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Breaking Quantum Limits with Collective Cavity-QED: Generation of Spin Squeezed States via Quantum Non-Demolition Measurements

Zilong Chen

Published Jan 1, 2013• 3 citations
OpenAlex

Abstract

Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.

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Cavity-aided nondemolition measurements for atom counting and spin squeezing

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Probing the collective spin state of an ensemble of atoms may provide a means to reduce heating via the photon recoil associated with the measurement and provide a robust, scalable route for preparing highly entangled states with spectroscopic sensitivity below the standard quantum limit for coherent spin states. The collective probing relies on obtaining a very large optical depth that can be effectively increased by placing the ensemble within an optical cavity such that the probe light passes many times through the ensemble. Here we provide expressions for measurement resolution and spectroscopic enhancement in such cavity-aided nondemolition measurements as a function of the cavity detuning. In particular, fundamental limits on spectroscopic enhancements in ${}^{87}\mathrm{Rb}$ are considered.

arXiv:1211.0723•Physical Review A•Apr 23, 2014•70 citations
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.
We use the vacuum Rabi splitting to perform quantum nondemolition measurements that prepare a conditionally spin squeezed state of a collective atomic psuedospin. We infer a 3.4(6) dB improvement in quantum phase estimation relative to the standard quantum limit for a coherent spin state composed of uncorrelated atoms. The measured collective spin is composed of the two-level clock states of nearly 10(6) (87)Rb atoms confined inside a low finesse F=710 optical cavity. This technique may improve atomic sensor precision and/or bandwidth, and may lead to more precise tests of fundamental physics.
By allowing a large ensemble of laser cooled and trapped 87Rb atoms to interact collectively with an optical cavity, I have explored two phenomena that may prove useful for enhancing precision measurements: superradiant lasing and spin squeezing.\nSuperradiant lasers have been proposed as future ultrastable optical frequency references, with predicted linewidths < 1 millihertz. These lasers operate in an unusual regime of laser physics where collective emission from an atomic ensemble maps the quantum phase stored in the atoms onto the optical cavity field. I will give an overview of my experimental work using a cold-atom, superradiant Raman laser as a model system to confirm a number of the key predictions concerning superradiant lasing, including the possibility of coherent emission with < 1 intracavity photon on average and greatly reduced sensitivity to cavity frequency noise.\nI also present work using cavity-aided, coherence-preserving measurements of the atomic state population to create entanglement between atoms. The entanglement enables more precise estimation of the quantum phase at the heart of nearly all precision measurements and sensors utilizing quantum objects. By utilizing a cycling transition for the quantum non-demolition probe, we have reduced by several orders of magnitude the measurement induced back-action caused by spontaneous Raman transitions. We directly observe, with no background subtraction, a spin squeezed state with sensitivity to measuring a quantum phase enhanced 10.5 times in variance (i.e. 10.2 dB) beyond the standard quantum limit for an unentangled state. This experimental breakthrough demonstrates that quantum-aided sensing techniques can realize large enough enhancements to have a substantial impact on precision measurements and may aid advances in technology as well as searches for new physics.
Building scalable quantum systems that demonstrate genuine performance enhancement based on entanglement is a major scientific goal for fields including computing, networking, simulations, and metrology. The tremendous challenge arises from the fragility of entanglement in increasingly larger sized quantum systems. Optical atomic clocks utilizing a large number of atoms have pushed the frontier of measurement science, building on precise engineering of quantum states and control of atomic interactions. However, today's state-of-the-art optical atomic clocks are limited by the quantum projection noise (QPN) defined by many uncorrelated atoms. Pioneering work on producing spin squeezed states of atoms has shown a path towards integrating entanglement into the best performing clocks. However, to directly demonstrate advantage of quantum entanglement in a working clock we must prevent backaction effects that degrade quantum coherence and introduce uncontrolled perturbations, as well as minimize the influence of technical noise arising from the interrogating clock laser. Here we present a new optical clock platform integrated with collective strong-coupling cavity QED for quantum non-demolition (QND) measurement. Optimizing the competition between spin measurement precision and loss of coherence, we measure a Wineland parameter of -1.8(7) dB for 1.9x104^44 atoms, thus verifying the presence of entanglement. Furthermore, a moving lattice allows the cavity to individually address two independent sub-ensembles, enabling us to spin squeeze two clock ensembles successively and compare their performance. This differential comparison between the two squeezed clocks directly verifies enhanced clock stability of 2.0(3) dB below QPN, and 0.6(3) dB above the standard quantum limit (SQL), at the measurement precision level of 10−17^{-17}−17, without subtracting any technical noise contributions.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
Atomic sensors are among the best devices for precision measurements of time, electric and magnetic fields, and inertial forces. However, all atomic sensors that utilise uncorrelated particles are ultimately limited by quantum projection noise, as is already the case for state-of-the-art atomic clocks. This so-called standard quantum limit (SQL) can be overcome by employing entanglement, a prime example being the spin-squeezed states. Spin squeezing can be produced in a quantum non-demolition (QND) measurement of the collective spin, particularly with cavity quantum electrodynamical (cQED) interactions. In this thesis, I present the second-generation trapped-atom clock on a chip (TACC) experiment, where we combine a metrology-grade compact clock with a miniature cQED platform to test quantum metrology protocols at a metrologically-relevant precision level. In a standard Ramsey spectroscopy, the stability of the apparatus is confirmed by a fractional frequency Allan deviation of 6E-13 at 1 s. We demonstrate spin squeezing by QND measurement, reaching 8(1) dB for 1.7E4 atoms, currently limited by decoherence due to technical noise. Cold collisions between atoms play an important role at this level of precision, leading to rich spin dynamics. Here we find that the interplay between cavity measurements and collisional spin dynamics manifests itself in a quantum amplification effect of the cavity measurement. A simple model is proposed, and is confirmed by initial measurements. New experiments in this direction may shed light on the surprising many-body physics in this sytem of interacting cold atoms.
Probing the collective spin state of an ensemble of atoms may provide a means to reduce heating via the photon recoil associated with the measurement and provide a robust, scalable route for preparing highly entangled states with spectroscopic sensitivity below the standard quantum limit for coherent spin states. The collective probing relies on obtaining a very large optical depth that can be effectively increased by placing the ensemble within an optical cavity such that the probe light passes many times through the ensemble. Here we provide expressions for measurement resolution and spectroscopic enhancement in such cavity-aided nondemolition measurements as a function of the cavity detuning. In particular, fundamental limits on spectroscopic enhancements in 87Rb{}^{87}\mathrm{Rb}87Rb are considered.