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Bulletin of the American Physical Society

Spin squeezing of $10^{11}$ atoms

Han Bao, Junlei Duan, Pengxiong Li, Xingda Lu, Weizhi Qu, Shenchao Jin, M.-Z. Wang, Irina V. Novikova, Eugeniy E. Mikhailov, Kaifeng Zhao, Heng Shen, Yanhong Xiao

Published Nov 16, 2018• 0 citations
OpenAlex

Abstract

Atomic ensemble with large number of quantum correlated particles is a desirable resource for precision measurement and quantum simulation. Being a type of quantum correlated state particularly useful for quantum metrology, spin squeezed state (SSS) has been pursued in both cold atom and vapor cell systems, and the largest ensemble so far contains $10^{8}$ atoms. We report experimental preparation of a SSS in a paraffin-coated macroscopic vapor cell in free space, containing $10^{11}$ $^{87}\text{Rb}$ atoms, by means of stroboscopic quantum non-demolition measurement. We observed $2.38\pm0.23~\text{dB}$ noise reduction, and $1.31\pm0.23~\text{dB}$ spin squeezing \emph{below coherent spin state} by the Wineland criterion. Our result present the highest angular resolution on the Bloch sphere in all SSS up to date, and will open possibilities to implement quantum control, metrology and quantum simulations using such large entangled atomic ensembles. The universal off-resonance interaction utilized here can also be straightforwardly expanded to other systems, such as trapped ions and mechanical oscillators, in the application of entanglement generation and open-system quantum simulations.

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Bulletin of the American Physical Society•Jun 12, 2015•4 citations
Spin squeezing of 101110^{11}1011 atoms
Atomic ensemble with large number of quantum correlated particles is a desirable resource for precision measurement and quantum simulation. Being a type of quantum correlated state particularly useful for quantum metrology, spin squeezed state (SSS) has been pursued in both cold atom and vapor cell systems, and the largest ensemble so far contains 10810^{8}108 atoms. We report experimental preparation of a SSS in a paraffin-coated macroscopic vapor cell in free space, containing 101110^{11}1011 87Rb^{87}\text{Rb}87Rb atoms, by means of stroboscopic quantum non-demolition measurement. We observed 2.38±0.23 dB2.38\pm0.23~\text{dB}2.38±0.23 dB noise reduction, and 1.31±0.23 dB1.31\pm0.23~\text{dB}1.31±0.23 dB spin squeezing \emph{below coherent spin state} by the Wineland criterion. Our result present the highest angular resolution on the Bloch sphere in all SSS up to date, and will open possibilities to implement quantum control, metrology and quantum simulations using such large entangled atomic ensembles. The universal off-resonance interaction utilized here can also be straightforwardly expanded to other systems, such as trapped ions and mechanical oscillators, in the application of entanglement generation and open-system quantum simulations.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.
We report the generation of spin squeezing and entanglement in a magnetically sensitive atomic ensemble, and entanglement-enhanced field measurements with this system. A maximal m(f) = ± 1 Raman coherence is prepared in an ensemble of 8.5 × 10(5) laser-cooled (87)Rb atoms in the f = 1 hyperfine ground state, and the collective spin is squeezed by synthesized optical quantum nondemolition measurement. This prepares a state with large spin alignment and noise below the projection-noise level in a mixed alignment-orientation variable. 3.2 dB of noise reduction is observed and 2.0 dB of squeezing by the Wineland criterion, implying both entanglement and metrological advantage. Enhanced sensitivity is demonstrated in field measurements using alignment-to-orientation conversion.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.