This thesis focuses on two problems in circuit quantum electrodynamics. We first investigate theoretically the coupling of a resonator to a continuous distribution of inhomogeneously broadened emitters. Studying this formalism is strongly motivated by recent proposals to use collections of emitters as quantum memories for individual excitations. Such systems benefit from the collective enhancement of the interaction strength, while keeping the relaxation properties of a single emitter. We discuss the influence of the emitters inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Taking into account the inhomogeneous broadening allows to simulate with a great accuracy a number of pioneer experimental results on a ensemble of NV centers. The modeling is shown to be a powerful tool to obtain the properties of the spin ensembles coupled to a resonator. We also suggest an original Josephson qubit readout method based on a dc-SQUID with high loop inductance. This system supports a diamond-shape artificial atom where we define logical and ancilla qubits coupled through a cross-Kerr like term. Depending on the logical qubit state, the ancilla is resonantly or dispersively coupled to the resonator, leading to a large contrast in the transmitted microwave signal amplitude. Simulations show that this original method can be faster and have higher fidelity than methods currently used in circuit QED.
PhD Thesis: Superconducting circuit quantum electrodynamics (QED) has developed into a powerful platform for studying the interaction between matter and different states of light. In this context, superconducting quantum bits (qubits) act as artificial atoms interacting with quantized modes of the electromagnetic field. The field can be trapped in superconducting microwave resonators or propagating in transmission lines. In this thesis, we particularly study circuit QED systems where microwave fields are coupled with superconducting flux and transmon qubits. We optimize the coherence properties of the resonators, by analyzing loss mechanisms at excitation powers of approximately one photon on average. We find that two-level fluctuators associated with oxide layers at substrate and metal surfaces and metal-metal interfaces represent the predominant loss channel. Furthermore, we show how broadband thermal photon fields influence the relaxation and dephasing properties of a superconducting transmon qubit. To this end, we study several second-order loss channels of the transmon qubit and find that the broadband fields introduce a larger decay rate than expected from the Purcell filter defined by the resonator. Additionally, we show that qubit dephasing at the flux-insensitive point as well as low-frequency parameter fluctuations can be enhanced by thermal fields. Finally, we study how artificial atoms react to changes in inherent properties of the light fields. We perform a detailed analysis of the photon statistics of thermal fields using their relation to the qubits coherence properties. We quantitatively recover the expected
n2+n-law for the photon number variance and confirm this result by direct correlation measurements. We then show a novel technique for the in-situ conversion of the interaction parity in light-matter interaction. To this end, we couple spatially controlled microwave fields to a flux qubit with two degrees of freedom.
Spin ensembles inside a cavity act as light-matter interfaces that play an eminentrole in the development of future quantum devices. An apparent asset of ensemble-based systems is the collective enhancement of the coupling strength, facilitating astrong interaction between the light and matter components. Particularly promisingin this regard, due to their convenient handling and integrability, are solid statespin ensembles such as nitrogen-vacancy centers in diamond, phosphorous donors in silicon, or rare earth doped crystals. Such ensemble-based setups, however, are almost inevitably inhomogeneously broadened as the different spins of the ensemble typically have different local environments leading to a spectral distribution in their transition frequencies. This so-called inhomogeneous broadening is a major source for decoherence in solid state systems and a major challenge to be addressed for future technical applications.In this thesis, we aim to provide the theoretical framework necessary to describeand understand various effects of inhomogeneously broadened spin ensembles coupled to a single-mode cavity—a system that has been realized in numerous different quantum optical setups and in very different parameter regimes.For macroscopic spin ensembles, i.e., ensembles consisting of a vast number ofspins, quantum fluctuations of the individual spins can typically be neglected, allowing a semiclassical description based on Maxwell-Bloch equations. Here, we study two prominent effects in the strongly nonlinear regime namely optical bistability, resembling a first-order phase transition, and critical slowing down. In particular, we show that the onset of bistability not only depends on the width of the spectral spin distribution but also strongly depends on its exact shape. Furthermore, we analyze the transient times of the cavity amplitude which show a power-law divergence when an external parameter is changed in the vicinity of the phase transition.This critical slowdown is demonstrated in collaboration with the group ofJörg Schmiedmayer at the Atominstitut of TU Wien. In the experiment, negativelycharged nitrogen vacancy centers in diamond are strongly coupled to a superconducting microwave resonator showing transient times of up to 11 hours.In mesoscopic spin ensembles with moderate numbers of constituents, quantumfluctuations gain importance, and semiclassical methods fail. We study thiscrossover between the semiclassical and the quantum regime using a cumulant expansion approach to study the semiclassical-to-quantum boundary for inhomogeneously broadened spin ensembles inside a cavity. In addition, we develop a time-adaptivevariational renormalization group method to calculate the full quantumdynamics of spin ensembles containing up to one hundred spins. With the aid ofthis method, we examine mesoscopic spin ensembles whose spin distributions form a comb-shaped structure. These so-called atomic frequency combs have promising properties for the storage of quantum information. On the one hand, we show that arbitrary multi-photon states are absorbed by the comb-shaped spin ensembleand re-emitted into the cavity at periodic time intervals. On the other hand, wedemonstrate that by means of such a spin ensemble a coherent input pulse can beconverted into periodic pulses of non-classical light.Finally, we address spin echoes, which are a fundamental part in nuclear magneticresonance as well as in electron spin resonance. Specifically, we transfer the Hahnecho to the strong coupling regime, where we find a new dynamical phenomenonfeaturing a periodic sequence of self-sustained echoes after a conventional Hahn echo pulse. In collaboration with the group of Hans Hübl at the Technical UniversityMunich, a first demonstration of this intriguing multiecho signature is presented inan electron spin resonance experiment with phosphorus donors in silicon.
In this thesis, experimentally relevant aspects and open questions of quantum information processing and measurement in circuit quantum electrodynamics have been investigated theoretically. Circuit quantum electrodynamics is a relatively young field combining superconducting transmission line resonators on-chip with superconducting quantum bits which serve as artificial atoms. Remarkable experiments have underlined the prospects of circuit QED as a possible architecture for quantum information processing as well as a framework within which quantum optics experiments can be performed. In contrast to their optical counterparts, these experiments reach the ultra-strong coupling limit and allow e.g. the generation of Fock states, the study of decoherence and the observation of quantum jumps. We present the physics of superconducting circuits based on the Josephson junction as a non-linear circuit element. We discuss the various types of quantum bits (qubits) before turning to an introduction on cavity QED and conclude the introduction with a brief presentation of the most relevant experiments and a short introduction to the principles and prospects of quantum information processing. Building on the pioneering theoretical and experimental work in which up to three qubits have been integrated on a chip and successfully coupled via a cavity mode, we propose a scheme to overcome the natural limits concerning scalability in these systems. Usually, scalability is severely limited by the resonance width of the qubit transitions and the attainable frequency range for both qubit transition and cavity resonance frequencies. This limits the present setups to at most ten qubits. As a possible solution, we propose and investigate a cross-bar grid layout of cavities with qubits at the intersections. It turns out that this setup, allowing for up to about 1000 qubits, offers significant advantages over e.g. nearest-neighbor coupling schemes. In addition, it can serve as a building block for a truly scalable scheme for fault-tolerant quantum information processing with superconducting circuits by combining 7x7 arrays in a staircase manner. Furthermore, we discuss and simulate different possibilities to improve upon the suggested scheme by e.g. using resonant gates and optimal control theory. Another focus of the present thesis is measurement physics. In order to investigate e.g. the possibilities of using a circuit QED system to dispersively detect single microwave photons or to generate multi-qubit entangled states, we introduce in a pedagogical manner the basics of stochastic master equations which generate quantum trajectories before turning to concrete applications. Quantum trajectories have proven to be a state-of-the-art tool to analyze measurement situations in a very realistic manner by giving access to both the measurement record as well as the internal quantum dynamics conditioned on this record. Using the method of quantum trajectories as generated by stochastic master equations, we discuss a scheme to efficiently generate multi-qubit entangled states in a very flexible way. The method is based on a collective, dispersive qubit readout. By this measurement, a suitable product state of N qubits can be reliably converted into e.g. an N-qubit Greenberger-Horne-Zeilinger or W state. We propose and discuss the scheme and investigate the effects of decoherence and parameter spread as they would be encountered in experiment. Last but not least, we propose and fully analyze a scheme to dispersively detect single itinerant microwave photons. While experiments to generate single microwave photons have already been successfully performed, their single-shot quantum non-demolition detection has not been possible so far. The scheme presented in this thesis closes this gap in the circuit QED toolbox and reaches detection efficiencies of 30% only limited by fundamental quantum mechanics in this case the Quantum Zeno effect. This detection scheme could be used in quantum communication or quantum cryptography applications.
Circuit Quantum Electrodynamics (cQED), the study of the interaction between superconducting circuits behaving as artificial atoms and 1-dimensional transmission-line resonators, has shown much promise for quantum information processing tasks.For the purposes of quantum computing it is usual to approximate the artificial atoms as 2-level qubits, and much effort has been expended on attempts to isolate these qubits from the environment and to invent ever more sophisticated control and measurement schemes.Rather than focussing on these technological aspects of the field, this thesis investigates the opportunities for using these carefully engineered systems for answering questions of fundamental physics.The low dissipation and small mode volume of the circuits allows easy access to the strong-coupling regime of quantum optics, where one can investigate the interaction of light and matter at the level of single atoms and photons.A signature of strong coupling is the splitting of the cavity transmission peak into a pair of resolvable peaks when a single resonant atom is placed inside the cavity-an effect known as vacuum Rabi splitting.The cQED architecture is ideally suited for going beyond this linear response effect.This thesis shows that increasing the drive power results in two unique nonlinear features in the transmitted heterodyne signal: the supersplitting of each vacuum Rabi peak into a doublet, and the appearance of additional peaks with the characteristic √ n spacing of the Jaynes-Cummings ladder.These constitute direct evidence for the coupling between the quantized microwave field and the anharmonic spectrum of a superconducting qubit acting as an artificial atom.This thesis also addresses the idea of Bell tests, which are experiments that aim to disprove certain types of classical theories, presenting a proposed method for preparing maximally entangled 3-qubit states via a 'preparation by measurement' scheme using an optimized filter on the time-dependent signal obtained via homodyne monitoring of the transmitted microwave field.
Artificially engineered atoms, built using superconducting electrical circuits, have had a broad impact on the field of quantum information and quantum computing. Based on the Josephson effect, superconducting qubits have provided a robust platform for engineering light-matter interactions at the single-photon level. The ability to precisely control and manipulate single photons using superconducting qubits and cavities, a field now popularly known as circuit quantum electrodynamics (circuit QED), has enabled new and novel regimes in quantum physics, which previously remained inaccessible. For instance, the coupling between individual photons and artificial atoms have been shown to reach the ultrastrong and deep-strong regimes, a feat which is difficult to achieve with natural atoms. The superconducting circuit platform is now a promising contender for building large-scale quantum processors, attracting large investments from academic, industry and government players. \n \nThis thesis uses superconducting circuits to engineer photon interactions in two separate studies. The first is aimed at studying the physics of ``giant" artificial-atoms. The second study explores the route towards building a quantum heat engine using two parametrically-coupled, superconducting microwave cavities. We review the theoretical ideas and concepts which motivate our work, along with discussions of the design methodology, simulations, fabrication, measurement setup and the experimental findings. \n \nIn the first study, we explore a giant artificial atom, formed from a transmon qubit, which is coupled to propagating microwaves at multiple points along an open transmission line. The multipoint coupling nature of the transmon allows its radiated field to interfere with itself leading to some striking ``giant" atom effects. For instance, we observe strong frequency dependent couplings of the transmon's transition levels to its electromagnetic environment, a feature which is not observed with ordinary artificial atoms. We measure large on/off ratios, as high as
380, for the coupling rate of the
ket0−ket1 transition. Furthermore, we show that we can enhance or suppress the coupling rate of the
ket1−ket2 transition relative to the
ket0−ket1 transition, by more than a factor of
200. The relative modulation of the coupling rates was exploited to engineer a metastable state in the giant transmon and demonstrate electromagnetically-induced transparency (EIT), a typical signature of a lambda system. Our results show that we can transform the ladder structure of an ordinary transmon into a more interesting lambda system using a giant transmon, thereby paving the way for exploring new possibilities to study three-level physics in a waveguide-QED setting. \n \nExtending giant atom physics to multiple giant atoms, we then explore a device with two giant artificial atoms connected in a braided configuration to a transmission line. The braided topology of the qubits, offers an interesting regime where the qubits can interact with each other in a decoherence-free environment, where the interaction is mediated by virtual photons in the transmission line. We probe the resonant behavior of the qubits at two different frequency bias points, where we observe qualitatively different scattering behavior. Furthermore, when probing for the Autler-Townes Splitting (ATS), multiple resonances are observed for both resonant and off-resonant cases instead of the familiar doublet in the ATS spectroscopy. This comes as a surprise as the frequency-level spacings in both qubits are nominally identical. We believe these features could be an indication of a novel resonant interaction between the qubits facilitated by the braided topology. An effort to understand this theoretically is underway. \n \nFor our second study, we explore a system with two parametrically-coupled superconducting resonators, which implements an optomechanical-like interaction in an all-electrical network. The nonlinear nature of this interaction is mediated by a superconducting quantum interference device (SQUID), where the current in one resonator couples to the photon number in the other resonator. We propose to use this system to build a ``photonic piston" engine in the quantum regime. We motivate the feasibility of the proposal by reviewing key theoretical results which demonstrate an Otto-cycle by appropriately driving the system with noise. Our experimental findings demonstrate the crucial nonlinear coupling that is required for the engine to work. We also show that we can increase the coupling strength between the resonators depending on the chosen flux operating point.