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Exploring Few-body Scattering Resonances in a Bose-Fermi Mixture: From Feshbach Dimers to Efimov Trimers

Tyler D. Cumby

Published Jan 1, 2012• 0 citations
OpenAlex

Abstract

This thesis presents experiments exploring Feshbach molecules and Efimov trimers in an ultracold Bose-Fermi atomic gas mixture of 40K and 87Rb. These bound states are accessed via scattering resonances, called Fano-Feshbach resonances, which arise as a consequence of a bound state being tuned through degeneracy with the threshold energy of colliding atoms. In addition to allowing the tunability of interactions, the Fano-Feshbach resonance allows for a weakly bound molecule state, called the Feshbach molecule state, to be populated. The efficiency of conversion to the Feshbach molecule state depends upon the rate with which the bound state energy is swept through degeneracy with atomic threshold energy. In regions of large scattering lengths, three-body bound states, called Efimov states, also influence inelastic Bose-Bose-Fermi collisions and boson+molecule collisions in our system. The work presented in this thesis utilizes a magnetically tunable Fano-Feshbach resonance to study Feshbach molecule creation in the perturbative limit (the limit of fast magnetic-field sweeps) and the saturated limit (the limit of slow sweeps), where a phenomenological model is applied to understand the conversion efficiency as well as the quantum degeneracy of the molecules. In addition, I present a study of boson+molecule collision rates and Bose-Bose-Fermi collision rates in order to observe signatures of Efimov states and compare against results in the gas mixture 41K-87Rb to address the question of universality of the three-body parameter in heteronuclear gas mixtures.

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This thesis presents experiments exploring Feshbach molecules and Efimov trimers in an ultracold Bose-Fermi atomic gas mixture of 40K and 87Rb. These bound states are accessed via scattering resonances, called Fano-Feshbach resonances, which arise as a consequence of a bound state being tuned through degeneracy with the threshold energy of colliding atoms. In addition to allowing the tunability of interactions, the Fano-Feshbach resonance allows for a weakly bound molecule state, called the Feshbach molecule state, to be populated. The efficiency of conversion to the Feshbach molecule state depends upon the rate with which the bound state energy is swept through degeneracy with atomic threshold energy. In regions of large scattering lengths, three-body bound states, called Efimov states, also influence inelastic Bose-Bose-Fermi collisions and boson+molecule collisions in our system. The work presented in this thesis utilizes a magnetically tunable Fano-Feshbach resonance to study Feshbach molecule creation in the perturbative limit (the limit of fast magnetic-field sweeps) and the saturated limit (the limit of slow sweeps), where a phenomenological model is applied to understand the conversion efficiency as well as the quantum degeneracy of the molecules. In addition, I present a study of boson+molecule collision rates and Bose-Bose-Fermi collision rates in order to observe signatures of Efimov states and compare against results in the gas mixture 41K-87Rb to address the question of universality of the three-body parameter in heteronuclear gas mixtures.
This thesis describes experiments on few-body interactions in a mixture of ultracold bosonic 87Rb and fermionic 40K atoms. Ultracold atoms are celebrated as a platform to explore fundamental quantum physics because their internal states, external potentials, and interactions with each other can be controlled by straightforward electrical and optical tools. In the case of Bose-Fermi mixtures, control comes at the cost of stability when strong interactions give rise to inelastic collisions that destroy the atomic samples. I present detailed measurements of the cross sections for these inelastic processes and discuss how they fit into an emerging pattern of resonances that is leading to better models of few-atom interactions. These phenomena have their roots in universal Efimov physics, which is a paradigm of quantum three-body interactions that was originally inspired by exotic nuclear states. I also discuss several methods to control the formation of KRb Feshbach molecules within the finite lifetime of the interacting K and Rb atomic mixture.
Few-body effects play an important role for the understanding of ultracold quantum gases. We make use of an effective field theory approach to investigate various aspects of universal few-body physics close to a Feshbach resonance. That is the regime where the scattering length is large compared to all other length scales of the system and thus determines the observables. It is also the regime where the Efimov effect whose main characteristic is the occurrence of a sequence of three-body bound states becomes important. At unitarity, i.e., for diverging scattering length, the ratio of binding energies of neighboring states approaches a constant. The existence of those trimers can be captured by a single three-body parameter and influences observables such as recombination rates. Starting from adequate Lagrangians, we derive atom-dimer scattering amplitudes that contain all information of interest about the three-particle systems. With this method, we first investigate the scattering of atoms and dimers at finite temperature in the presence of the Efimov effect. We calculate the dimer relaxation rate and obtain good agreement with available experimental data. Furthermore, heteronuclear mixtures exhibiting large interspecies scattering length are studied in detail. If bosons are the majority species, the Efimov effect occurs in an S-wave channel and we are able to compute three-body recombination and dimer relaxation rates. The results are compared to the outcome of two existing experiments. For mainly fermionic systems, the Efimov effect is only present in an overall P-wave and three-body recombination at threshold vanishes. However, in mixtures of atoms and dimers, scattering cross sections and dimer relaxation show the typical Efimov behavior of log-periodicity. We also consider two-dimensional Bose gases, where the Efimov effect does not occur. For those systems, we derive an equation including the first non-universal corrections and deduce three-body observables such as binding energies and atom-dimer scattering parameters.
This thesis reports on experiments studying the few-body physics of three distinguishable fermionic atoms with large scattering lengths. The experiments were performed with ultracold gases of fermionic 6Li atoms in three different hyperfine states. By tuning the strength of the interactions between the atoms with Feshbach resonances and measuring the rate constants for inelastic three-atom and atom-dimer collisions the intersections of two universal trimer states with the three-atom and atom-dimer continuum could be located. Subsequently, one of these Efimov states was directly observed with RF-association spectroscopy. Using this technique the binding energy of this Efimov state was measured as a function of the strength of the interparticle interactions. The experiments presented in this thesis provide a nearly complete understanding of the universal few-body physics of three-component Fermi gases of 6Li atoms. This understanding will be the foundation for future studies of the many-body physics of three-component Fermi gases.
We convert a strongly interacting ultracold Bose gas into a mixture of atoms and molecules by sweeping the interactions from resonant to weak. By analyzing the decay dynamics of the molecular gas, we show that in addition to Feshbach dimers it contains Efimov trimers. Typically around 8% of the total atomic population is bound into trimers, identified by their density-independent lifetime of about 100 μs. The lifetime of the Feshbach dimers shows a density dependence due to inelastic atom-dimer collisions, in agreement with theoretical calculations. We also vary the density of the gas across a factor of 250 and investigate the corresponding atom loss rate at the interaction resonance.
The progression from two- through few- to many-body physics is an open and interesting question. Experiments that can test these theories must walk the fine line between cultivating a rich many-body system, yet preventing the interactions from completely destroying the system before study. This thesis explores the two- and few-body interactions present in a resonantly interacting degenerate Bose gas. We explore these interactions as a function of the density of the initial Bose-Einstein condensate. We use loss rates to characterize the interactions and find that a significant portion of the perceived atomic loss is from sweeping the atoms into loosely bound molecules.The decay dynamics identify a molecule mixture of both Feshbach dimers and Efimov trimers
Recent measurements of Efimov resonances for a number of ultracold atom species have revealed an unexpected universality, in which three-body scattering properties are determined by the van der Waals length of the two-body interaction potential. To investigate whether this universality extends to heteronuclear mixtures, we measure loss rate coefficients in an ultracold trapped gas of 40K and 87Rb atoms. We find an Efimov-like resonance in the rate of inelastic collisions between 40K87Rb Feshbach molecules and 87Rb atoms. However, we do not observe any Efimov-related resonances in the rates of inelastic collisions between three atoms. These observations are compared to previous measurements by the LENS group of Efimov resonances in a 41K and 87Rb mixture as well as to recent predictions.