Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.
Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.
Ultracold atomic gases with tunable interactions offer an ideal platform for studying interacting quantum matter. While the few- and many-body physics are generally complex and intractable, the problem can be greatly simplified in an atomic gas by a controlled separation of relevant length and energy scales. Precise control of experimental parameters, via Feshbach resonances, optical potentials and radio-frequency radiation, enables deterministic measurements of few-body physics, including universal physics and the Efimov effect. In this thesis, I present our recent studies on precisely measuring two- and three-body physics in an ultracold Bose gas. I begin by describing our new apparatus used for generating and studying ultracold 39K gas samples. Then, I focus on our precision spectroscopy of Feshbach dimer binding energies, spanning three orders of magnitude and with sub-kilohertz resolution. These measurements enable us to locate a Feshbach resonance and determine scattering length values with unprecedented accuracy. Finally, I present our precise measurements locating an exotic three-body state, specifically the Efimov ground state. We find that the trimer state location significantly deviates from the value predicted by van der Waals universality. Due to small experimental and systematic uncertainties, our measurement is the strongest evidence of departure from the universal value and is the first observed deviation near a Feshbach resonance of intermediate strength.
We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).
We create weakly bound Feshbach molecules in ultracold Fermi gas 40 K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.
We create weakly bound Feshbach molecules in ultracold Fermi gas 4~K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency （RF） technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.
The susceptibility of ultracold gases to precise manipulation via external fields makes them ideal systems to study fundamental quantum mechanical phenomena. Various regimes, which are not possible to reach in condensed matter or nuclear physics, can be probed with these quantum gases. Especially the tunability of the interactions and confining potentials make that these ultracold gases offer unique possibilities to explore and study universal behavior. The tunability of the dominant two-body interactions in dilute ultracold atomic gases stems from the presence of Feshbach resonances. Via these resonances pairs of ultracold atoms can be associated to form ultracold molecules. In fact, measurements of Feshbach resonance positions can be used to reveal part of the underlying molecular structure. Vica versa, accurate molecular Born-Oppenheimer potentials can be used as input for full numerical coupled-channels calculations to reliably predict Feshbach resonances. For most of the heteronuclear mixtures currently studied however, the relevant molecular potentials are not accurate enough. As the coupled-channels method is often too elaborate and too time consuming to be used to fit the measured data to enable the construction of more accurate potentials, a need for accurate models which complement this established method is created. In this thesis we have developed a simplified model for resonant scattering of two ultracold atoms which fulfills this need. The asymptotic bound-state model (ABM) is a hierarchical model which can be systematically increased in complexity and accuracy. In its most simple form, the ABM only needs two parameters to predict the position and strength of Feshbach resonances: Two binding energies corresponding to the least bound state of the two molecular potentials involved. We demonstrate that this model, although it is solely based on bound states, can incorporate threshold effects. Additionally, the model can be extended to include: Multiple vibrational levels, overlapping resonances, and magnetic dipole-dipole interactions. This versatile model allows for a description of Feshbach resonances in a large variety of systems without accurate knowledge of the relevant molecular Born-Oppenheimer potentials. Being computationally light, the ABM can be used to analyze measurements of Feshbach resonances and hereby expose the basic underlying molecular structure. Additionally, the ABM is well suited to map out all available Feshbach resonances in a system. This ability is particularly useful when an optimal resonance is required for a certain experiment. For the 6Li-40K mixture we have utilized this ability to experimentally observe a strong Feshbach resonance which offers promising perspectives to reach the strongly interacting universal regime in a mass-imbalanced Fermi gas. By analyzing the various inelastic decay processes and the accuracy of the ab initio Born-Oppenheimer potentials, we predict a strong resonance in a mixture of metastable bosonic and fermionic helium atoms. For the homonuclear (bosonic as well as fermionic) helium gas we do not find strong resonances. For an ultracold gas of 40K atoms, an elaborate combined theoretical and experimental effort is presented to map out the Feshbach resonance structure. On the experimental side we observed 36 Feshbach resonances, 31 of which where observed for the first time. These observations are in excellent agreement with coupled-channels calculations which use unmodified Born-Oppenheimer potentials as input. On the theoretical side, we present a comparison between different simplified models of resonance scattering and the full numerical coupled-channels calculations. We have developed the resonant state model (RSM) to describe the resonant scattering of two ultracold atoms. This model is founded on resonant states, the natural (eigen) frequencies of the two-body system, and their non-trivial properties. Threshold effects are implicitly build into the RSM. The RSM can describe the effect of the continuum of scattering states, states which are neglected in the ABM, on the position and strength of a Feshbach resonance by only a few resonant states. Especially when a low-energy resonance is embedded in the continuum of scattering states, the effect of these states on the Feshbach resonance cannot be neglected. The RSM can be viewed as the natural generalization of the ABM. As the RSM can be based on just a few resonant states, it retains the computational simplicity of the ABM. Using the tunability of two-body interactions induced by a Feshbach resonance, we describe a crossover for a rotating Fermi gas between two strongly-correlated many-body states. We demonstrate that the correlation induced long-range interaction will shift the crossover with respect to the non-rotating case.
This thesis presents experiments exploring Feshbach molecules and Efimov trimers in an ultracold Bose-Fermi atomic gas mixture of 40K and 87Rb. These bound states are accessed via scattering resonances, called Fano-Feshbach resonances, which arise as a consequence of a bound state being tuned through degeneracy with the threshold energy of colliding atoms. In addition to allowing the tunability of interactions, the Fano-Feshbach resonance allows for a weakly bound molecule state, called the Feshbach molecule state, to be populated. The efficiency of conversion to the Feshbach molecule state depends upon the rate with which the bound state energy is swept through degeneracy with atomic threshold energy. In regions of large scattering lengths, three-body bound states, called Efimov states, also influence inelastic Bose-Bose-Fermi collisions and boson+molecule collisions in our system. The work presented in this thesis utilizes a magnetically tunable Fano-Feshbach resonance to study Feshbach molecule creation in the perturbative limit (the limit of fast magnetic-field sweeps) and the saturated limit (the limit of slow sweeps), where a phenomenological model is applied to understand the conversion efficiency as well as the quantum degeneracy of the molecules. In addition, I present a study of boson+molecule collision rates and Bose-Bose-Fermi collision rates in order to observe signatures of Efimov states and compare against results in the gas mixture 41K-87Rb to address the question of universality of the three-body parameter in heteronuclear gas mixtures.