Axions are a compelling dark matter candidate suggested by theories beyond the Standard Model. The predicted axion-electron coupling and the resulting pseudomagnetic field allow for laboratory axion searches. Here we report an experimental axion search via a superconductor-spin hybrid magnetometer. A state-of-the-art broadband magnetometer with a sensitivity of sub-100 aT/Hz$^{1/2}$ at tens of kHz has been realized by coupling a ferrite spin sensor to a readout system based on a superconducting quantum interference device. The most stringent terrestrial constraints on the axion-electron coupling have been established in the frequency range 5$\sim$60 kHz. In the future, an improvement on the constraints of more than 4 orders of magnitude is foreseeable through arrays of superconductor-spin hybrid magnetometers with optimized designs. This work demonstrates the potential of superconductor-spin hybrid magnetometers in high-precision magnetic field sensing and the study of fundamental physics.
Axions are a compelling dark matter candidate suggested by theories beyond the Standard Model. The predicted axion-electron coupling and the resulting pseudomagnetic field allow for laboratory axion searches. Here we report an experimental axion search via a superconductor-spin hybrid magnetometer. A state-of-the-art broadband magnetometer with a sensitivity of sub-100 aT/Hz1/2 at tens of kHz has been realized by coupling a ferrite spin sensor to a readout system based on a superconducting quantum interference device. The most stringent terrestrial constraints on the axion-electron coupling have been established in the frequency range 5∼60 kHz. In the future, an improvement on the constraints of more than 4 orders of magnitude is foreseeable through arrays of superconductor-spin hybrid magnetometers with optimized designs. This work demonstrates the potential of superconductor-spin hybrid magnetometers in high-precision magnetic field sensing and the study of fundamental physics.
We propose a magnetic resonance force microscopy (MRFM) search for axion dark matter around 1 GHz. The experiment leverages the axion's derivative coupling to electrons, which induces an effective A.C. magnetic field on a sample of electron spins polarized by a D.C. magnetic field and a micromagnet. A second pump field at a nearby frequency enhances the signal, with the detuning matched to the resonant frequency of a magnet-loaded mechanical oscillator. The resulting spin-dependent force is detected with hih sensitivity via optical interferometry. Accounting for the relevant noise sources, we show that current technology can be used to put constraints competitive with those from laboratory experiments with just a minute of integration time. Furthermore, varying the pump field frequency and D.C. magnetic field allows one to scan the axion mass. Finally, we explore this setup's capability to put constraints on other dark matter - Standard Model couplings.
Conventional nuclear magnetic resonance searches for the galactic axion wind lose sensitivity at low frequencies due to the unfavourable scaling of inductive readout. Here, we propose a hybrid architecture where the hyperfine interaction transduces axion-driven nuclear precession into a high-bandwidth electron-spin readout channel. We demonstrate analytically that this dispersive upconversion preserves the specific sidereal and annual modulation signatures required to distinguish dark matter signals from instrumental backgrounds. When instantiated in a silicon 209Bi donor platform, the hybrid sensor is projected to outperform direct nuclear detection by more than an order of magnitude over the 10−16−10−10eV wide mass range. With collective enhancement, the design reaches a 5σ sensitivity to DFSZ axion-nucleon couplings within one year, establishing hyperfine-mediated sensing as a competitive path for compact, solid-state dark matter searches.
Direct detection of dark matter remains an important outstanding problem since abundant astrophysical evidence points towards its existence, but no experiment has succeeded in detecting it. Axions and axion-like-particles are some of the most compelling candidates for dark matter given their appearance in many theories of physics beyond the Standard Model and their relatively unexplored parameter space compared to other candidates. Recently, the Cosmic Axion Spin Precession Experiment-Electric (CASPEr-e) has used nuclear magnetic resonance (NMR) to search for effective magnetic fields created by axionic dark matter. By decreasing technical noise sources, CASPEr-e is projected to reach the standard quantum limit where spin projection noise is the dominant noise source limiting sensitivity. However, some axion models predict axion couplings to normal matter that would be too small for even a quantum limited CASPEr-e experiment to detect. This creates a need for surpassing the spin projection noise limit in NMR dark matter searches. In this thesis, I explore the prospects for surpassing the quantum limit in NMR by using spin squeezed states, entangled states with variance in one projection reduced below the standard quantum limit. First, I propose an experimental scheme for generating squeezed states by coupling the spins to an off-resonant circuit to create a One-Axis-Twist Hamiltonian. Then, using exact results and numerical simulations, I determine the amount of squeezing that can be achieved given decoherence and noise. Next, I perform modeling to show that squeezing can accelerate dark matter searches despite earlier results that argued squeezing cannot improve experimental sensitivity when subject to decoherence. Finally, I apply these results to the CASPEr-e experiment and show that at axion frequencies near 100MHz, squeezing can speed up the experiment by a factor of up to 30, corresponding to a sensitivity improvement by a factor of over 5.
Since the 1950s, experiments searching for the neutron electric dipole moment have increased in sensitivity by six orders of magnitude. Yet, the current experimental sensitivity lies well above that predicted from standard model calculations. Corrections from physics beyond the standard model increase the predicted size of the nEDM, resulting in the nextgeneration of experiments hovering tantalisingly close to the detection sensitivity, to either verify or quash standard model extensions. One such experiment, n2EDM, currently in the commissioning stage at the Paul Scherrer Institute in Switzerland, hopes to measure the nEDM with a sensitivity improvement over its predecessor. This thesis details the design, measurement and analysis of hybrid 3He/alkali magnetometers for both accurate and precise magnetic field readings at low and zero fields, crucial for the development of ever-more sensitive fundamental physics searches. The work exploits the precise nature of alkali (87Rb and 133Cs) magnetometry techniques to measure the simultaneous Larmor precession of polarised 3He, avoiding light shifts commonly associated with optically pumped magnetometers. The first part of this work demonstrates the use of a hybrid 3He/87Rb magnetometer for the minimisation of remnant fields in a magnetically shielded environment, resulting in absolute low-field readings below 5 pT. Furthermore, the hybrid magnetometer was shown to be applicable for the reduction of gradient fields by optimising the effective 3He T2 time. This new technique represents a convenient and consistent way to achieve a near-zero magnetic field environment for precision experiments. Second, a new measurement technique was demonstrated using a hybrid 3He/133Cs magnetometer in a 1 µT field, placing experimental limits on the coupling of axion-like dark matter to nucleons. The measurement excluded axion coupling strength to 2:5 x 10-1 GeV-1 for axion masses between 10-20 to 10-17 eV at the 95% level. With the resulting exclusion region weaker than previous measurements, possible improvements to the apparatus should drive the development of a low-cost long-term axion interaction search.
One of the areas of research of the Superconducting Quantum Systems and Materials (SQMS) center is the application of quantum sensing to fundamental physics searches, demonstrating that quantum sensors can greatly improve the sensitivity of experiments searching for Beyond the Standard Model (BSM) physics, or performing high-precision measurements. Theorists have developed many ideas for BSM physics that would result in interactions that can in principle be detected, but with signals small enough that they haven t been observed yet. In this field, the capability to lower the detector s thermal noise to few or dozens of mK, and to use QIS technologies such as Josephson Parametric Amplifiers and photon counters (in-situ or itinerant) enable us to reach unprecedented sensitivities and faster scan rates. Here is presented an overview of the quantum sensing efforts at SQMS [1], focusing on theoretical advancements and experimental searches for Dark Sector particles (as dark matter candidates and not), gravitational waves, and precision measurements. The experiments conducted, or under preparation, include axion dark matter (DM) [2, 3], dark photon DM searches [4,5], light-shining-through-wall experiments [6], cavity-based searches for high frequency gravitational waves [7], and measurements of the electron magnetic moment [8]. [1] Berlin, A., et al. "Searches for new particles, dark matter, and gravitational waves with SRF cavities." arXiv preprint arXiv:2203.12714 (2022). [2] Giaccone, B., et al. "Design of axion and axion dark matter searches based on ultra high Q SRF cavities." arXiv preprint arXiv:2207.11346 (2022). [3] Braggio, C., et al. "Quantum-enhanced sensing of axion dark matter with a transmon-based single microwave photon counter." arXiv preprint arXiv:2403.02321 (2024). [4] Fan, X., et al. "One-electron quantum cyclotron as a milli-eV dark-photon detector." Physical review letters 129.26 (2022): 261801. [5] Cervantes, R., et al. "Deepest sensitivity to wavelike dark photon dark matter with superconducting radio frequency cavities." Physical Review D 110.4 (2024): 043022. [6] Romanenko, A., et al. "Search for dark photons with superconducting radio frequency cavities." Physical review letters 130.26 (2023): 261801. [7] Berlin, A., et al. "Electromagnetic cavities as mechanical bars for gravitational waves." Physical Review D 108.8 (2023): 084058. [8] Fan, X., et al. "Measurement of the electron magnetic moment." Physical review letters 130.7 (2023): 071801.
Searches for axion and axionlike dark matter based on solid-state spin qubits are fundamentally limited by strong longitudinal dephasing, which rapidly suppresses the sensitivity gains offered by entanglement. Here we show that quantum error correction (QEC) can substantially enhance axion search sensitivity in realistic semiconductor spin qubit platforms by mitigating this dominant noise source. By integrating an optimally chosen repetition code QEC with logical GHZ block entanglement, we derive closed-form expressions for the quantum Fisher information that explicitly incorporate the finite coherence time of the axion field. Our analysis demonstrates that modest QEC cycle frequencies are sufficient to significantly reduce the effective dephasing rate, thereby restoring a broad parameter regime in which entanglement-enhanced sensing surpasses the standard quantum limit. Projecting these results onto CMOS-compatible device parameters, we find that QEC-protected entangled sensing can revive otherwise inaccessible quantum advantages, yielding up to order-of-magnitude improvements in sensitivity to the axion-electron coupling gae. These results establish a practical and theoretically controlled pathway for using QEC to improve qubit array searches for physics beyond the Standard Model.