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arXiv:1507.01630 · Physical Review A

Quantum nonlinear cavity quantum electrodynamics with coherently prepared atoms

Guoqing Yang, Wen-ju Gu, Gao‐xiang Li, Bichen Zou, Yifu Zhu

Published Sep 14, 2015• 13 citations
arXivHTMLPDF

Abstract

We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom cavity quantum electrodynamics (CQED) system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon excitations in the CQED system, it is possible to observe the direct three-photon excitation of the higher-order ladder states of the CQED system. We report an experiment with cold Rb atoms confined in an optical cavity and demonstrate such interference control of the multiphoton excitations of the CQED system. The observed nonlinear excitation of the CQED ladder states agrees with a theoretical analysis based on a fully quantized treatment of the CQED system, but disagrees with the semiclassical analysis of the CQED system. Thus it represents a direct observation of the quantum nature of the multiatom CQED system and opens new ways to explore quantum nonlinearity and its applications in quantum optical systems in which multiple absorbers or emitters are coupled with photons in confined cavity structures.

DOI
10.1103/physreva.92.033822

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We propose a method to study the quantum nonlinearity and observe the multiphoton transitions in a multiatom cavity quantum electrodynamics (CQED) system. We show that by inducing simultaneously destructive quantum interference for the single-photon and two-photon excitations in the CQED system, it is possible to observe the direct three-photon excitation of the higher-order ladder states of the CQED system. We report an experiment with cold Rb atoms confined in an optical cavity and demonstrate such interference control of the multiphoton excitations of the CQED system. The observed nonlinear excitation of the CQED ladder states agrees with a theoretical analysis based on a fully quantized treatment of the CQED system, but disagrees with the semiclassical analysis of the CQED system. Thus it represents a direct observation of the quantum nature of the multiatom CQED system and opens new ways to explore quantum nonlinearity and its applications in quantum optical systems in which multiple absorbers or emitters are coupled with photons in confined cavity structures.
We show that by manipulating quantum interference in a multi-atom cavity quantum electrodynamics (CQED) system, the nonlinear excitation of the cavity-atom polariton can be resonantly enhanced while the linear excitation is suppressed. Under the appropriate conditions, it is possible to selectively enhance or suppress the polariton excitation with two free-pace laser fields. We report on an experiment with cold Rb atoms in an optical cavity and present experimental results that demonstrate such interference control of the CQED excitation and its direct application to studies of all-optical switching and cross-phase modulation of the cavity-transmitted light.
We propose and analyze a scheme for controlling coherent photon transmission and reflection in a cavity-quantum-electrodynamics (CQED) system consisting of an optical resonator coupled with three-level atoms coherently prepared by a control laser from free space. When the control laser is off and the cavity is excited by two identical light fields from two ends of the cavity, the two input light fields can be completely absorbed by the CQED system and the light energy is converted into the excitation of the polariton states, but no light can escape from the cavity. Two distinct cases of controlling the perfect photon absorption are analyzed: (a) when the control laser is tuned to the atomic resonance and creates electromagnetically induced transparency, the perfect photon absorption is suppressed and the input light fields are nearly completely transmitted through the cavity; (b) when the control laser is tuned to the polariton state resonance and inhibits the polariton state excitation, the perfect photon absorption is again suppressed and the input light fields are nearly completely reflected from the cavity. Thus, the CQED system can act as a perfect absorber or near-perfect transmitter and/or reflector by simply turning the control laser off or on. Such interference control of the coherent photon-atom interaction in the CQED system should be useful for a variety of applications in optical logical devices.
It has been shown that perfect photon absorption can occur in the linear excitation regime of cavity quantum electrodynamics (CQED), in which photons from two identical light fields coupled into two ends of the cavity are completely absorbed and result in excitation of the polariton state of the CQED system. The output light from the cavity is totally suppressed by destructive interference and the polariton state can only decay incoherently back to the ground state. Here we analyze perfect photon absorption and the onset of optical bistability in the nonlinear regime of the CQED and show that perfect photon absorption persists in the nonlinear regime of the CQED below the threshold of optical bistability. Therefore perfect photon absorption is a phenomenon that can be observed in both linear and nonlinear regimes of CQED. Furthermore, our study reveals that optical bistability is influenced by input-light interference and can be manipulated by varying the relative phase of the two input fields.
We show that by manipulating quantum interference in a multi-atom cavity QED system, the nonlinear excitation of the cavity-atom polariton can be resonantly enhanced while the linear excitation is suppressed. Under appropriate conditions, it is possible to selectively enhance or suppress the polariton excitation with two free-pace laser fields. We report an experiment with cold Rb atoms in an optical cavity and present experimental results that demonstrate such interference control of the cavity QED excitation and its direct applications for studies of all-optical switching and cross-phase modulation of the cavity transmitted light.
We study atomic coherence and interference in four-level atoms confined in an optical cavity and explores the interplay between cavity QED and electromagnetically induced transparency (EIT). The destructive interference can be induced in the coupled cavity-atom system with a free-space control laser tuned to the normal mode resonance and leads to suppression of the normal mode excitation. Then by adding a pump laser coupled to the four-level atoms from free space, the control-laser induced destructive interference can be reversed and the normal mode excitation is restored. When the free-space control laser is tuned to the atomic resonance and forms a Λ-type EIT configuration with the cavity-atom system, EIT is manifested as a narrow transmission peak of a weak probe laser coupled into the cavity mode. With the free-space pump laser driving the cavity-confined atoms in a four-level configuration, the narrow transmission peak of the cavity EIT can be split into two peaks and the dressed intra-cavity dark states are created analogous to the dressed states in free space. We report experimental studies of such coherently coupled cavity-atom system realized with cold Rb atoms confined in an optical cavity and discuss possible applications in quantum nonlinear optics and quantum information science.
The Jaynes–Cummings (JC) model has been the theoretical workhorse for understanding cavity quantum electrodynamics (QED) and for exploring multiphoton effects caused by the quantization of light. Today, it is an indispensable tool used to describe a variety of quantum optical systems, including semiconductor quantum-dot (QD) cavities, atoms in cavities, and superconducting circuits. Unfortunately, dissipation in many cavity-QED systems, especially QD structures, can strongly inhibit any direct spectral features of higher lying photon states and their spectral anharmonicities. In this work, we introduce a strategy to directly access and probe these multiphoton states and show that they can be directly observed even in the presence of a significant amount of dissipation. Our excitation scheme employs off-resonant excitation of a coupled QD cavity system using a nonlinear coherent drive, and the computed fluorescence spectra demonstrate the feasibility of the direct spectroscopic observation of higher rungs of the JC ladder using realistic QD cavity systems.