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Hybrid 3He and alkali magnetometry techniques for fundamental physics experiments

C. Abel

Published Mar 6, 2020• 0 citations
OpenAlex

Abstract

Since the 1950s, experiments searching for the neutron electric dipole moment have increased in sensitivity by six orders of magnitude. Yet, the current experimental sensitivity lies well above that predicted from standard model calculations. Corrections from physics beyond the standard model increase the predicted size of the nEDM, resulting in the nextgeneration of experiments hovering tantalisingly close to the detection sensitivity, to either verify or quash standard model extensions. One such experiment, n2EDM, currently in the commissioning stage at the Paul Scherrer Institute in Switzerland, hopes to measure the nEDM with a sensitivity improvement over its predecessor. This thesis details the design, measurement and analysis of hybrid 3He/alkali magnetometers for both accurate and precise magnetic field readings at low and zero fields, crucial for the development of ever-more sensitive fundamental physics searches. The work exploits the precise nature of alkali (87Rb and 133Cs) magnetometry techniques to measure the simultaneous Larmor precession of polarised 3He, avoiding light shifts commonly associated with optically pumped magnetometers. The first part of this work demonstrates the use of a hybrid 3He/87Rb magnetometer for the minimisation of remnant fields in a magnetically shielded environment, resulting in absolute low-field readings below 5 pT. Furthermore, the hybrid magnetometer was shown to be applicable for the reduction of gradient fields by optimising the effective 3He T2 time. This new technique represents a convenient and consistent way to achieve a near-zero magnetic field environment for precision experiments. Second, a new measurement technique was demonstrated using a hybrid 3He/133Cs magnetometer in a 1 µT field, placing experimental limits on the coupling of axion-like dark matter to nucleons. The measurement excluded axion coupling strength to 2:5 x 10-1 GeV-1 for axion masses between 10-20 to 10-17 eV at the 95% level. With the resulting exclusion region weaker than previous measurements, possible improvements to the apparatus should drive the development of a low-cost long-term axion interaction search.

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Since the 1950s, experiments searching for the neutron electric dipole moment have increased in sensitivity by six orders of magnitude. Yet, the current experimental sensitivity lies well above that predicted from standard model calculations. Corrections from physics beyond the standard model increase the predicted size of the nEDM, resulting in the nextgeneration of experiments hovering tantalisingly close to the detection sensitivity, to either verify or quash standard model extensions. One such experiment, n2EDM, currently in the commissioning stage at the Paul Scherrer Institute in Switzerland, hopes to measure the nEDM with a sensitivity improvement over its predecessor. This thesis details the design, measurement and analysis of hybrid 3He/alkali magnetometers for both accurate and precise magnetic field readings at low and zero fields, crucial for the development of ever-more sensitive fundamental physics searches. The work exploits the precise nature of alkali (87Rb and 133Cs) magnetometry techniques to measure the simultaneous Larmor precession of polarised 3He, avoiding light shifts commonly associated with optically pumped magnetometers. The first part of this work demonstrates the use of a hybrid 3He/87Rb magnetometer for the minimisation of remnant fields in a magnetically shielded environment, resulting in absolute low-field readings below 5 pT. Furthermore, the hybrid magnetometer was shown to be applicable for the reduction of gradient fields by optimising the effective 3He T2 time. This new technique represents a convenient and consistent way to achieve a near-zero magnetic field environment for precision experiments. Second, a new measurement technique was demonstrated using a hybrid 3He/133Cs magnetometer in a 1 µT field, placing experimental limits on the coupling of axion-like dark matter to nucleons. The measurement excluded axion coupling strength to 2:5 x 10-1 GeV-1 for axion masses between 10-20 to 10-17 eV at the 95% level. With the resulting exclusion region weaker than previous measurements, possible improvements to the apparatus should drive the development of a low-cost long-term axion interaction search.
Axions are a compelling dark matter candidate suggested by theories beyond the Standard Model. The predicted axion-electron coupling and the resulting pseudomagnetic field allow for laboratory axion searches. Here we report an experimental axion search via a superconductor-spin hybrid magnetometer. A state-of-the-art broadband magnetometer with a sensitivity of sub-100 aT/Hz1/2^{1/2}1/2 at tens of kHz has been realized by coupling a ferrite spin sensor to a readout system based on a superconducting quantum interference device. The most stringent terrestrial constraints on the axion-electron coupling have been established in the frequency range 5$\sim$60 kHz. In the future, an improvement on the constraints of more than 4 orders of magnitude is foreseeable through arrays of superconductor-spin hybrid magnetometers with optimized designs. This work demonstrates the potential of superconductor-spin hybrid magnetometers in high-precision magnetic field sensing and the study of fundamental physics.
The development of an experimental apparatus to produce Bose-Einstein condensates (BECs) of ⁸⁷Rb atoms and their application to magnetometry are discussed. Optical detection of atomic Larmor precession is a widely explored method for high-sensitivity measurements of magnetic fields. In this context, short laser/atom interaction time, atomic thermal diffusion and decoherence effects are among the main limitations. In this thesis, we overcome such problems by using spin-polarised ⁸⁷Rb ultra-cold atoms as the sensing element. After the atoms are polarised, a resonant pulse of radio-frequency excites Larmor precession, which is sensitive to external magnetic fields. By measuring the perturbations of the radio-frequency induced spin precession, information on the magnetic fields of interest. This is achieved by monitoring the polarisation plane’s rotation of a linearly polarised resonant laser probe. In the first part of this thesis, the building and optimisation of a laser-cooling set up to obtain a BEC in a hybrid trap is reported. In order to achieve the Phase Space Density (PSD) required for BEC, several different stages of trapping and cooling are necessary. Each phase has been implemented and optimised. The first step consists in the magneto-optical trap (MOT). Here a velocity dependent damping force and a spatially dependent confining force give the largest changes in PSD. Then atoms are loaded into a hybrid trap obtained by overlapping a quadrupole magnetic potential and a far detuned optical crossed dipole trap. The final stage for the condensation consists of forced evaporative cooling, both via magnetic and optical evaporation. In the second part of the thesis, a general overview of the principles of optical atomic magnetometry is provided and the advantages of using ultra-cold atoms with respect to conventional thermal vapours are discussed. The implementation, operation and a preliminary characterisation of the ultra-cold atom magnetometer are described along with the preliminary results collected. Finally, a plan for future improvements of its sensitivity is presented.
Direct detection of dark matter remains an important outstanding problem since abundant astrophysical evidence points towards its existence, but no experiment has succeeded in detecting it. Axions and axion-like-particles are some of the most compelling candidates for dark matter given their appearance in many theories of physics beyond the Standard Model and their relatively unexplored parameter space compared to other candidates. Recently, the Cosmic Axion Spin Precession Experiment-Electric (CASPEr-e) has used nuclear magnetic resonance (NMR) to search for effective magnetic fields created by axionic dark matter. By decreasing technical noise sources, CASPEr-e is projected to reach the standard quantum limit where spin projection noise is the dominant noise source limiting sensitivity. However, some axion models predict axion couplings to normal matter that would be too small for even a quantum limited CASPEr-e experiment to detect. This creates a need for surpassing the spin projection noise limit in NMR dark matter searches. In this thesis, I explore the prospects for surpassing the quantum limit in NMR by using spin squeezed states, entangled states with variance in one projection reduced below the standard quantum limit. First, I propose an experimental scheme for generating squeezed states by coupling the spins to an off-resonant circuit to create a One-Axis-Twist Hamiltonian. Then, using exact results and numerical simulations, I determine the amount of squeezing that can be achieved given decoherence and noise. Next, I perform modeling to show that squeezing can accelerate dark matter searches despite earlier results that argued squeezing cannot improve experimental sensitivity when subject to decoherence. Finally, I apply these results to the CASPEr-e experiment and show that at axion frequencies near 100MHz, squeezing can speed up the experiment by a factor of up to 30, corresponding to a sensitivity improvement by a factor of over 5.
The ability to measure the magnetic fields around celestial bodies enables various insights into processes and phenomena deep within such bodies.The use of magnetometry in space missions dates back to the 1950s, and a number of different technologies have been used to measure these fields, ranging from fluxgates to Anisotropic Magneto Resistance (AMR) sensors.Optically-pumped magnetometers (OPMs) represent the state-of-the-art in magnetic field sensitivity. 1 Such sensors rely upon the interaction of laser light to spin polarise a warm vapour of neutral atoms.Detecting the precession of these spins, again with laser light, is a direct way to measure a magnetic field and is relatable to fundamental constants.Improvements in quantum technology within the last decade have led to the miniaturisation of these sensors.We have now reached the point where compact, lightweight, and low power devices offer greater sensitivity to magnetic fields than any other technology.In this work, we identify the following four key space application areas in which OPMs may offer significant advantages over existing technologies: Environments in which high sensitivity is needed at low magnetic fields (10s of nT), full vector read-out with high directional sensitivity and reduced SWaP compared to helium magnetometers, miniaturised and lightweight scalar magnetometers to complement vector fluxgate measurements, vector or scalar sensors that need high (40 dB) gradiometer performance.This work identifies OPM configurations for each area and makes a first estimate of size, weight and power requirements for each.By enabling improvements in magnetic field sensitivity, this represents an exciting prospect for precision magnetic field measurements while also saving mass and reducing complexity.
We demonstrate the use of a hybrid 3He/87 magnetometer to measure absolute magnetic fields in the pT range. The measurements were undertaken by probing time-dependent 3He magnetisation using 87Rb zero-field magnetometers. Measurements were taken to demonstrate the use of the magnetometer in cancelling residual fields within a magnetic shield. It was shown that the absolute field could be reduced to the 10 pT level by using field readings from the magnetometer. Furthermore, the hybrid magnetometer was shown to be applicable for the reduction of gradient fields by optimising the effective 3He T2 time. This procedure represents a convenient and consistent way to provide a near zero magnetic field environment which can be potentially used as a base for generating desired magnetic field configurations for use in precision measurements.
We demonstrate the use of a hybrid 3He/87 magnetometer to measure absolute magnetic fields in the pT range. The measurements were undertaken by probing time-dependent 3He magnetisation using 87Rb zero-field magnetometers. Measurements were taken to demonstrate the use of the magnetometer in cancelling residual fields within a magnetic shield. It was shown that the absolute field could be reduced to the 10 pT level by using field readings from the magnetometer. Furthermore, the hybrid magnetometer was shown to be applicable for the reduction of gradient fields by optimising the effective 3He T2 time. This procedure represents a convenient and consistent way to provide a near zero magnetic field environment which can be potentially used as a base for generating desired magnetic field configurations for use in precision measurements.