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Physical Review A

Light shifts in a pulsed cold-atom coherent-population-trapping clock

E. Blanshan, Simon Rochester, Elizabeth A. Donley, John E. Kitching

Published Apr 10, 2015• 42 citations
Publisher

Abstract

Field-grade atomic clocks capable of primary standard performance in compact physics packages would be of significant value in applications ranging from network synchronization to inertial navigation. A coherent-population-trapping clock featuring laser-cooled $^{87}\mathrm{Rb}$ atoms and pulsed Ramsey interrogation is a strong candidate for this technology if the frequency biases can be minimized and controlled. Here we characterize the light shift in a cold-atom coherent-population-trapping clock, explaining observed shifts in terms of phase shifts that arise during the formation of dark-state coherences combined with optical-pumping effects caused by unwanted incoherent light in the interrogation spectrum. Measurements are compared with existing and new theoretical treatments, and a laser configuration is identified that would reduce clock frequency uncertainty from light shifts to a fractional frequency level of $\ensuremath{\Delta}\ensuremath{\nu}/\ensuremath{\nu}=4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}14}$ per 100 kHz of laser frequency uncertainty.

DOI
10.1103/physreva.91.041401

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Field-grade atomic clocks capable of primary standard performance in compact physics packages would be of significant value in applications ranging from network synchronization to inertial navigation. A coherent-population-trapping clock featuring laser-cooled 87Rb^{87}\mathrm{Rb}87Rb atoms and pulsed Ramsey interrogation is a strong candidate for this technology if the frequency biases can be minimized and controlled. Here we characterize the light shift in a cold-atom coherent-population-trapping clock, explaining observed shifts in terms of phase shifts that arise during the formation of dark-state coherences combined with optical-pumping effects caused by unwanted incoherent light in the interrogation spectrum. Measurements are compared with existing and new theoretical treatments, and a laser configuration is identified that would reduce clock frequency uncertainty from light shifts to a fractional frequency level of \ensuremathΔ\ensuremathν/\ensuremathν=4\ifmmode×\else\texttimes\fi10\ensuremath−14\ensuremath{\Delta}\ensuremath{\nu}/\ensuremath{\nu}=4\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}14}\ensuremathΔ\ensuremathν/\ensuremathν=4\ifmmode×\else\texttimes\fi10\ensuremath−14 per 100 kHz of laser frequency uncertainty.
Field-grade atomic clocks capable of primary standard performance in compact physics packages would be of significant value in a variety of applications ranging from network synchronization and secure communications to GPS hold-over and inertial navigation. A cold-atom coherent population trapping (CACPT) clock featuring laser-cooled 87RB atoms and pulsed Ramsey interrogation is a strong candidate for this technology if the principal frequency shifts can be controlled and the performance degradation associated with miniaturization can be overcome. In this thesis, research focused on the development of this type of compact atomic clock is presented. To address the low atom numbers obtained in small cold-atom sources, experiments were performed in which an atomic beam was decelerated with bichromatic stimulated laser forces and loaded into a mm-scale magneto-optical trap, increasing the atom number by a factor of 12.5x. A CACPT clock using the high-contrast lin||lin optical interrogation technique was developed and achieved a stability of 7 × 10-13 after one hour of integration. Doppler shifts in the clock are explained using a simple kinematic model and canceled by interrogating the atoms with a counter-propagating CPT configuration. Finally, a thorough characterization of the AC-stark effect in lin||lin CPT was performed. Observed shifts are explained in terms of contributions from coherent CPT-generating couplings and population transfer effects caused by optical pumping from incoherent light. Measurements are compared with existing and new theoretical treatments, and a laser configuration is identified that reduces clock drift from light shifts to less than 10-14 for the current system.
A compact cold-atom clock based on coherent population trapping (CPT) has been developed. The clock typically demonstrates a short-term fractional frequency stability of 4×10−11/√τ, limited by frequency noise on the interrogation lasers. The clock interrogates a sample of 2×105atoms under free-fall with typical cycle and Ramsey periods of 50 ms and 16 ms, respectively. The largest two systematic frequency shifts that can limit the clock's long-term stability are the light shift and the Doppler shift.
An upgrade in the laser system for our cold-atom clock based on coherent population trapping is described that makes use of an electro-optic modulator to significantly improve the phase coherence of the interrogation spectrum relative to what was achieved with our previous phase-locked loop approach. With this improvement in phase coherence, we have observed a reduction in the light shift by over two orders of magnitude. We present the impact of this improvement on the performance of the clock, for which the light shift was previously dominated by the incoherent light in the laser spectrum. We also demonstrate a new optical setup to reduce the Doppler shift.
We present a coherent population trapping clock system based on laser-cooled 87Rb atoms. The clock consists of a frequency-stabilized CPT interrogation laser and a cooling laser as well as a compact magneto-optical trap, a high-performance microwave synthesizer, and a signal detection system. The resonance signal in the continuous wave regime exhibits an absorption contrast of ∼ 50%. In the Ramsey interrogation method, the linewidth of the central fringe is 31.25 Hz. The system achieves fractional frequency stability of 2.4 × 10 − 11 / τ , which goes down to 1.8 × 10−13 at 20000 s. The results validate that cold atom interrogation can improve the long-term frequency stability of coherent population trapping clocks and holds the potential for developing compact/miniature cold atoms clocks.
A review of a cold-atom clock based on coherent population trapping that highlights recent progress will be presented. Improvements in the coherence of the interrogation spectrum have resulted in the generation of dark states in the cold Rb atoms with essentially 100 % transmission – evidence that decoherence in this system is negligible. This improvement in coherence has resulted in improved short-term stability at the level of 1.5E-11 fractional frequency stability for a one second integration period. In combination with improved interrogation schemes, the improved spectrum has also resulted in dramatically smaller light shifts and improved long-term frequency stability – with the clock averaging down to the level of 1E-13 fractional frequency stability on time scales of over 10,000 seconds.
Sophisticated Ramsey-based interrogation protocols using composite laser pulse sequences have been recently proposed to provide next-generation high-precision atomic clocks with a near perfect elimination of frequency shifts induced during the atom-probing field interaction. We propose here a simple alternative approach to the autobalanced Ramsey interrogation protocol and demonstrate its application to a cold-atom microwave clock based on coherent population trapping (CPT). The main originality of the method, based on two consecutive Ramsey sequences with different dark periods, is to sample the central Ramsey fringes with frequency jumps finely adjusted by an additional frequency-displacement concomitant parameter, scaling as the inverse of the dark period. The advantage of this displaced frequency-jump Ramsey method is that the local oscillator (LO) frequency is used as a single physical variable to control both servo loops of the sequence, simplifying its implementation and avoiding noise associated with controlling the LO phase. When tested using a CPT cold-atom clock, the DFJR scheme reduces the sensitivity of the clock frequency to variations of the light shifts by more than an order of magnitude compared with the standard Ramsey interrogation. This simple method can be applied in a wide variety of Ramsey-spectroscopy based applications including frequency metrology with CPT-based and optical atomic clocks, mass spectrometry, and precision spectroscopy.