transition systems. In the improved system, a Brewster-angle glass vapor cell with a length of 30 mm was used and heated to 110°C, achieving a linewidth of 1.69 MHz full width at half maximum (FWHM) and a SNR of 20 dB. The system demonstrated a instability of 9.86×10-11 over a 1-second averaging time and a minimum instability of 5.79×10-11 over a 5.7-second averaging time. This achievement provides key technological support for the practical application of the next generation of miniaturized optical atomic clocks, with the potential for widespread use in portable metrology equipment and space science through integrated design and noise suppression optimization in the future.
We present the development and complete spectral characterization of our compact and frequency-stabilized laser heads, to be used for rubidium atomic clocks and basic spectroscopy. The light source is a Distributed Feed-Back (DFB) laser diode emitting at 780 nm or 795 nm. The laser frequency is stabilized on a sub-Doppler absorption peak of the 87Rb atom, obtained from an evacuated rubidium cell. These laser heads, including the electronics for the light signals detection, have an overall volume of 0.63 liters. We also present a variant of the laser head into which is integrated an Acousto-Optical Modulator (AOM) that precisely detunes the laser frequency in order to minimize the AC Stark shift in Rb atomic clocks.