High-energy scattering spectroscopy is a widely established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of density-modulated states within a classical-field approach. I focus on the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. Using relevant Ans\"atze for the fields of dipolar supersolid states in these regimes, I specify and illustrate the scaling laws relating the three observables. This work was first prompted to develop an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. Beyond this specific application, this works provides a simple and general framework to describe density-modulated states and in particular the intriguing case of supersolids. It describes key properties characterizing the supersolid order and highlights possibilities for probing such properties based on high-energy scattering response.
High-energy scattering spectroscopy is a widely established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of density-modulated states within a classical-field approach. I focus on the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. Using relevant Ans"atze for the fields of dipolar supersolid states in these regimes, I specify and illustrate the scaling laws relating the three observables. This work was first prompted to develop an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. Beyond this specific application, this works provides a simple and general framework to describe density-modulated states and in particular the intriguing case of supersolids. It describes key properties characterizing the supersolid order and highlights possibilities for probing such properties based on high-energy scattering response.
High-energy scattering spectroscopy is a widely-established technique for probing the characteristic properties of complex physical systems. Motivated by the recent observation of long-sought supersolid states in dipolar quantum Bose gases, I investigate the general relationships existing between the density contrast, the superfluid fraction, and the response to a high-energy scattering probe of such exotic states within a simple model. I focus on the scaling laws relating these three observables in the two extreme regimes of shallow and deep supersolids, which are of particular interest in describing the phase transitions of the supersolid to a uniform superfluid and an incoherent crystal state, respectively. I illustrate and specify the general formulae using relevant ansatzes for the supersolid states of dipolar gases in these regimes. This work brings an intuitive understanding of a concomitant study based on experiments and mean-field numerical simulations. It generally highlights new possibilities for probing supersolid states while providing a simple framework to describe such intriguing states.
We develop a linear-response theory to provide a unified description of two recent spectroscopy protocols for probing one-dimensional supersolid states realized in cold-atom systems. Both protocols involve applying a periodic optical potential to excite the supersolid and determine its excitation frequencies and density response characteristics. This information can be used to estimate the superfluid fraction. We validate our linear-response theory against nonlinear mean-field simulations of the dynamics for ring, box, and harmonically trapped cases. A key focus is the behavior at the band edge---the regime occurring when the optical potential used to excite the system has a wavelength that is twice the value of the supersolid lattice constant. Here symmetry can be used to selectively excite a mode from one of the two low-energy gapless excitation bands. We also consider the application of the spectroscopy protocols to determine the superfluid fraction, showing the relationship to hydrodynamic theory and a Josephson-junction array model. Our analysis and results suggest that the phase protocol we introduce has potential advantages for experimental application over the density protocol.
Bose-Einstein condensation is a macroscopic quantum phenomenon where cooling down a gas of bosonic particles to ultracold temperatures results in the macroscopic occupation of the lowest energy state. This new state of matter has been used as a quantum simulator of many-body phenomena and theories due to its extreme tunability and controllability. An important example of such a many-body system is the polaron which, in its most general form, describes an impurity interacting with a bosonic bath. In the case of ultracold Bose gases, the impurity interacts with and is dressed by the Bogoliubov excitations of the gas. A supersolid is a state of matter that exhibits both superfluidity and crystalline order, which are seemingly irreconcilable properties. It has recently been observed in dipolar ultracold Bose gases, where it arises from the long-range anisotropic dipole-dipole interactions, and also other systems. The breaking of both translational symmetry and gauge symmetry results in multiple excitation modes in the supersolid. In this thesis, the charged Bose polaron and an impurity in a dipolar ultracold Bose gas exhibiting supersolidity (the supersolid Bose polaron) are studied. The ground-state properties of the charged Bose polaron are discussed using a variational path-integral approach. Absorption spectroscopy is proposed as a probe of the charged Bose polaron, and the optical response is studied for weak impurity-boson interactions. Next, the one-dimensional dipolar supersolid Bose polaron is investigated where multiple approaches are used for the derivation of the ground-state properties. The study of the polaron problem with a supersolid background is of particular interest because of the rich excitation spectrum of the supersolid. Interesting phenomena, such as possible localization of the polaron to a single droplet for strong interactions, are observed. The absorption spectrum of a charged impurity in the supersolid is also derived, which, because of the different excitation modes of the supersolid, shows multiple peaks from which information such as the superfluid fraction may be obtained.
In the short time since the first observation of supersolid states of ultracold dipolar atoms, substantial progress has been made in understanding the zero-temperature phase diagram and low-energy excitations of these systems. Less is known, however, about their finite-temperature properties, particularly relevant for supersolids formed by cooling through direct evaporation. Here, we explore this realm by characterizing the evaporative formation and subsequent decay of a dipolar supersolid by combining high-resolution in-trap imaging with time-of-flight observables. As our atomic system cools toward quantum degeneracy, it first undergoes a transition from thermal gas to a crystalline state with the appearance of periodic density modulation. This is followed by a transition to a supersolid state with the emergence of long-range phase coherence. Further, we explore the role of temperature in the development of the modulated state.
This thesis discusses the experiments on 2D dipolar Bose gas of ultracold erbium atoms. Long-range and anisotropic dipole-dipole interaction induces complex orders in quantum many-body systems. Highly magnetic lanthanide atoms such as dysprosium and erbium have the largest magnetic moment in the periodic table, which has attracted significant attention in the past decades. Starting from quantum degenerate dysprosium and erbium atoms, exotic phases like quantum droplets, supersolid, dipolar quantum solid in the Hubbard regime have been studied. However, the 2D dipolar superfluid still remains understudied, despite being theoretically discussed for over two decades. Although tremendous theoretical proposals predict different phenomena in 2D dipolar superfluids, our first interest is to know how the superfluidity emerges in the 2D dipolar gases at finite temperatures. Our observations suggest that the superfluid transition can be well described by the Berezinskii-Kosterlitz-Thouless transition with an effective contact interaction as a function of dipolar orientation. With the 2D dipolar superfluid with strong DDI, we characterized the elementary excitation of the matter: the collective breathing mode. Our measurements establish how the competition between local and nonlocal interaction in strongly dipolar 2D superfluid retains quasi-scale invariance or strongly breaks scale invariance. By further searching the interaction parameters, we created stripes with global coherence, which are the first supersolid stripes in 2D. Experiments including measuring density fluctuation, coherence, and collective mode have been performed to understand the 2D supersolid. At last, we also observe unconventional light scattering from round-disk dipolar BECs, which provides new possibilities for atom optics.
Abstract Supersolid states simultaneously feature properties typically associated with a solid and with a superfluid. Like a solid, they possess crystalline order, manifesting as a periodic modulation of the particle density; but unlike a typical solid, they also have superfluid properties, resulting from coherent particle delocalization across the system. Such states were initially envisioned in the context of bulk solid helium, as a possible answer to the question of whether a solid could have superfluid properties1–5. Although supersolidity has not been observed in solid helium (despite much effort)6, ultracold atomic gases provide an alternative approach, recently enabling the observation and study of supersolids with dipolar atoms7–16. However, unlike the proposed phenomena in helium, these gaseous systems have so far only shown supersolidity along a single direction. Here we demonstrate the extension of supersolid properties into two dimensions by preparing a supersolid quantum gas of dysprosium atoms on both sides of a structural phase transition similar to those occurring in ionic chains17–20, quantum wires21, 22 and theoretically in chains of individual dipolar particles23, 24. This opens the possibility of studying rich excitation properties25–28, including vortex formation29–31, and ground-state phases with varied geometrical structure7, 32 in a highly flexible and controllable system.