Supersolids are states of matter that spontaneously break two continuous symmetries: translational invariance due to the appearance of a crystal structure and phase invariance due to phase locking of single-particle wave functions, responsible for superfluid phenomena. While originally predicted to be present in solid helium, ultracold quantum gases provided a first platform to observe supersolids, with particular success coming from dipolar atoms. Phase locking in dipolar supersolids has been probed through e.g. measurements of the phase coherence and gapless Goldstone modes, but quantized vortices, a hydrodynamic fingerprint of superfluidity, have not yet been observed. Here, with the prerequisite pieces at our disposal, namely a method to generate vortices in dipolar gases and supersolids with two-dimensional crystalline order, we report on the theoretical investigation and experimental observation of vortices in the supersolid phase. Our work reveals a fundamental difference in vortex seeding dynamics between unmodulated and modulated quantum fluids. This opens the door to study the hydrodynamic properties of exotic quantum systems with multiple spontaneously broken symmetries, in disparate domains such as quantum crystals and neutron stars.
Supersolids are states of matter that spontaneously break two continuous symmetries: translational invariance due to the appearance of a crystal structure and phase invariance due to phase locking of single-particle wave functions, responsible for superfluid phenomena. While originally predicted to be present in solid helium, ultracold quantum gases provided a first platform to observe supersolids, with particular success coming from dipolar atoms. Phase locking in dipolar supersolids has been probed through e.g. measurements of the phase coherence and gapless Goldstone modes, but quantized vortices, a hydrodynamic fingerprint of superfluidity, have not yet been observed. Here, with the prerequisite pieces at our disposal, namely a method to generate vortices in dipolar gases and supersolids with two-dimensional crystalline order, we report on the theoretical investigation and experimental observation of vortices in the supersolid phase. Our work reveals a fundamental difference in vortex seeding dynamics between unmodulated and modulated quantum fluids. This opens the door to study the hydrodynamic properties of exotic quantum systems with multiple spontaneously broken symmetries, in disparate domains such as quantum crystals and neutron stars.
Abstract Synchronization is a widespread phenomenon in natural and engineered systems, governing the emergence of collective dynamics in different domains including biology and classical and quantum physics. In quantum many-body systems, synchronization has emerged as a tool to probe out-of-equilibrium behaviour and internal correlations. Supersolids—quantum phases that combine crystalline order and superfluidity—offer a platform to explore synchronization in systems with coexisting broken symmetries. Here we investigate the dynamics of a dipolar supersolid subjected to external rotation. We show that, above a critical driving frequency, the crystal revolution undergoes a sudden synchronization with the rotating field seeded by the nucleation of quantized vortices, hallmark of superfluidity. This transition reflects the interplay between the solid-like and superfluid responses of the system. By comparing simulations of the extended Gross–Pitaevskii equation with experimental observations, we demonstrate that synchronization can serve as a dynamical indicator for vortex nucleation. This approach provides a complementary method to determine the critical rotation frequency for vortex formation in supersolids.
Abstract Supersolid states simultaneously feature properties typically associated with a solid and with a superfluid. Like a solid, they possess crystalline order, manifesting as a periodic modulation of the particle density; but unlike a typical solid, they also have superfluid properties, resulting from coherent particle delocalization across the system. Such states were initially envisioned in the context of bulk solid helium, as a possible answer to the question of whether a solid could have superfluid properties1–5. Although supersolidity has not been observed in solid helium (despite much effort)6, ultracold atomic gases provide an alternative approach, recently enabling the observation and study of supersolids with dipolar atoms7–16. However, unlike the proposed phenomena in helium, these gaseous systems have so far only shown supersolidity along a single direction. Here we demonstrate the extension of supersolid properties into two dimensions by preparing a supersolid quantum gas of dysprosium atoms on both sides of a structural phase transition similar to those occurring in ionic chains17–20, quantum wires21, 22 and theoretically in chains of individual dipolar particles23, 24. This opens the possibility of studying rich excitation properties25–28, including vortex formation29–31, and ground-state phases with varied geometrical structure7, 32 in a highly flexible and controllable system.
Supersolids are a fundamental quantum phase of matter where the global phase and translational symmetries are spontaneously broken.The recently discovered supersolidity in quantum gases of strongly magnetic atoms gives the opportunity to explore in depth how superfluidity and crystalline order are mixed in this fascinating phase.The dipolar supersolid is usually created from a Bose-Einstein condensate, i.e., a standard superfluid, crossing a quantum phase transition that is related to the crystallization transitions of ordinary matter.In this work, we assess experimentally and theoretically the character of the superfluidsupersolid quantum phase transition.We find that one-row supersolids can have already two types of phase transitions, discontinuous and continuous, that are reminiscent of the first-and second-order transitions predicted in the thermodynamic limit in 2D and 1D, respectively.The dimensional crossover is peculiar to supersolids, is controlled via the transverse confinement and the atom number, and can be justified on the general ground of the Landau theory of phase transitions.The quasiadiabatic crossing of a continuous phase transition opens new directions of investigation for supersolids.
Fluctuations typically destroy long-range order in two-dimensional (2D) systems, posing a fundamental challenge to the existence of exotic states like supersolids, which paradoxically combine solid-like structure with frictionless superfluid flow. While long-predicted, the definitive observation of a 2D supersolid has remained an outstanding experimental goal. Here, we report the observation of a supersolid stripe phase in a strongly dipolar quantum gas of erbium atoms confined to 2D. We directly image the periodic density modulation, confirming its global phase coherence through matter-wave interference and demonstrating its phase rigidity relevant to the low-energy Goldstone mode, consistent with numerical calculations. Through collective excitation measurements, we demonstrate the hydrodynamic behavior of the supersolid. This work highlights a novel mechanism for supersolid formation in low dimensions, and opens the door for future research on the intricate interplay between temperature, supersolidity, and dimensionality.
This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.
Rotation is a natural tool in ultracold gases to break time-reversal symmetry, yet its impact on the collective excitations of supersolids remains largely unexplored. We show theoretically that tuning the rotation frequency, rather than the interparticle interactions, can trigger the superfluid-to-supersolid transition in Bose-Einstein condensates. Computing excitation spectra in the presence of vortices and persistent currents, we uncover a vortex-driven desoftening mechanism whereby quantized vorticity elevates the gapless Goldstone mode to a finite-energy roton, restoring superfluidity. This effect results in reentrant supersolid phases as a function of rotation frequency, revealing a fundamental coupling between topological defects and crystalline order.