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Preparation of single-photon states via cavity-assisted spontaneous parametric down-conversion for quantum memory based on Y7LiF4:Nd3+ crystal

D O Akat’ev, Латыпов Ильнур Зиннурович, Andrey V. Shkalikov, А. А. Калачев

Published Jan 1, 2017• 1 citation
Publisher

Abstract

We report on the realization of a tunable single-photon source compatible with quantum memories based on isotopically pure Y7LiF4 crystals doped with Nd3+ ions. The source is based on spontaneous parametric down-conversion in a PPLN crystal placed in a resonator. The latter is formed by two mirrors which are transparent for the pump (532 nm) and idler (1377 nm) fields but high reflective for the signal field (867 nm). The width of the second-order cross-correlation function between the signal and idler photons is determined to be 1.5 ns for the cavity length of 8 cm, which corresponds to a cavity bandwidth of 100 MHz.

DOI
10.1051/epjconf/201716102026

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Physical Review A•Nov 20, 2023•10 citations
We report on the realization of a tunable single-photon source compatible with quantum memories based on isotopically pure Y7LiF4 crystals doped with Nd3+ ions. The source is based on spontaneous parametric down-conversion in a PPLN crystal placed in a resonator. The latter is formed by two mirrors which are transparent for the pump (532 nm) and idler (1377 nm) fields but high reflective for the signal field (867 nm). The width of the second-order cross-correlation function between the signal and idler photons is determined to be 1.5 ns for the cavity length of 8 cm, which corresponds to a cavity bandwidth of 100 MHz.
The storage of a signal of a single-photon source based on spontaneous parametric down-conversion in a periodically poled MgO:PPLN crystal in a quantum memory based on an atomic frequency comb in an isotopically pure 143Nd:Y7LiF4^{{{\text{143}}}}{\text{Nd}}{\kern 1pt} {\text{:}}{\kern 1pt} {{{\text{Y}}}^{{\text{7}}}}{\text{Li}}{{{\text{F}}}_{{\text{4}}}}143Nd:Y7LiF4​ crystal has been demonstrated.
Abstract We demonstrate an ultrabright, narrow-band and frequency-tunable photon-pair source based on cavity-enhanced spontaneous parametric down conversion (SPDC) which is compatible with atomic transition of rubidium D 2 -line (780 nm) or cesium D 2 -line (852 nm). With the pump beam alternating between a high and a low power phase, the output is switching between the optical parametric oscillator (OPO) and photon-pair generation mode. We utilize the OPO output light to lock the cavity length to maintain the double resonances of signal and idler, as well as to lock the signal frequency to cesium atomic transition. With a type-II phase matching and a double-passed pump scheme such that the cluster frequency spacing is larger than the SPDC bandwidth, the photon-pair output is in a nearly single-mode operation as confirmed by a scanning Fabry–Perot interferometer with its output detected by a photomultiplier. The achieved generation and detection rates are 7.24 × 10 5 and 6142 s −1 mW −1 , respectively. The correlation time of the photon pair is 21.6(2.2) ns, corresponding to a bandwidth of 2 π × 6.6(6) MHz. The spectral brightness is 1.06 × 10 5 s −1 mW −1 MHz −1 . This is a relatively high value under a single-mode operation with the cavity-SPDC scheme. The generated single photons can be readily used in experiments related to atomic quantum memories.
We present a source of ultra-narrow band, widely non degenerate photon pairs source compatible with quantum repeaters architectures. One photon is compatible with a solid state Praseodymium (Pr3+) doped crystal spin wave quantum memory, and the other photon is at telecommunication wavelengths, such that it can be transmitted over large distances in optical fibers. Pr3+doped solids absorbing photons at 606 nm have shown very promising properties as QM for light. Despite this fact, so far no experiment demonstrated storage of quantum light in Pr3+doped crystals. The main challenge to realize such a source is that the bandwidth of the memory is limited to a few MHz by the excited state spacing of the ions. To achieve the required narrow linewidth we use widely non-degenerate cavity enhanced spontaneous down conversion (SPDC). We measure a correlation time of 104 ns, the longest reported to date for SPDC emitted photons, corresponding to around 2 MHz bandwidth. In addition, the number of longitudinal modes emitted by the source is strongly reduced, thanks to a clustering effect, which facilitates the filtering to reach single mode operation.
Cavity-enhanced spontaneous parametric down-conversion (SPDC) can be used to implement heralded single-photon sources with narrow bandwidth down to tens of megahertz, thus compatible with atom-based quantum memories. In this work, we propose and study the cavities that are either singly resonant at the frequency of only one of the generated photons or doubly resonant at the frequency of one generated photon and for the pump field. We derive analytical expressions for the generation rate and the spectral brightness as a function of the main structure parameters. Our analysis shows that by exploiting counterpropagating SPDC inside a cavity with properly designed distributed Bragg reflectors, pure narrow-band heralded single photons can be generated. In particular, when a pulsed pump illuminates a 1-mm-long singly resonant cavity, the bandwidth of the resonant and the nonresonant photons will be 120 MHz and 5.7 GHz, respectively, with heralded single-photon purity as high as 0.993. Due to its small absorption probability inside the cavity, the heralding efficiency can approach unity if the nonresonant partner is used as a heralded single photon. Finally, we also show that continuous-wave excitation of a 1-cm-long cavity resonant for the pump and copropagating fields can provide photon pairs in a narrow bandwidth of 10 MHz with spectral brightness as high as $2\ifmmode\times\else\texttimes\fi{}{10}^{6}$ $({\text{s}\phantom{\rule{4.pt}{0ex}}\text{mW}\phantom{\rule{4.pt}{0ex}}\text{MHz})}^{\ensuremath{-}1}$. This source can efficiently couple with quantum memories and can find applications in quantum information processing and communication.