This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.
This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.
Two-dimensional (2D) dipolar atomic gases present unique opportunities for exploring novel quantum phases due to their anisotropic and long-range interactions. However, the behavior of strongly dipolar Bose gases in 2D remains unclear, especially when dipoles are tilted. Here, we demonstrate the creation and characterization of strongly dipolar 2D condensates in a quasi-2D harmonic trap with tunable dipole orientation. By investigating scale invariance properties through breathing collective mode measurements, we observe significant breaking of scale invariance when dipoles are tilted in-plane indicating the dominance of the nonlocal dipole-dipole interactions (DDIs) in this regime. Interestingly, the breaking of the scale invariant dynamics is accompanied by an increase in quantum fluctuations, as shown by comparison with mean-field and beyond mean-field theoretical studies. Our experiments also reveal that at critical tilt angles around 70°, stripe-type density modulations emerge, suggesting the presence of a roton spectrum in 2D, while the system still shows hydrodynamic nature with the phase-locking breathing behavior. This observation elucidates the many-body effect induced by DDIs in 2D, thus marking a crucial step toward realizing 2D supersolids and other exotic quantum phases.
Dipolar quantum gases, encompassing atoms and molecules with significant dipole moments, exhibit unique long-range and anisotropic dipole-dipole interactions (DDI), distinguishing them from systems dominated by short-range contact interactions. This review explores their behavior across dimensions, focusing on magnetic atoms in quasi-2D in comparison to 3D. In 3D, strong DDI leads to phenomena like anisotropic superfluidity, quantum droplets stabilized by Lee-Huang-Yang corrections, and supersolid states with density modulations. In 2D, we discuss a new scenario where DDI induces angle-dependent Berezinskii-Kosterlitz-Thouless transitions and potential supersolidity, as suggested by recent experimental realizations of strongly dipolar systems in quasi-2D geometries. We identify key challenges for future experimental and theoretical work on strongly dipolar 2D systems. The review concludes by highlighting how these unique 2D dipolar systems could advance fundamental research as well as simulate novel physical phenomena.
Long-range and anisotropic dipolar interactions induce complex order in quantum systems, particularly interesting in 2D where superfluidity emerges via the Berezinskii-Kosterlitz-Thouless (BKT) mechanism. We observe a superfluid phase with algebraically decaying correlation in a quasi-2D dipolar Bose gas of erbium atoms and further identify the superfluid phase transition by monitoring extended coherence. We also measure equations of state with tunable dipolar interactions. Our findings show a transition point shift due to dipole orientation, aligning with BKT transition with effective short-range interaction. However, we observe that in-plane tilted dipoles show nonlocal effects in the superfluid regime, preventing the effective short-range interaction from revealing universal behavior near the BKT critical point. We also measure anisotropic atom number fluctuations in the superfluid regime, highlighting its dipolar nature. Our results provide a foundation for understanding dipolar bosons in 2D and pave the way for investigating complex orders in dipolar superfluids.
Fluctuations typically destroy long-range order in two-dimensional (2D) systems, posing a fundamental challenge to the existence of exotic states like supersolids, which paradoxically combine solid-like structure with frictionless superfluid flow. While long-predicted, the definitive observation of a 2D supersolid has remained an outstanding experimental goal. Here, we report the observation of a supersolid stripe phase in a strongly dipolar quantum gas of erbium atoms confined to 2D. We directly image the periodic density modulation, confirming its global phase coherence through matter-wave interference and demonstrating its phase rigidity relevant to the low-energy Goldstone mode, consistent with numerical calculations. Through collective excitation measurements, we demonstrate the hydrodynamic behavior of the supersolid. This work highlights a novel mechanism for supersolid formation in low dimensions, and opens the door for future research on the intricate interplay between temperature, supersolidity, and dimensionality.
Since the achievement of quantum degeneracy in gases of chromium atoms in 2004, the experimental investigation of ultracold gases made of highly magnetic atoms has blossomed. The field has yielded the observation of many unprecedented phenomena, in particular those in which long-range and anisotropic dipole-dipole interactions (DDIs) play a crucial role. In this review, we aim to present the aspects of the magnetic quantum-gas platform that make it unique for exploring ultracold and quantum physics as well as to give a thorough overview of experimental achievements. Highly magnetic atoms distinguish themselves by the fact that their electronic ground-state configuration possesses a large electronic total angular momentum. This results in a large magnetic moment and a rich electronic transition spectrum. Such transitions are useful for cooling, trapping, and manipulating these atoms. The complex atomic structure and large dipolar moments of these atoms also lead to a dense spectrum of resonances in their two-body scattering behaviour. These resonances can be used to control the interatomic interactions and, in particular, the relative importance of contact over dipolar interactions. These features provide exquisite control knobs for exploring the few- and many-body physics of dipolar quantum gases. The study of dipolar effects in magnetic quantum gases has covered various few-body phenomena that are based on elastic and inelastic anisotropic scattering. Various many-body effects have also been demonstrated. These affect both the shape, stability, dynamics, and excitations of fully polarised repulsive Bose or Fermi gases. Beyond the mean-field instability, strong dipolar interactions competing with slightly weaker contact interactions between magnetic bosons yield new quantum-stabilised states, among which are self-bound droplets, droplet assemblies, and supersolids. Dipolar interactions also deeply affect the physics of atomic gases with an internal degree of freedom as these interactions intrinsically couple spin and atomic motion. Finally, long-range dipolar interactions can stabilise strongly correlated excited states of 1D gases and also impact the physics of lattice-confined systems, both at the spin-polarised level (Hubbard models with off-site interactions) and at the spinful level (XYZ models). In the present manuscript, we aim to provide an extensive overview of the various related experimental achievements up to the present.
Ultracold dilute atomic gases are highly controllable systems whose properties are fundamentally determined by the interatomic interactions.In typical experiments on ultra cold gases particles interact dominantly via a short-range isotropic potential.However, during the last years a new generation of experiments is starting to explore systems, where an additional interaction, the long-range and anisotropic dipole-dipole interaction plays a significant or possibly dominant role.The effects induced by the anisotropy of the dipole-dipole interaction are crucially enhanced if the dipolar gas is confined in a deep optical lattice.In this thesis we study novel phenomena in such systems of dipolar gases in deep optical lattices.The nonlocal nonlinearity introduced by the dipole-dipole interaction plays a crucial role in the physics of dipolar Bose-Einstein condensates.In particular, it may distort significantly the stability of straight vortex lines.Remarkably, in the presence of a periodic potential along the vortex line, the spectrum of transverse modes shows a roton-like minimum, which eventually destabilizes the straight vortex when the BEC as a whole is still stable, opening the possibility for new scenarios for vortex line configurations in dipolar gases.We have analyzed this instability, and showed that it leads to a second-order-like phase transition from a straight vortex line into novel helical or snake-like configurations, depending on the dipole orientation.Strong 1D lattices usually lead to unconnected two-dimensional gases.The long-range character of the dipole-dipole interactions leads to a novel scenario where non-overlapping gases at different sites may interact significantly.We show that the excitations of non-overlapping condensates in 1D optical lattices acquire a band-like character, being collectively shared by different sites.In particular, the hybridization of the modes significantly enhances the rotonization of the excitations, and may induce roton-instability.We discuss the observability of this effect in on-going experiments.Fermionic polar molecules in deep 1D optical lattices may form selfassembled filaments when the electric dipoles are oriented along the lattice axis.These composites are bosons or fermions depending on the number of molecules per chain, leading to a peculiar and complex Bose-Fermi mixture, vi which we discuss in detail for the simplest case of a three-well potential.We show that the interplay between filament binding energy, transverse filament modes, and trimer Fermi energy leads to a rich variety of possible scenarios ranging from a degenerate Fermi gas of trimers to a binary mixture of two different types of bosonic dimers.We study the intriguing zero temperature and finite temperature physics of these composites for the particular case of an ideal filament gas loaded in 1D sites, and discuss possible methods to probe these chain mixtures.