This thesis focuses on two problems in circuit quantum electrodynamics. We first investigate theoretically the coupling of a resonator to a continuous distribution of inhomogeneously broadened emitters. Studying this formalism is strongly motivated by recent proposals to use collections of emitters as quantum memories for individual excitations. Such systems benefit from the collective enhancement of the interaction strength, while keeping the relaxation properties of a single emitter. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Taking into account the inhomogeneous broadening allows to simulate with a great accuracy a number of pioneer experimental results on a ensemble of NV centers. The modeling is shown to be a powerful tool to obtain the properties of the spin ensembles coupled to a resonator. We also suggest an original Josephson qubit readout method based on a dc-SQUID with high loop inductance. This system supports a diamond-shape artificial atom where we define logical and ancilla qubits coupled through a cross-Kerr like term. Depending on the logical qubit state, the ancilla is resonantly or dispersively coupled to the resonator, leading to a large contrast in the transmitted microwave signal amplitude. Simulations show that this original method can be faster and have higher fidelity than methods currently used in circuit QED.
This thesis focuses on two problems in circuit quantum electrodynamics. We first investigate theoretically the coupling of a resonator to a continuous distribution of inhomogeneously broadened emitters. Studying this formalism is strongly motivated by recent proposals to use collections of emitters as quantum memories for individual excitations. Such systems benefit from the collective enhancement of the interaction strength, while keeping the relaxation properties of a single emitter. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Taking into account the inhomogeneous broadening allows to simulate with a great accuracy a number of pioneer experimental results on a ensemble of NV centers. The modeling is shown to be a powerful tool to obtain the properties of the spin ensembles coupled to a resonator. We also suggest an original Josephson qubit readout method based on a dc-SQUID with high loop inductance. This system supports a diamond-shape artificial atom where we define logical and ancilla qubits coupled through a cross-Kerr like term. Depending on the logical qubit state, the ancilla is resonantly or dispersively coupled to the resonator, leading to a large contrast in the transmitted microwave signal amplitude. Simulations show that this original method can be faster and have higher fidelity than methods currently used in circuit QED.
This thesis focuses on two problems in circuit quantum electrodynamics. We first investigate theoretically the coupling of a resonator to a continuous distribution of inhomogeneously broadened emitters. Studying this formalism is strongly motivated by recent proposals to use collections of emitters as quantum memories for individual excitations. Such systems benefit from the collective enhancement of the interaction strength, while keeping the relaxation properties of a single emitter. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Taking into account the inhomogeneous broadening allows to simulate with a great accuracy a number of pioneer experimental results on a ensemble of NV centers. The modeling is shown to be a powerful tool to obtain the properties of the spin ensembles coupled to a resonator. We also suggest an original Josephson qubit readout method based on a dc-SQUID with high loop inductance. This system supports a diamond-shape artificial atom where we define logical and ancilla qubits coupled through a cross-Kerr like term. Depending on the logical qubit state, the ancilla is resonantly or dispersively coupled to the resonator, leading to a large contrast in the transmitted microwave signal amplitude. Simulations show that this original method can be faster and have higher fidelity than methods currently used in circuit QED.
We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters' inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitter ensembles. When two different ensembles of emitters are coupled to the resonator, they support a peculiar collective dark state, which is also very attractive for the storage of quantum information.
Spin ensembles inside a cavity act as light-matter interfaces that play an eminentrole in the development of future quantum devices. An apparent asset of ensemble-based systems is the collective enhancement of the coupling strength, facilitating astrong interaction between the light and matter components. Particularly promisingin this regard, due to their convenient handling and integrability, are solid statespin ensembles such as nitrogen-vacancy centers in diamond, phosphorous donors in silicon, or rare earth doped crystals. Such ensemble-based setups, however, are almost inevitably inhomogeneously broadened as the different spins of the ensemble typically have different local environments leading to a spectral distribution in their transition frequencies. This so-called inhomogeneous broadening is a major source for decoherence in solid state systems and a major challenge to be addressed for future technical applications.In this thesis, we aim to provide the theoretical framework necessary to describeand understand various effects of inhomogeneously broadened spin ensembles coupled to a single-mode cavity—a system that has been realized in numerous different quantum optical setups and in very different parameter regimes.For macroscopic spin ensembles, i.e., ensembles consisting of a vast number ofspins, quantum fluctuations of the individual spins can typically be neglected, allowing a semiclassical description based on Maxwell-Bloch equations. Here, we study two prominent effects in the strongly nonlinear regime namely optical bistability, resembling a first-order phase transition, and critical slowing down. In particular, we show that the onset of bistability not only depends on the width of the spectral spin distribution but also strongly depends on its exact shape. Furthermore, we analyze the transient times of the cavity amplitude which show a power-law divergence when an external parameter is changed in the vicinity of the phase transition.This critical slowdown is demonstrated in collaboration with the group ofJörg Schmiedmayer at the Atominstitut of TU Wien. In the experiment, negativelycharged nitrogen vacancy centers in diamond are strongly coupled to a superconducting microwave resonator showing transient times of up to 11 hours.In mesoscopic spin ensembles with moderate numbers of constituents, quantumfluctuations gain importance, and semiclassical methods fail. We study thiscrossover between the semiclassical and the quantum regime using a cumulant expansion approach to study the semiclassical-to-quantum boundary for inhomogeneously broadened spin ensembles inside a cavity. In addition, we develop a time-adaptivevariational renormalization group method to calculate the full quantumdynamics of spin ensembles containing up to one hundred spins. With the aid ofthis method, we examine mesoscopic spin ensembles whose spin distributions form a comb-shaped structure. These so-called atomic frequency combs have promising properties for the storage of quantum information. On the one hand, we show that arbitrary multi-photon states are absorbed by the comb-shaped spin ensembleand re-emitted into the cavity at periodic time intervals. On the other hand, wedemonstrate that by means of such a spin ensemble a coherent input pulse can beconverted into periodic pulses of non-classical light.Finally, we address spin echoes, which are a fundamental part in nuclear magneticresonance as well as in electron spin resonance. Specifically, we transfer the Hahnecho to the strong coupling regime, where we find a new dynamical phenomenonfeaturing a periodic sequence of self-sustained echoes after a conventional Hahn echo pulse. In collaboration with the group of Hans Hübl at the Technical UniversityMunich, a first demonstration of this intriguing multiecho signature is presented inan electron spin resonance experiment with phosphorus donors in silicon.
In the last couple of years much effort has been dedicated to the development and the investigation of hybrid quantum devices, which combine the advantages of very dissimilar quantum systems for the realization of efficient quantum computation and communication technologies. Particularly interesting in this regard are solid-state quantum memories based on ensembles of spins (e.g. nitrogen vacancy defects in diamond or rare-earth doped crystals) coupled to superconducting microwave cavities. Here the spin-ensemble acts as a robust memory where the collective coupling to the cavity mode allows for the coherent transfer of quantum information. The major downside of ensembles inside solid-state systems is their natural tendency to exhibit inhomogeneous broadening of the transition frequencies, which makes experiments as well as their theoretical description very challenging. On the theoretical side it is primarily the computational complexity due to the exponential growth of the associated Hilbert space with the system size that inevitably calls for approximation schemes. To date, the theoretical description of large spin-cavity systems is mainly limited to weak driving fields, where the number of spin-excitations in the ensemble is negligible, corresponding to a Holstein-Primakoff approximation, or to mean-field approaches, where correlations within the system are neglected. In this thesis we aim to develop a model that accurately accounts for the dynamics of large inhomogeneously broadened spin ensembles, coupled to a single cavity mode, even in the case of strong driving fields. In particular we employ the generalized cumulant expansion method to account for correlations within the system, which allows us to go beyond the Holstein-Primakoff and mean-field approximations. As a first step, we demonstrate the applicability of the cumulant expansion technique to the well-studied Jaynes-Cummings model and investigate its main limitations. We then move on to the Tavis-Cummings model with multiple spins inside the cavity and generalize our approach to ensembles containing a very large number of spins (ca. 10 12). Our model aims not only to provide a proper description of ensemble-based quantum memories, but also to serve as a novel tool for the investigation of interesting new physics arising from cooperative effects in inhomogeneous ensembles.
PhD Thesis: Superconducting circuit quantum electrodynamics (QED) has developed into a powerful platform for studying the interaction between matter and different states of light. In this context, superconducting quantum bits (qubits) act as artificial atoms interacting with quantized modes of the electromagnetic field. The field can be trapped in superconducting microwave resonators or propagating in transmission lines. In this thesis, we particularly study circuit QED systems where microwave fields are coupled with superconducting flux and transmon qubits. We optimize the coherence properties of the resonators, by analyzing loss mechanisms at excitation powers of approximately one photon on average. We find that two-level fluctuators associated with oxide layers at substrate and metal surfaces and metal-metal interfaces represent the predominant loss channel. Furthermore, we show how broadband thermal photon fields influence the relaxation and dephasing properties of a superconducting transmon qubit. To this end, we study several second-order loss channels of the transmon qubit and find that the broadband fields introduce a larger decay rate than expected from the Purcell filter defined by the resonator. Additionally, we show that qubit dephasing at the flux-insensitive point as well as low-frequency parameter fluctuations can be enhanced by thermal fields. Finally, we study how artificial atoms react to changes in inherent properties of the light fields. We perform a detailed analysis of the photon statistics of thermal fields using their relation to the qubits coherence properties. We quantitatively recover the expected n2+n-law for the photon number variance and confirm this result by direct correlation measurements. We then show a novel technique for the in-situ conversion of the interaction parity in light-matter interaction. To this end, we couple spatially controlled microwave fields to a flux qubit with two degrees of freedom.
In this thesis, experimentally relevant aspects and open questions of quantum information processing and measurement in circuit quantum electrodynamics have been investigated theoretically. Circuit quantum electrodynamics is a relatively young field combining superconducting transmission line resonators on-chip with superconducting quantum bits which serve as artificial atoms. Remarkable experiments have underlined the prospects of circuit QED as a possible architecture for quantum information processing as well as a framework within which quantum optics experiments can be performed. In contrast to their optical counterparts, these experiments reach the ultra-strong coupling limit and allow e.g. the generation of Fock states, the study of decoherence and the observation of quantum jumps. We present the physics of superconducting circuits based on the Josephson junction as a non-linear circuit element. We discuss the various types of quantum bits (qubits) before turning to an introduction on cavity QED and conclude the introduction with a brief presentation of the most relevant experiments and a short introduction to the principles and prospects of quantum information processing. Building on the pioneering theoretical and experimental work in which up to three qubits have been integrated on a chip and successfully coupled via a cavity mode, we propose a scheme to overcome the natural limits concerning scalability in these systems. Usually, scalability is severely limited by the resonance width of the qubit transitions and the attainable frequency range for both qubit transition and cavity resonance frequencies. This limits the present setups to at most ten qubits. As a possible solution, we propose and investigate a cross-bar grid layout of cavities with qubits at the intersections. It turns out that this setup, allowing for up to about 1000 qubits, offers significant advantages over e.g. nearest-neighbor coupling schemes. In addition, it can serve as a building block for a truly scalable scheme for fault-tolerant quantum information processing with superconducting circuits by combining 7x7 arrays in a staircase manner. Furthermore, we discuss and simulate different possibilities to improve upon the suggested scheme by e.g. using resonant gates and optimal control theory. Another focus of the present thesis is measurement physics. In order to investigate e.g. the possibilities of using a circuit QED system to dispersively detect single microwave photons or to generate multi-qubit entangled states, we introduce in a pedagogical manner the basics of stochastic master equations which generate quantum trajectories before turning to concrete applications. Quantum trajectories have proven to be a state-of-the-art tool to analyze measurement situations in a very realistic manner by giving access to both the measurement record as well as the internal quantum dynamics conditioned on this record. Using the method of quantum trajectories as generated by stochastic master equations, we discuss a scheme to efficiently generate multi-qubit entangled states in a very flexible way. The method is based on a collective, dispersive qubit readout. By this measurement, a suitable product state of N qubits can be reliably converted into e.g. an N-qubit Greenberger-Horne-Zeilinger or W state. We propose and discuss the scheme and investigate the effects of decoherence and parameter spread as they would be encountered in experiment. Last but not least, we propose and fully analyze a scheme to dispersively detect single itinerant microwave photons. While experiments to generate single microwave photons have already been successfully performed, their single-shot quantum non-demolition detection has not been possible so far. The scheme presented in this thesis closes this gap in the circuit QED toolbox and reaches detection efficiencies of 30% only limited by fundamental quantum mechanics in this case the Quantum Zeno effect. This detection scheme could be used in quantum communication or quantum cryptography applications.