Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1211.1512 · Physical Review Letters

Precise Characterization of Li6 Feshbach Resonances Using Trap-Sideband-Resolved RF Spectroscopy of Weakly Bound Molecules

G. Zürn, Thomas Lompe, A. N. Wenz, Selim Jochim, Paul S. Julienne, Jeremy M. Hutson

Published Mar 25, 2013• 250 citations
arXivHTMLPDF

Abstract

We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).

DOI
10.1103/physrevlett.110.135301

Related papers

Accounting for Confinement Shifts on the Binding Energies of 39K Feshbach Molecules

Jared Popowski

Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.

•Jan 1, 2019•0 citations

Precise Determination of Li6 Cold Collision Parameters by Radio-Frequency Spectroscopy on Weakly Bound Molecules

M. Bartenstein, A. Altmeyer, S. Riedl +9 more

We employ radio-frequency spectroscopy on weakly bound (6)Li(2) molecules to precisely determine the molecular binding energies and the energy splittings between molecular states for different magnetic fields. These measurements allow us to extract the interaction parameters of ultracold (6)Li atoms based on a multichannel quantum scattering model. We determine the singlet and triplet scattering lengths to be a(s) = 45.167(8)a(0) and a(t) = -2140(18)a(0) (1a(0) = 0.052 917 7 nm), and the positions of the broad Feshbach resonances in the energetically lowest three s-wave scattering channels to be 83.41(15), 69.04(5), and 81.12(10) mT.

arXiv:cond-mat/0408673•Physical Review Letters•Mar 18, 2005•302 citations

Radio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gas

Lianghui Huang, Pengjun Wang, Zhengkun Fu +1 more

We create weakly bound Feshbach molecules in ultracold Fermi gas 40 K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.

Chinese Physics B•Jan 1, 2014•6 citations

Radio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gasRadio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gasRadio-frequency spectroscopy of weakly bound molecules in ultracold Fermi gas

黄良辉, 王鹏军, 付正坤 +1 more

We create weakly bound Feshbach molecules in ultracold Fermi gas 4~K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.

中国物理B:英文版•Jan 1, 2014•0 citations

Feshbach resonances in cold atomic gases

E. G. M. van Kempen

The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.

•Jan 1, 2006•1 citation

High-Sensitivity rf Spectroscopy of a Strongly Interacting Fermi Gas

Constantine Shkedrov, Yanay Florshaim, Gal Ness +2 more

rf spectroscopy is one of the most powerful probing techniques in the field of ultracold gases. We report on a novel rf spectroscopy scheme with which we can detect very weak signals of only a few atoms. Using this method, we extended the experimentally accessible photon-energies range by an order of magnitude compared to previous studies. We directly verify a universal property of fermions with short-range interactions which is a power-law scaling of the rf spectrum tail all the way up to the interaction scale. We also determine, with high precision, the trap average contact parameter for different interaction strength. Finally, we employ our technique to precisely measure the binding energy of Feshbach molecules in an extended range of magnetic fields. These data are used to extract a new calibration of the Feshbach resonance between the two lowest energy levels of ^{40}K.

arXiv:1803.01770•Physical Review Letters•Aug 30, 2018•26 citations
We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).
Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.
We employ radio-frequency spectroscopy on weakly bound (6)Li(2) molecules to precisely determine the molecular binding energies and the energy splittings between molecular states for different magnetic fields. These measurements allow us to extract the interaction parameters of ultracold (6)Li atoms based on a multichannel quantum scattering model. We determine the singlet and triplet scattering lengths to be a(s) = 45.167(8)a(0) and a(t) = -2140(18)a(0) (1a(0) = 0.052 917 7 nm), and the positions of the broad Feshbach resonances in the energetically lowest three s-wave scattering channels to be 83.41(15), 69.04(5), and 81.12(10) mT.
We create weakly bound Feshbach molecules in ultracold Fermi gas 40 K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.
We create weakly bound Feshbach molecules in ultracold Fermi gas 4~K by sweeping a magnetic field across a broad Feshbach resonance point 202.2 G with a rate of 20 ms/G and perform the dissociation process using radio-frequency (RF) technology. From RF spectroscopy, we obtain the binding energy of the weakly bound molecules in the vicinity of Feshbach resonance. Our measurement also shows that the number of atoms generated from the dissociation process is different at various magnetic fields with the same RF amplitude, which gives us a deeper understanding of weakly bound Feshbach molecules.
The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.
rf spectroscopy is one of the most powerful probing techniques in the field of ultracold gases. We report on a novel rf spectroscopy scheme with which we can detect very weak signals of only a few atoms. Using this method, we extended the experimentally accessible photon-energies range by an order of magnitude compared to previous studies. We directly verify a universal property of fermions with short-range interactions which is a power-law scaling of the rf spectrum tail all the way up to the interaction scale. We also determine, with high precision, the trap average contact parameter for different interaction strength. Finally, we employ our technique to precisely measure the binding energy of Feshbach molecules in an extended range of magnetic fields. These data are used to extract a new calibration of the Feshbach resonance between the two lowest energy levels of ^{40}K.