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Journal of Physics Conference Series

Measurements of quantum defect in RydbergD-states for lithium atoms

D A Murashkin, Sergey A. Saakyan, Vladimir A. Sautenkov, Boris B. Zelener

Published Nov 1, 2016• 1 citation
Publisher

Abstract

We have developed an effective spectroscopic method for measure the energy spectra of highly excited ultracold atoms using the registration of resonance fluorescence of atoms in magneto-optical trap during two-step cw excitation of Rydberg states by uv laser. Using this method it was obtained the value of the quantum defect was determined for Rydberg states nD of lithium-7 atoms δ = 0.00192(17).

DOI
10.1088/1742-6596/774/1/012166

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Journal of Physics Conference Series•Nov 1, 2016•0 citations
We have developed an effective spectroscopic method for measure the energy spectra of highly excited ultracold atoms using the registration of resonance fluorescence of atoms in magneto-optical trap during two-step cw excitation of Rydberg states by uv laser. Using this method it was obtained the value of the quantum defect was determined for Rydberg states nD of lithium-7 atoms δ = 0.00192(17).
The spectra of excited lithium-7 atoms prepared in a magneto-optical trap are studied using a UV laser. The laser diagnostics of the energy of Rydberg atoms is developed based on measurements of the change in resonance fluorescence intensity of ultracold atoms as the exciting UV radiation frequency passes through the Rydberg transition frequency. The energies of various nS configurations are obtained in a broad range of the principal quantum number n from 38 to 165. The values of the quantum defect and ionization energy obtained in experiments and predicted theoretically are discussed.
In this work, we discuss two-photon excitation and diagnostic of ultracold Rydberg atoms in a magneto-optical trap. Lithium atoms were excited by using ultraviolet cw laser. For identification of Rydberg transitions, we recorded resonance fluorescence of ultracold atoms. Spectra of transitions 2P- n S, 2p- n D were measured. Our results are in good agreement with calculations and experimental data available in literature. Presented work is a part of our project focused on preparation and study of Rydberg matter and ultracold plasma.
This work is aimed at preparing highly excited optically cooled lithium-7 atoms for producing a strongly nonideal plasma and Rydberg matter. A setup implementing a novel nondestructive technique for preparation and diagnostics of highly excited Rydberg atomic states is constructed. The operation of this setup is based on the usage of a cw high-power ultraviolet laser combined with a magneto-optical trap. The diagnostics of highly excited states is performed by the direct recording of the variations in the fluorescence of ultracold lithium-7 atoms in the magneto-optical trap.
Energy spectra of ultracold Rydberg lithium atoms are discussed. Our technique has been used for the experimental observation of coherent and non-coherent components of two-step excitation in Rydberg states. The high sensitivity of the technique has allowed us to record narrow coherent resonance at 2 P -41 D . The width of this resonance is 3 times less than width of non-coherent resonance. The coherent resonance is observed when the laser is detuned by ±803.5 MHz from the atomic transition 2 P 3/2 .