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Evidence of superfluidity in a dipolar supersolid

Giulio Biagioni

Published Jan 1, 2021• 0 citations
Publisher

Abstract

The elusive supersolid, an exotic quantum phase that combines the properties of a crystalline solid and those of a superfluid, has been recently discovered in a system of Bose-condensed strongly magnetic atoms. In this paper, I report on an experiment that directly demonstrates the superfluid behavior of the dipolar supersolid measuring its anomalous response to a rotational excitation. I complement the illustration of the experimental results with a review and an original interpretation of a seminal model due to Leggett.

DOI
10.1393/ncc/i2021-21107-5

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The elusive supersolid, an exotic quantum phase that combines the properties of a crystalline solid and those of a superfluid, has been recently discovered in a system of Bose-condensed strongly magnetic atoms. In this paper, I report on an experiment that directly demonstrates the superfluid behavior of the dipolar supersolid measuring its anomalous response to a rotational excitation. I complement the illustration of the experimental results with a review and an original interpretation of a seminal model due to Leggett.
A key manifestation of superfluidity in liquids and gases is a reduction of the moment of inertia under slow rotations. Nonclassical rotational effects have also been considered in the context of the elusive supersolid phase of matter, in which superfluidity coexists with a lattice structure. Here, we show that the recently discovered supersolid phase in dipolar quantum gases features a reduced moment of inertia. Using a dipolar gas of dysprosium atoms, we studied a peculiar rotational oscillation mode in a harmonic potential, the scissors mode, previously investigated in ordinary superfluids. From the measured moment of inertia, we deduced a superfluid fraction that is different from zero and of order of unity, providing direct evidence of the superfluid nature of the dipolar supersolid.
Supersolids are states of matter that spontaneously break two continuous symmetries: translational invariance due to the appearance of a crystal structure and phase invariance due to phase locking of single-particle wave functions, responsible for superfluid phenomena. While originally predicted to be present in solid helium, ultracold quantum gases provided a first platform to observe supersolids, with particular success coming from dipolar atoms. Phase locking in dipolar supersolids has been probed through e.g. measurements of the phase coherence and gapless Goldstone modes, but quantized vortices, a hydrodynamic fingerprint of superfluidity, have not yet been observed. Here, with the prerequisite pieces at our disposal, namely a method to generate vortices in dipolar gases and supersolids with two-dimensional crystalline order, we report on the theoretical investigation and experimental observation of vortices in the supersolid phase. Our work reveals a fundamental difference in vortex seeding dynamics between unmodulated and modulated quantum fluids. This opens the door to study the hydrodynamic properties of exotic quantum systems with multiple spontaneously broken symmetries, in disparate domains such as quantum crystals and neutron stars.
Abstract Supersolid states simultaneously feature properties typically associated with a solid and with a superfluid. Like a solid, they possess crystalline order, manifesting as a periodic modulation of the particle density; but unlike a typical solid, they also have superfluid properties, resulting from coherent particle delocalization across the system. Such states were initially envisioned in the context of bulk solid helium, as a possible answer to the question of whether a solid could have superfluid properties1–5. Although supersolidity has not been observed in solid helium (despite much effort)6, ultracold atomic gases provide an alternative approach, recently enabling the observation and study of supersolids with dipolar atoms7–16. However, unlike the proposed phenomena in helium, these gaseous systems have so far only shown supersolidity along a single direction. Here we demonstrate the extension of supersolid properties into two dimensions by preparing a supersolid quantum gas of dysprosium atoms on both sides of a structural phase transition similar to those occurring in ionic chains17–20, quantum wires21, 22 and theoretically in chains of individual dipolar particles23, 24. This opens the possibility of studying rich excitation properties25–28, including vortex formation29–31, and ground-state phases with varied geometrical structure7, 32 in a highly flexible and controllable system.
We study the spectrum of elementary excitations of a dipolar Bose gas in a three-dimensional anisotropic trap across the superfluid-supersolid phase transition. Theoretically, we show that, when entering the supersolid phase, two distinct excitation branches appear, respectively associated with dominantly crystal and superfluid excitations. These results confirm infinite-system predictions, showing that finite-size effects play only a small qualitative role, and connect the two branches to the simultaneous occurrence of crystal and superfluid orders. Experimentally, we probe compressional excitations in an Er quantum gas across the phase diagram. While in the Bose-Einstein condensate regime the system exhibits an ordinary quadrupole oscillation, in the supersolid regime we observe a striking two-frequency response of the system, related to the two spontaneously broken symmetries.
This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.