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arXiv:1803.01770 · Physical Review Letters

High-Sensitivity rf Spectroscopy of a Strongly Interacting Fermi Gas

Constantine Shkedrov, Yanay Florshaim, Gal Ness, Andrey Gandman, Yoav Sagi

Published Aug 30, 2018• 26 citations
arXivHTMLPDF

Abstract

rf spectroscopy is one of the most powerful probing techniques in the field of ultracold gases. We report on a novel rf spectroscopy scheme with which we can detect very weak signals of only a few atoms. Using this method, we extended the experimentally accessible photon-energies range by an order of magnitude compared to previous studies. We directly verify a universal property of fermions with short-range interactions which is a power-law scaling of the rf spectrum tail all the way up to the interaction scale. We also determine, with high precision, the trap average contact parameter for different interaction strength. Finally, we employ our technique to precisely measure the binding energy of Feshbach molecules in an extended range of magnetic fields. These data are used to extract a new calibration of the Feshbach resonance between the two lowest energy levels of ^{40}K.

DOI
10.1103/physrevlett.121.093402

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rf spectroscopy is one of the most powerful probing techniques in the field of ultracold gases. We report on a novel rf spectroscopy scheme with which we can detect very weak signals of only a few atoms. Using this method, we extended the experimentally accessible photon-energies range by an order of magnitude compared to previous studies. We directly verify a universal property of fermions with short-range interactions which is a power-law scaling of the rf spectrum tail all the way up to the interaction scale. We also determine, with high precision, the trap average contact parameter for different interaction strength. Finally, we employ our technique to precisely measure the binding energy of Feshbach molecules in an extended range of magnetic fields. These data are used to extract a new calibration of the Feshbach resonance between the two lowest energy levels of ^{40}K.
Ultracold 39K gases provide an ideal platform to study quantum few- and many-body systems, due to the high degree of control present in these systems. In particular, Feshbach resonances facilitate a magnetically tunable interaction strength between the atoms in the gas, and allow the formation of two- and three-body bound states, called Feshbach molecules and Efimov trimers respectively. Radio-frequency dissociation spectroscopy of weakly bound Feshbach molecules is one of the most precise ways to characterize the properties of a Feshbach resonance. We apply a numerical method to our Feshbach molecule binding energy data to compute the shift in the molecule’s binding energy due to the presence of a confining potential. These simulations are first used to replicate the confinement shift found for 6Li Feshbach molecules by another group, and then to correct our measurement results for the binding energy of 39K Feshbach molecules. The correction of these measurements is necessary for our determination of the Feshbach resonance location with unprecedented accuracy.
We perform radio-frequency dissociation spectroscopy of weakly bound 6Li2 Feshbach molecules using low-density samples of about 30 molecules in an optical dipole trap. Combined with a high magnetic field stability, this allows us to resolve the discrete trap levels in the radio-frequency dissociation spectra. This novel technique allows the binding energy of Feshbach molecules to be determined with unprecedented precision. We use these measurements as an input for a fit to the 6Li scattering potential using coupled-channel calculations. From this new potential, we determine the pole positions of the broad 6Li Feshbach resonances with an accuracy better than 7×10(-4) of the resonance widths. This eliminates the dominant uncertainty for current precision measurements of the equation of state of strongly interacting Fermi gases. As an important consequence, our results imply a corrected value for the Bertsch parameter ξ measured by Ku et al. [Science 335, 563 (2012)], which is ξ=0.370(5)(8).
The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.
Universal relations that hold for any state provide powerful constraints on systems consisting of fermions with two spin states interacting with a large scattering length. In radio-frequency (rf) spectroscopy, the mean shift in the rf frequency and the large-frequency tail of the rf transition rate are proportional to the contact, which measures the density of pairs with small separations. We show that these universal relations can be derived and extended by using the short-time operator product expansion of quantum field theory. This is a general method for identifying aspects of many-body physics that are controlled by few-body physics.
Using radio-frequency (rf) spectroscopy, we measure the ppp-wave contacts in a Fermi gas of 6Li^{6}\mathrm{Li}6Li atoms near the ppp-wave Feshbach resonance. The rf spectrum exhibits clear asymptotic behavior, characterized by ${\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\ensuremath{\omega}}}^{\ensuremath{-}1/2}$ and ${\stackrel{\ifmmode \tilde{}\else \~{}\fi{}}{\ensuremath{\omega}}}^{\ensuremath{-}3/2}$ dependencies. The magnetic-field dependence of the ppp-wave contacts agrees reasonably well with the virial expansion theory in a detuned magnetic-field range, validating the theory near half of the Fermi temperature. The ppp-wave contacts measured in this article constitute a second data set, complementing the data obtained from the 40K^{40}\mathrm{K}40K system and contributing valuable insights into ppp-wave interactions in ultracold Fermi gases.
The experimental realization of stable, ultracold Fermi gases near a Feshbach resonance allows to study gases with attractive interactions of essentially arbitrary strength. They extend the classic paradigm of BCS into a regime which has never been accessible before. We review the theoretical concepts which have been developed in this context, including the Tan relations and the notion of fixed points at zero density, which are at the origin of universality. We discuss in detail the universal thermodynamics of the unitary Fermi gas which allows a fit free comparison between theory and experiment for this strongly interacting system. In addition, we adress the consequences of scale invariance at infinite scattering length and the subtle violation of scale invariance in two dimensions. Finally we discuss the Fermionic excitation spectrum accessible in momentum resolved RF-spectroscopy and the origin of universal lower bounds for the shear viscosity and the spin diffusion constant.