Chinese Physics B

Radio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gas

Lianghui Huang, Pengjun Wang, Zhengkun Fu, Jing Zhang

Published Jan 1, 2014• 6 citations

Abstract

We create weakly bound Feshbach molecules in ultracold Fermi gas 40 K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.

DOI: 10.1088/1674-1056/23/1/013402

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Chinese Physics B

Radio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gas

Lianghui Huang, Pengjun Wang, Zhengkun Fu, Jing Zhang

Published Jan 1, 2014• 6 citations

Publisher

Abstract

DOI: 10.1088/1674-1056/23/1/013402

Related papers

黄良辉, 王鹏军, 付正坤 +1 more

We create weakly bound Feshbach molecules in ultracold Fermi gas 4~K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency （RF） technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.We create weakly bound Feshbach molecules in ultracold Fermi gas 4~K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency （RF） technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.

中国物理B：英文版Jan 1, 20140 citations

Accounting for Confinement Shifts on the Binding Energies of 39K Feshbach Molecules

Jared Popowski

Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.

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Precise Characterization of Li6 Feshbach Resonances Using Trap-Sideband-Resolved RF Spectroscopy of Weakly Bound Molecules

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We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).

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We report on the formation of ultracold weakly bound Feshbach molecules of 23Na40K, the first fermionic molecule that is chemically stable in its absolute ground state. The lifetime of the nearly degenerate molecular gas exceeds 100 ms in the vicinity of the Feshbach resonance. The measured dependence of the molecular binding energy on the magnetic field demonstrates the open-channel character of the molecules over a wide field range and implies significant singlet admixture. This will enable efficient transfer into the singlet vibrational ground state, resulting in a stable molecular Fermi gas with strong dipolar interactions.We report on the formation of ultracold weakly bound Feshbach molecules of 23Na40K, the first fermionic molecule that is chemically stable in its absolute ground state. The lifetime of the nearly degenerate molecular gas exceeds 100 ms in the vicinity of the Feshbach resonance. The measured dependence of the molecular binding energy on the magnetic field demonstrates the open-channel character of the molecules over a wide field range and implies significant singlet admixture. This will enable efficient transfer into the singlet vibrational ground state, resulting in a stable molecular Fermi gas with strong dipolar interactions.

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Formation of ultracold weakly bound dimers of bosonic 23Na39K

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We create weakly bound bosonic ${}^{23}{\mathrm{Na}}^{39}\mathrm{K}$ molecules in a mixture of ultracold $^{23}\mathrm{Na}$ and $^{39}\mathrm{K}$ . The creation is done in the vicinity of a so far undetected Feshbach resonance at about 196 G which we identify in this work by atom-loss spectroscopy. We investigate the involved molecular state by performing destructive radio-frequency binding-energy measurements. For the constructive molecule creation we use radio-frequency pulses with which we assemble up to 6000 molecules. We analyze the molecule creation efficiency as a function of the radio-frequency pulse duration and the atom number ratio between $^{23}\mathrm{Na}$ and $^{39}\mathrm{K}$ . We find an overall optimal efficiency of $6\phantom{\rule{0.16em}{0ex}}%$ referring to the $^{39}\mathrm{K}$ atom number. The measured lifetime of the molecules in the bath of trapped atoms is about 0.3 ms.We create weakly bound bosonic ${}^{23}{\mathrm{Na}}^{39}\mathrm{K}$ molecules in a mixture of ultracold $^{23}\mathrm{Na}$ and $^{39}\mathrm{K}$. The creation is done in the vicinity of a so far undetected Feshbach resonance at about 196 G which we identify in this work by atom-loss spectroscopy. We investigate the involved molecular state by performing destructive radio-frequency binding-energy measurements. For the constructive molecule creation we use radio-frequency pulses with which we assemble up to 6000 molecules. We analyze the molecule creation efficiency as a function of the radio-frequency pulse duration and the atom number ratio between $^{23}\mathrm{Na}$ and $^{39}\mathrm{K}$. We find an overall optimal efficiency of $6\phantom{\rule{0.16em}{0ex}}%$ referring to the $^{39}\mathrm{K}$ atom number. The measured lifetime of the molecules in the bath of trapped atoms is about 0.3 ms.

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Momentum-resolved Raman spectroscopy of bound molecules in ultracold Fermi gas

Zhengkun Fu, Pengjun Wang, Lianghui Huang +2 more

The binding energy of Feshbach molecules from a two-component Fermi gas of ${}^{40}$ K atoms has been experimentally measured with the momentum-resolved Raman spectroscopy. Comparing with the radio-frequency spectroscopy, in the present experiment the signal of unpaired (free atoms) and the bound molecules can be directly observed and the binding energy can be simultaneously determined in a single running experiment. The energy-momentum dispersion spectra of the ultracold Fermi gas in the BEC side are also measured and reconstructed. The present experimental technology of the momentum-resolved Raman spectroscopy can be easily extended to perform spatially momentum-resolved Raman spectroscopy and to obtain the response spectra of a homogeneous system in the local density approximation.The binding energy of Feshbach molecules from a two-component Fermi gas of ${}^{40}$K atoms has been experimentally measured with the momentum-resolved Raman spectroscopy. Comparing with the radio-frequency spectroscopy, in the present experiment the signal of unpaired (free atoms) and the bound molecules can be directly observed and the binding energy can be simultaneously determined in a single running experiment. The energy-momentum dispersion spectra of the ultracold Fermi gas in the BEC side are also measured and reconstructed. The present experimental technology of the momentum-resolved Raman spectroscopy can be easily extended to perform spatially momentum-resolved Raman spectroscopy and to obtain the response spectra of a homogeneous system in the local density approximation.

arXiv:1208.4718Physical Review ASep 7, 20129 citations

We create weakly bound bosonic

{}^{23}{\mathrm{Na}}^{39}\mathrm{K}

molecules in a mixture of ultracold

^{23}\mathrm{Na}

and

^{39}\mathrm{K}

. The creation is done in the vicinity of a so far undetected Feshbach resonance at about 196 G which we identify in this work by atom-loss spectroscopy. We investigate the involved molecular state by performing destructive radio-frequency binding-energy measurements. For the constructive molecule creation we use radio-frequency pulses with which we assemble up to 6000 molecules. We analyze the molecule creation efficiency as a function of the radio-frequency pulse duration and the atom number ratio between

^{23}\mathrm{Na}

and

^{39}\mathrm{K}

. We find an overall optimal efficiency of

6\phantom{\rule{0.16em}{0ex}}%

referring to the

^{39}\mathrm{K}

atom number. The measured lifetime of the molecules in the bath of trapped atoms is about 0.3 ms.

The binding energy of Feshbach molecules from a two-component Fermi gas of

{}^{40}

K atoms has been experimentally measured with the momentum-resolved Raman spectroscopy. Comparing with the radio-frequency spectroscopy, in the present experiment the signal of unpaired (free atoms) and the bound molecules can be directly observed and the binding energy can be simultaneously determined in a single running experiment. The energy-momentum dispersion spectra of the ultracold Fermi gas in the BEC side are also measured and reconstructed. The present experimental technology of the momentum-resolved Raman spectroscopy can be easily extended to perform spatially momentum-resolved Raman spectroscopy and to obtain the response spectra of a homogeneous system in the local density approximation.