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arXiv:1111.6969 · Physical Review Letters

Magnetic Sensitivity Beyond the Projection Noise Limit by Spin Squeezing

R. J. Sewell, Marco Koschorreck, M. Napolitano, B. Dubost, N. Behbood, Morgan W. Mitchell

Published Dec 19, 2012• 325 citations
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Abstract

We report the generation of spin squeezing and entanglement in a magnetically sensitive atomic ensemble, and entanglement-enhanced field measurements with this system. A maximal m(f) = ± 1 Raman coherence is prepared in an ensemble of 8.5 × 10(5) laser-cooled (87)Rb atoms in the f = 1 hyperfine ground state, and the collective spin is squeezed by synthesized optical quantum nondemolition measurement. This prepares a state with large spin alignment and noise below the projection-noise level in a mixed alignment-orientation variable. 3.2 dB of noise reduction is observed and 2.0 dB of squeezing by the Wineland criterion, implying both entanglement and metrological advantage. Enhanced sensitivity is demonstrated in field measurements using alignment-to-orientation conversion.

DOI
10.1103/physrevlett.109.253605

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Conference on Lasers and Electro-Optics•Jan 1, 2010•1 citation
We report the generation of spin squeezing and entanglement in a magnetically sensitive atomic ensemble, and entanglement-enhanced field measurements with this system. A maximal m(f) = ± 1 Raman coherence is prepared in an ensemble of 8.5 × 10(5) laser-cooled (87)Rb atoms in the f = 1 hyperfine ground state, and the collective spin is squeezed by synthesized optical quantum nondemolition measurement. This prepares a state with large spin alignment and noise below the projection-noise level in a mixed alignment-orientation variable. 3.2 dB of noise reduction is observed and 2.0 dB of squeezing by the Wineland criterion, implying both entanglement and metrological advantage. Enhanced sensitivity is demonstrated in field measurements using alignment-to-orientation conversion.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
We report a nonlinear alignment-to-orientation conversion measurement of atomic spins that simultaneously shows super-Heisenberg scaling and achieves projection-noise limited sensitivity of 990 spins, 20 dB more sensitive than the previous best nonlinear measurement. Using this technique, we have recently demonstrated conditional spin squeezing of the atomic ensemble, and entanglement-enhanced measurement sensitivity useful for optical magnetometry. In addition, we use a novel technique to explicitly certify that the measurement fulfills all the conditions required for quantum non-demolition measurement.
At the beginning of the 20th century measurement precision was related exclusively to the capabilities of the experimenter and the apparatus. Any imprecision was attributed to imperfect devices for the measurement. Later on, when the quantumness of objects like photons, electrons, or atoms, was recognized, it became clear that the measurement and the object to be measured could no longer be separated. Both follow the laws of quantum physics which impose limits on the accuracy of any measurement. In the last three decades, a lot of research has been dedicated to find strategies to overcome these limitations. This new field of quantum metrology is where this work is placed. This thesis describes the generation of interparticle entanglement in form of a squeezed spin state in a cloud of cold 87Rb atoms by performing nondestructive spin measurements. Towards this goal, we have implemented a shot-noise limited polarization probing and detection system, atom counting by means of absorption imaging, spin state preparation via optical pumping and nondestructive spin state detection. The quantum noise limited spin readout with polarized light is characterized in two complementary ways in terms of sensitivity and all possible quantum and classical noise sources are measured. To address the rich opportunities provided in the multilevel structure of 87Rb with dispersive probing, we have developed and implemented a frequency offsetlock which allows a large tuning range of several GHz for the dispersive probing. Working with a magnetically sensitive atomic system triggered the development of a magnetic field imaging technique. This applies the elongated atomic sample and internal atomic states as a way of measuring magnetic fields over several millimeters with micrometer resolution and sensitivities down to a few tens of pT/ Hz. We developed a new method for tomographic measurements of the atomic density matrix. Based on our ability of shot noise limited detection of polarization rotations we can in principle, characterize the whole atomic spin state. First, measurements are shown and possible improvements are discussed. An in depth characterization of the light-atom interaction between polarized pulses of light and collective atomic states are the basis for measurements at the quantum level. On one side, we apply classical measurements of spin polarized atoms to measure the strength of the lightatom interaction. On the other side, we use quantum measurements of unpolarized atomic states to characterize all noise sources both technical and quantum. One of the major results of this thesis is the realization of quantum nondemolition measurements in a largespin system. We realized limitations to the performance of the QND measurement implied by higher order light shifts in multilevel atoms, which are often neglected for these kind of systems. We develop a technique which suppresses the detrimental effects of higher order light shifts and recovers an ideal QND measurement. The thesis culminates in the demonstration of spin squeezing in the magnetically sensitive ground state of 87Rb. We achieve a quantum noise reduction by 3 dB, where metrological sensitivity is improved by 2 dB beyond the standard quantum limit of a coherent spin state with the same spin polarization. We address the question how spatial and temporal inhomogeneities both in light and atoms influence the preparation of nonclassical states. An existing covariance matrix approach is extended and we apply it to study effects of detector time resolution, spatial inhomogeneities and atomic motion.
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.