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Journal of Physics Conference Series

Coherent magneto-optical resonances in hot potassium vapor

S. Gateva, S. Tsvetkov, G. Todorov, Silvia Gozzini, K. A. Nasyrov, C. Andreeva, S. Cartaleva

Published Mar 1, 2021• 0 citations
Publisher

Abstract

Abstract In this communication, we present experimental results on the preparation of magneto-optical resonances in potassium. The magneto-optical resonances are registered in Hanle configuration, i.e. monitoring the atomic fluorescence vs the applied magnetic field scanned around zero value. The excitation of the second resonance line with a wavelength of 404.4 nm leads both to direct fluorescence at 404.4 nm and to a cascade decay with fluorescence at 770.1 nm and 764.5 nm (first resonance line transitions). This transfer is evidenced by the registration of a narrow magneto-optical resonance in the fluorescence. It should also be noted that even after multiple cascade transitions, the resonance observed on the infrared lines has a much better signal/noise ratio compared to that on the excited second resonance line. Therefore, the study of these sub-Doppler-width magneto-optical resonances in hot potassium vapor will be useful for the further development of high-resolution magneto-optical laser spectroscopy.

DOI
10.1088/1742-6596/1859/1/012022

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Abstract In this communication, we present experimental results on the preparation of magneto-optical resonances in potassium. The magneto-optical resonances are registered in Hanle configuration, i.e. monitoring the atomic fluorescence vs the applied magnetic field scanned around zero value. The excitation of the second resonance line with a wavelength of 404.4 nm leads both to direct fluorescence at 404.4 nm and to a cascade decay with fluorescence at 770.1 nm and 764.5 nm (first resonance line transitions). This transfer is evidenced by the registration of a narrow magneto-optical resonance in the fluorescence. It should also be noted that even after multiple cascade transitions, the resonance observed on the infrared lines has a much better signal/noise ratio compared to that on the excited second resonance line. Therefore, the study of these sub-Doppler-width magneto-optical resonances in hot potassium vapor will be useful for the further development of high-resolution magneto-optical laser spectroscopy.
Experimental investigation of magneto-optical resonances on the potassium D2 line with λ=766.7 nm from the point of view of magnetometry applications is reported. The resonances are registered in a modified Hanle effect configuration based on counterpropagating pump and probe laser beams with orthogonal linear polarizations in a buffer gas cell with dimensions (diameter and length) of 8 mm. The amplitude, width, and contrast of the resonances registered in fluorescence and transmission are measured. The transformation of the bright magneto-optical resonances detected in fluorescence to dark ones by controlling the optical thickness of potassium vapor is analyzed. The influence of the laser intensity, buffer gas, and transverse magnetic field are considered. The experimental results show the system’s potential for magnetic field sensing and self-calibration.
Abstract The coherent magneto-optical resonances on the potassium D2 line are investigated from the point of view of magnetometry applications. The measurements are performed in Hanle configuration with potassium excited by circularly polarized laser beam in cell with dimensions 8 mm and buffer gas 30 Torr Ne. The parameters of the resonances registered in fluorescence and transmission are compared. The capability of the laser system to work with magnetically unshielded cell is demonstrated. The registration of bright and dark magneto-optical resonances detected in fluorescence by controlling the optical thickness of potassium vapor is discussed. The influence of the laser power and transverse magnetic field are considered. The experimental results show the potential of the system for magnetic field sensing and calibration.
We present experimental investigation on the fluorescence profiles observed by excitation of the hyperfine transitions of the second resonance line of potassium with a wavelength of 404.4 nm in dependence on the atomic density. This leads to both direct decay of the excited level population to the ground state (violet fluorescence), and to cascade decay via the first resonance lines (infrared fluorescence). It has been shown that the behavior of these two fluorescence profiles is different: increasing the atomic density, the violet fluorescence profile exhibits a well-pronounced self-absorption dip, while the infrared line does not show any narrow-width reduced absorption structure. Moreover, the profiles of the infrared line have a higher signal-to-noise ratio than that of the violet line. Our investigations show that beside atomic population, atomic polarization is also transferred by the cascade transitions. This is evidenced by registration of coherent magneto-optical resonances at the two fluorescence lines. The signal-to-noise ratio of these resonances registered at the first resonance line is significantly higher than at those obtained at the second resonance line. The proposed study makes it possible to examine cascade transitions in alkali atoms, particularly the preservation of atomic polarization, i.e. the coherence transfer by cascade transitions.
We present the results of an experimental as well as a theoretical study of nonlinear magneto-optical resonances in diatomic potassium molecules in the electronic ground state with large values of the angular momentum quantum number $J\ensuremath{\sim}100$. At zero magnetic field, the absorption transitions are suppressed because of population trapping in the ground state due to Zeeman coherences between magnetic sublevels of this state along with depopulation pumping. The destruction of such coherences in an external magnetic field was used to study the resonances in this work. K2{}_{2}2​ molecules were formed in a glass cell filled with potassium metal at a temperature above 150 ${}^{\ensuremath{\circ}}$C. The cell was placed in an oven and was located in a homogeneous magnetic field B, which was scanned from 0 to 0.7 T. QQQ-type and RRR-type transitions were excited with a tunable, single-mode diode laser with a central wavelength of 660 nm. Well-pronounced nonlinear Hanle effect signals were observed in the intensities of the linearly polarized components of the laser-induced fluorescence (LIF) detected in the direction parallel to the B field with polarization vectors parallel (Ipar{I}_{\text{par}}Ipar​) and perpendicular (Iper{I}_{\text{per}}Iper​) to the polarization vector of the exciting laser radiation, which was orthogonal to B. The intensities of the LIF components were detected for different experimental parameters, such as laser power density and vapor temperature, in order to compare them with numerical simulations that were based on the optical Bloch equations for the density matrix. We report good agreement of our measurements with numerical simulations. Narrow, subnatural linewidth dark resonances in Iper(B){I}_{\text{per}}(B)Iper​(B) were detected and explained.
The ultra-narrow resonances, obtained in the coherent spectroscopy of alkali atoms, originate from the destruction of the laser-induced coherence in the ground state. In the case of a single frequency, near-resonant excitation and a suitable geometry of irradiation and observation by scanning a weak magnetic field, one observes coherent population trapping in a Hanle - configuration. The laser field transfers the nonlinear interference resonances created in the degenerate Zeeman sublevels of the ground states to the upper level. As a result, the well-known ground state Hanle - effect is observed in the fluorescence. We investigated theoretically and experimentally the shape, amplitude and sign of these resonances and their dependence on the excitation and registration conditions. The experiment was performed on the D1 87Rb line. Results of the computations were compared with the measurements for corresponding experimental conditions.
We present the observation of coherent population trapping resonances on the second resonance line of potassium: 4s 2 S 1/2 → 5p 2 P 3/2 with wavelength of 404.4 nm.Moreover, a transfer of the coherent population trapping resonance occurs to the excited 4p 2 P 1/2 and 4p 2 P 3/2 states of the first resonance line due to cascade transitions.This transfer is evidenced by the observation of narrow resonances at the infrared 4s 2 S 1/2 → 4p 2 P 1/2 and 4s 2 S 1/2 → 4p 2 P 3/2 transitions when alkali excitation is performed at the 404.4 nm violet line.