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What can be learnt on a supersolid from its high-energy scattering response? Analytical considerations

Lauriane Chomaz

Published May 4, 2020• 0 citations
OpenAlex

Abstract

High-energy scattering spectroscopy is a widely-established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of such exotic states within a simple model. I focus on the scaling laws relating these three observables in the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. I illustrate and specify the general formulae using relevant ansatzes for the supersolid states of dipolar gases in these regimes. This work brings an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. It generally highlights new possibilities for probing supersolid states while providing a simple framework to describe such intriguing states.

Related papers

Probing the supersolid order via high-energy scattering: Analytical relations among the response, density modulation, and superfluid fraction

Lauriane Chomaz

High-energy scattering spectroscopy is a widely established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of density-modulated states within a classical-field approach. I focus on the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. Using relevant Ans\"atze for the fields of dipolar supersolid states in these regimes, I specify and illustrate the scaling laws relating the three observables. This work was first prompted to develop an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. Beyond this specific application, this works provides a simple and general framework to describe density-modulated states and in particular the intriguing case of supersolids. It describes key properties characterizing the supersolid order and highlights possibilities for probing such properties based on high-energy scattering response.

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Bose polarons in superfluids and supersolids

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Bose-Einstein condensation is a macroscopic quantum phenomenon where cooling down a gas of bosonic particles to ultracold temperatures results in the macroscopic occupation of the lowest energy state. This new state of matter has been used as a quantum simulator of many-body phenomena and theories due to its extreme tunability and controllability. An important example of such a many-body system is the polaron which, in its most general form, describes an impurity interacting with a bosonic bath. In the case of ultracold Bose gases, the impurity interacts with and is dressed by the Bogoliubov excitations of the gas. A supersolid is a state of matter that exhibits both superfluidity and crystalline order, which are seemingly irreconcilable properties. It has recently been observed in dipolar ultracold Bose gases, where it arises from the long-range anisotropic dipole-dipole interactions, and also other systems. The breaking of both translational symmetry and gauge symmetry results in multiple excitation modes in the supersolid. In this thesis, the charged Bose polaron and an impurity in a dipolar ultracold Bose gas exhibiting supersolidity (the supersolid Bose polaron) are studied. The ground-state properties of the charged Bose polaron are discussed using a variational path-integral approach. Absorption spectroscopy is proposed as a probe of the charged Bose polaron, and the optical response is studied for weak impurity-boson interactions. Next, the one-dimensional dipolar supersolid Bose polaron is investigated where multiple approaches are used for the derivation of the ground-state properties. The study of the polaron problem with a supersolid background is of particular interest because of the rich excitation spectrum of the supersolid. Interesting phenomena, such as possible localization of the polaron to a single droplet for strong interactions, are observed. The absorption spectrum of a charged impurity in the supersolid is also derived, which, because of the different excitation modes of the supersolid, shows multiple peaks from which information such as the superfluid fraction may be obtained.

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The Excitation Spectra of a Supersolid

Lily Platt

This thesis explores the excitation spectra of supersolids - materials that remarkably manifest both lattice structure and superfluidity. We focus on an ultracold dilute gas exhibiting one-dimensional crystal structure with two gapless excitation branches. Two distinct supersolid systems are examined: a one dimensional Bose-Einstein condensate with softcore interactions, and a three dimensional dipolar Bose Einstein condensate confined within an infinitely long tube-shape potential. We investigate the crystal-like excitations of the supersolid through the use of the linear chain model and by introducing an elastic constant derived from ground-state calculations. Subsequently, we adopt a hydrodynamic approach based on an effective Lagrangian, which depends upon three fields, corresponding to lattice deformations, defect density current, the global phase fluctuations and four elastic parameters. This description of the supersolid allows for the determination of low-energy excitations, as well as the behaviour of the associated density and phase fluctuations of the two gapless branches. We validate our predictions for the low energy excitations by comparison to results from directly solving the Bogoliubov-de-Gennes equations, finding excellent agreement. This thesis provides a deeper understanding of the different types of supersolid systems, and how their low-energy behaviour depends upon their characteristic elastic energy scales.

•Sep 20, 2024•0 citations
High-energy scattering spectroscopy is a widely-established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of such exotic states within a simple model. I focus on the scaling laws relating these three observables in the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. I illustrate and specify the general formulae using relevant ansatzes for the supersolid states of dipolar gases in these regimes. This work brings an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. It generally highlights new possibilities for probing supersolid states while providing a simple framework to describe such intriguing states.
High-energy scattering spectroscopy is a widely established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of density-modulated states within a classical-field approach. I focus on the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. Using relevant Ans\"atze for the fields of dipolar supersolid states in these regimes, I specify and illustrate the scaling laws relating the three observables. This work was first prompted to develop an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. Beyond this specific application, this works provides a simple and general framework to describe density-modulated states and in particular the intriguing case of supersolids. It describes key properties characterizing the supersolid order and highlights possibilities for probing such properties based on high-energy scattering response.
Bose-Einstein condensation is a macroscopic quantum phenomenon where cooling down a gas of bosonic particles to ultracold temperatures results in the macroscopic occupation of the lowest energy state. This new state of matter has been used as a quantum simulator of many-body phenomena and theories due to its extreme tunability and controllability. An important example of such a many-body system is the polaron which, in its most general form, describes an impurity interacting with a bosonic bath. In the case of ultracold Bose gases, the impurity interacts with and is dressed by the Bogoliubov excitations of the gas. A supersolid is a state of matter that exhibits both superfluidity and crystalline order, which are seemingly irreconcilable properties. It has recently been observed in dipolar ultracold Bose gases, where it arises from the long-range anisotropic dipole-dipole interactions, and also other systems. The breaking of both translational symmetry and gauge symmetry results in multiple excitation modes in the supersolid. In this thesis, the charged Bose polaron and an impurity in a dipolar ultracold Bose gas exhibiting supersolidity (the supersolid Bose polaron) are studied. The ground-state properties of the charged Bose polaron are discussed using a variational path-integral approach. Absorption spectroscopy is proposed as a probe of the charged Bose polaron, and the optical response is studied for weak impurity-boson interactions. Next, the one-dimensional dipolar supersolid Bose polaron is investigated where multiple approaches are used for the derivation of the ground-state properties. The study of the polaron problem with a supersolid background is of particular interest because of the rich excitation spectrum of the supersolid. Interesting phenomena, such as possible localization of the polaron to a single droplet for strong interactions, are observed. The absorption spectrum of a charged impurity in the supersolid is also derived, which, because of the different excitation modes of the supersolid, shows multiple peaks from which information such as the superfluid fraction may be obtained.
This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.
The elusive supersolid, an exotic quantum phase that combines the properties of a crystalline solid and those of a superfluid, has been recently discovered in a system of Bose-condensed strongly magnetic atoms. In this paper, I report on an experiment that directly demonstrates the superfluid behavior of the dipolar supersolid measuring its anomalous response to a rotational excitation. I complement the illustration of the experimental results with a review and an original interpretation of a seminal model due to Leggett.
We develop a linear-response theory to provide a unified description of two recent spectroscopy protocols for probing one-dimensional supersolid states realized in cold-atom systems. Both protocols involve applying a periodic optical potential to excite the supersolid and determine its excitation frequencies and density response characteristics. This information can be used to estimate the superfluid fraction. We validate our linear-response theory against nonlinear mean-field simulations of the dynamics for ring, box, and harmonically trapped cases. A key focus is the behavior at the band edge---the regime occurring when the optical potential used to excite the system has a wavelength that is twice the value of the supersolid lattice constant. Here symmetry can be used to selectively excite a mode from one of the two low-energy gapless excitation bands. We also consider the application of the spectroscopy protocols to determine the superfluid fraction, showing the relationship to hydrodynamic theory and a Josephson-junction array model. Our analysis and results suggest that the phase protocol we introduce has potential advantages for experimental application over the density protocol.
This thesis explores the excitation spectra of supersolids - materials that remarkably manifest both lattice structure and superfluidity. We focus on an ultracold dilute gas exhibiting one-dimensional crystal structure with two gapless excitation branches. Two distinct supersolid systems are examined: a one dimensional Bose-Einstein condensate with softcore interactions, and a three dimensional dipolar Bose Einstein condensate confined within an infinitely long tube-shape potential. We investigate the crystal-like excitations of the supersolid through the use of the linear chain model and by introducing an elastic constant derived from ground-state calculations. Subsequently, we adopt a hydrodynamic approach based on an effective Lagrangian, which depends upon three fields, corresponding to lattice deformations, defect density current, the global phase fluctuations and four elastic parameters. This description of the supersolid allows for the determination of low-energy excitations, as well as the behaviour of the associated density and phase fluctuations of the two gapless branches. We validate our predictions for the low energy excitations by comparison to results from directly solving the Bogoliubov-de-Gennes equations, finding excellent agreement. This thesis provides a deeper understanding of the different types of supersolid systems, and how their low-energy behaviour depends upon their characteristic elastic energy scales.