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Optica

Spectral multiphoton effects and quantum anharmonicities in dissipative cavity-QED systems via off-resonant coherent excitation

E. Illes, C. Roy, Stephen Hughes

Published Jul 31, 2015• 7 citations
Publisher

Abstract

The Jaynes–Cummings (JC) model has been the theoretical workhorse for understanding cavity quantum electrodynamics (QED) and for exploring multiphoton effects caused by the quantization of light. Today, it is an indispensable tool used to describe a variety of quantum optical systems, including semiconductor quantum-dot (QD) cavities, atoms in cavities, and superconducting circuits. Unfortunately, dissipation in many cavity-QED systems, especially QD structures, can strongly inhibit any direct spectral features of higher lying photon states and their spectral anharmonicities. In this work, we introduce a strategy to directly access and probe these multiphoton states and show that they can be directly observed even in the presence of a significant amount of dissipation. Our excitation scheme employs off-resonant excitation of a coupled QD cavity system using a nonlinear coherent drive, and the computed fluorescence spectra demonstrate the feasibility of the direct spectroscopic observation of higher rungs of the JC ladder using realistic QD cavity systems.

DOI
10.1364/optica.2.000689

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The Jaynes–Cummings (JC) model has been the theoretical workhorse for understanding cavity quantum electrodynamics (QED) and for exploring multiphoton effects caused by the quantization of light. Today, it is an indispensable tool used to describe a variety of quantum optical systems, including semiconductor quantum-dot (QD) cavities, atoms in cavities, and superconducting circuits. Unfortunately, dissipation in many cavity-QED systems, especially QD structures, can strongly inhibit any direct spectral features of higher lying photon states and their spectral anharmonicities. In this work, we introduce a strategy to directly access and probe these multiphoton states and show that they can be directly observed even in the presence of a significant amount of dissipation. Our excitation scheme employs off-resonant excitation of a coupled QD cavity system using a nonlinear coherent drive, and the computed fluorescence spectra demonstrate the feasibility of the direct spectroscopic observation of higher rungs of the JC ladder using realistic QD cavity systems.
Interaction between light and matter generates optical nonlinearities, which are particularly pronounced in the quantum strong coupling regime. When a single bosonic mode couples to a single fermionic mode, a Jaynes–Cummings (JC) ladder is formed, which we realize here using cavity photons and quantum dot excitons. We measure and model the coherent anharmonic response of this strongly coupled exciton–cavity system at resonance. Injecting two photons into the cavity, we demonstrate a larger polariton splitting with respect to the vacuum Rabi splitting. This is achieved using coherent nonlinear spectroscopy, specifically four-wave mixing, where the coherence between the ground state and the first (second) rung of the JC ladder can be interrogated for positive (negative) delays. With increasing excitation intensity and thus rising average number of injected photons, we observe spectral signatures of the quantum-to-classical crossover of the strong coupling regime.
We investigate the cavity excitation spectrum and the photon number distribution in a cavity QED system driven by a broadband squeezed vacuum. In an empty cavity, we show that only states with even number of photons can be measured under resonant condition since the squeezed vacuum consists of states with even number of photons only. When a single atom is trapped in the cavity, the strong coupling between the atom and cavity results in energy splittings of the system, and there exist two peaks in the cavity excitation spectrum at two-photon transition frequencies. At the central frequency, however, all photon states can be detected because of the interaction between the atom and cavity. Therefore, it can be used to detect whether a single atom is trapped in the cavity. We also show that the squeezed vacuum can promote multiphoton excitations in the cavity. Using a coherent probe field, it is possible to explore higher Jaynes-Cummings doublet even if the probe field intensity is very weak.
Light and matter can be unified under the strong coupling regime, creating superpositions of both, called dressed states or polaritons. After initially being demonstrated in bulk semiconductors and atomic systems ,strong coupling phenomena have been realized in solid state optical microcavities. They form an essential ingredient in the exciting physics spanning from many-body quantum coherence phenomena, like Bose-Einstein condensation and superfluidity, to cavity quantum electrodynamics (cQED). A widely used approach within cQED is the Jaynes-Cummings (JC) model that describes the interaction of a single fermionic two-level system with a single bosonic photon mode. For a photon number larger than one, known as quantum strong coupling (QSC), a significant anharmonicity is predicted for the ladder-like spectrum of dressed states. For optical transitions in semiconductor nanostructures, first signatures of the quantum strong coupling were recently published. In our latest report we applied advanced coherent nonlinear spectroscopy to explore a strongly coupled exciton-cavity system. Specifically, we measured and simulated its four-wave mixing (FWM) response, granting direct access to the first two rungs of the JC ladder. This paper summarizes the main results of Ref. 15 and adds FWM experiments obtained on a micropillar cavity in which a doublet of quantum dot (QD) excitons interacts with the cavity mode in the limit of weak to strong coupling.
We theoretically study the bichromatic driving of a solid-state cavity quantum electrodynamics (QED) system as a means of probing cavity dressed state transitions and observing the coherent interaction between the system and the light field. We show that this method can enable the observation of the higher order cavity dressed states, supersplitting and ac-Stark shift in a solid-state system comprised of a quantum dot (QD) strongly coupled to a photonic crystal cavity for the on- and far off-resonant cases. For the off-resonant case, phonons mediate off-resonant coupling between the QD and the photonic resonator, a phenomenon unique to solid-state cavity QED.
We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom cavity quantum electrodynamics (CQED) system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon excitations in the CQED system, it is possible to observe the direct three-photon excitation of the higher-order ladder states of the CQED system. We report an experiment with cold Rb atoms confined in an optical cavity and demonstrate such interference control of the multiphoton excitations of the CQED system. The observed nonlinear excitation of the CQED ladder states agrees with a theoretical analysis based on a fully quantized treatment of the CQED system, but disagrees with the semiclassical analysis of the CQED system. Thus it represents a direct observation of the quantum nature of the multiatom CQED system and opens new ways to explore quantum nonlinearity and its applications in quantum optical systems in which multiple absorbers or emitters are coupled with photons in confined cavity structures.