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arXiv:1903.00566 · Applied Physics Letters

Reduction of light shifts in Ramsey spectroscopy with a combined error signal

M. Shuker, J. W. Pollock, Rodolphe Boudot, V. I. Yudin, A. V. Taichenachev, J. Kitching, E. A. Donley

Published Apr 8, 2019• 27 citations
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Abstract

Light-induced frequency shifts can be a key limiting contribution to the mid- and long-term frequency instabilities in atomic clocks. In this letter, we demonstrate the experimental implementation of the combined error signal interrogation protocol to a cold-atom clock based on coherent population trapping (CPT) and Ramsey spectroscopy. The method uses a single error signal that results from the normalized combination of two error signals extracted from two Ramsey sequences of different dark periods. The single combined error signal is used to stabilize the atomic clock frequency. Compared to the standard Ramsey-CPT interrogation, this method reduces the clock frequency sensitivity to light-shift variations by more than one order of magnitude. This method can be applied in various kinds of Ramsey-based atomic clocks, sensors, and instruments.

DOI
10.1063/1.5093921

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Light-induced frequency shifts can be a key limiting contribution to the mid- and long-term frequency instabilities in atomic clocks. In this letter, we demonstrate the experimental implementation of the combined error signal interrogation protocol to a cold-atom clock based on coherent population trapping (CPT) and Ramsey spectroscopy. The method uses a single error signal that results from the normalized combination of two error signals extracted from two Ramsey sequences of different dark periods. The single combined error signal is used to stabilize the atomic clock frequency. Compared to the standard Ramsey-CPT interrogation, this method reduces the clock frequency sensitivity to light-shift variations by more than one order of magnitude. This method can be applied in various kinds of Ramsey-based atomic clocks, sensors, and instruments.
Light shifts are known to be an important limitation to the mid- and long-term fractional frequency stability of different types of atomic clocks. In this article, we demonstrate the experimental implementation of an anti-light-shift interrogation protocol onto a continuous-wave (cw) microcell atomic clock based on coherent population trapping (CPT). The method, inspired by the autobalanced Ramsey spectroscopy technique demonstrated in pulsed atomic clocks, consists in the extraction of atomic based information from two successive light-shifted clock frequencies obtained at two different laser-power values. Two error signals, computed from the linear combination of signals acquired along a symmetric sequence, are managed in a dual-loop configuration to generate a clock frequency free from light shift. Using this method, the sensitivity of the clock frequency to both laser-power and microwave-power variations can be reduced by more than an order of magnitude compared to normal operation. In the present experiment, the consideration of the nonlinear light-shift dependence allows enhancement of the light-shift mitigation. The implemented technique allows an improvement of the clock Allan deviation for time scales higher than 1000 s. This method can be applied in various kinds of atomic clocks such as CPT-based atomic clocks, double-resonance Rb\mathrm{Rb}Rb clocks, or cell-stabilized lasers.
Sophisticated Ramsey-based interrogation protocols using composite laser pulse sequences have been recently proposed to provide next-generation high-precision atomic clocks with a near perfect elimination of frequency shifts induced during the atom-probing field interaction. We propose here a simple alternative approach to the autobalanced Ramsey interrogation protocol and demonstrate its application to a cold-atom microwave clock based on coherent population trapping (CPT). The main originality of the method, based on two consecutive Ramsey sequences with different dark periods, is to sample the central Ramsey fringes with frequency jumps finely adjusted by an additional frequency-displacement concomitant parameter, scaling as the inverse of the dark period. The advantage of this displaced frequency-jump Ramsey method is that the local oscillator (LO) frequency is used as a single physical variable to control both servo loops of the sequence, simplifying its implementation and avoiding noise associated with controlling the LO phase. When tested using a CPT cold-atom clock, the DFJR scheme reduces the sensitivity of the clock frequency to variations of the light shifts by more than an order of magnitude compared with the standard Ramsey interrogation. This simple method can be applied in a wide variety of Ramsey-spectroscopy based applications including frequency metrology with CPT-based and optical atomic clocks, mass spectrometry, and precision spectroscopy.
Abstract Light shifts induced during atom–light interactions significantly affect the medium- and long-term frequency stability of atomic clocks. Here, we employ composite laser pulse sequences to mitigate interrogation-induced light shifts in a cold-atom coherent-population-trapping clock. We obtain the anti-symmetry error signal via modulating the local oscillator phase in the free-evolution time of Ramsey interferometry. Utilizing this signal, we employ two feedback loops to simultaneously eliminate light shifts and stabilize the clock frequency using the auto-balanced Ramsey (ABR) spectroscopy scheme. Our experimental results demonstrate that this approach can reduce the clock frequency’s sensitivity to variations in light shifts by implementing four Ramsey sub-sequences. Furthermore, we show that the ABR spectroscopy scheme enhances the long-term frequency stability of the atomic clock when the averaging time τ > 5000 s.
We present a rigorous justification for the applicability of the recently developed methods of generalized autobalanced Ramsey spectroscopy (GABRS) [V. I. Yudin et al., Phys. Rev. Appl. 9, 054034 (2018)] and combined error signal in Ramsey spectroscopy (CESRS) [ , New J. Phys. 20, 123016 (2018)] for resonances of coherent population trapping (CPT). A protocol of modified combined error signal for CPT resonances is also proposed, in which two successive interrogations of atoms under different times of free evolution are integrated in one cycle. The implementation of the GABRS and CESRS methods in a compact atomic clock based on the CPT effect allows us to significantly suppress the light shift and its fluctuation, which will lead to an improvement in the long-term stability and accuracy of these devices. Moreover, these spectroscopic schemes are insensitive to various distortions of the pulse shape, relaxation processes, errors in the generation of phase jumps, etc., which provides their high reliability and immunity to perturbations.
We have developed a universal method to form the reference signal for the stabilization of arbitrary atomic clocks based on Ramsey spectroscopy. Our approach uses an interrogation scheme of the atomic system with two different Ramsey periods and a specially constructed combined error signal (CES) computed by subtracting two error signals with the appropriate calibration factor. CES spectroscopy allows for perfect elimination of probe-induced light shifts and does not suffer from the effects of relaxation, time-dependent pulse fluctuations and phase-jump modulation errors and other imperfections of the interrogation procedure. The method is simpler than recently developed auto-balanced Ramsey spectroscopy techniques (Sanner et al 2018 Phys. Rev. Lett. 120 053602; Yudin et al 2018 Phys. Rev. Appl. 9 054034), because it uses a single error signal that feeds back on the clock frequency. The use of CES is a general technique that can be applied to many applications of precision spectroscopy.
We investigate the application of Ramsey spectroscopy for the development of a microcell atomic clock based on coherent population trapping (CPT). The dependence of the central Ramsey-CPT fringe properties on key experimental parameters is first studied for optimization of the clock’s short-term frequency stability. The sensitivity of the clock frequency to light-shift effects is then studied. In comparison with the continuous-wave (CW) regime case, the sensitivity of the clock frequency to laser power variations is reduced by a factor up to 14 and 40.3 for dark times of 150 and450 μs450~\mu \text{s}450 μs, respectively, at the expense of intensity 3.75 times higher for short-term stability optimization. The dependence of the clock frequency on the microwave power is also reduced in the Ramsey case. We demonstrate that the Ramsey-CPT interrogation improves the clock Allan deviation for averaging times higher than 100 s. With a dark time of450 μs450~\mu \text{s}450 μs, a clock fractional frequency stability of3.8×10−123.8 \times 10^{-12}3.8×10−12at 104s is obtained, in comparison with the level of8×10−118\times 10^{-11}8×10−11obtained in the standard CW case, in similar environmental conditions. These results demonstrate that Ramsey-based interrogation protocols might be an attractive approach for the development of chip-scale atomic clocks (CSACs) with enhanced mid- and long-term stability.