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arXiv:1104.0898 · New Journal of Physics

Bichromatic driving of a solid-state cavity quantum electrodynamics system

Alexander T. Papageorge, Arka Majumdar, Erik D. Kim, Jelena Vuckovic A

Published Jan 17, 2012• 18 citations
arXivHTMLPDF

Abstract

We theoretically study the bichromatic driving of a solid-state cavity quantum electrodynamics (QED) system as a means of probing cavity dressed state transitions and observing the coherent interaction between the system and the light field. We show that this method can enable the observation of the higher order cavity dressed states, supersplitting and ac-Stark shift in a solid-state system comprised of a quantum dot (QD) strongly coupled to a photonic crystal cavity for the on- and far off-resonant cases. For the off-resonant case, phonons mediate off-resonant coupling between the QD and the photonic resonator, a phenomenon unique to solid-state cavity QED.

DOI
10.1088/1367-2630/14/1/013028

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We theoretically study the bichromatic driving of a solid-state cavity quantum electrodynamics (QED) system as a means of probing cavity dressed state transitions and observing the coherent interaction between the system and the light field. We show that this method can enable the observation of the higher order cavity dressed states, supersplitting and ac-Stark shift in a solid-state system comprised of a quantum dot (QD) strongly coupled to a photonic crystal cavity for the on- and far off-resonant cases. For the off-resonant case, phonons mediate off-resonant coupling between the QD and the photonic resonator, a phenomenon unique to solid-state cavity QED.
In recent experiments on coupled quantum dot (QD) optical cavity systems, a pronounced interaction between the dot and the cavity has been observed even for detunings of many cavity linewidths. This interaction has been attributed to an incoherent phonon-mediated scattering process and is absent in atomic systems. Here, we demonstrate that despite its incoherent nature, this process preserves the signatures of coherent interaction between a QD and a strong driving laser, which may be observed via the optical emission from the off-resonant cavity. Under bichromatic driving of the QD, the cavity emission exhibits spectral features consistent with optical dressing of the QD transition. These cavity emission measurements are more akin to absorption measurements of a strongly driven QD rather than resonance fluorescence measurements. In addition to revealing new aspects of the off-resonant QD-cavity interaction, this result provides a new, simpler means of coherently probing QDs and opens the possibility of employing off-resonant cavities to optically interface QD nodes in quantum networks.
E. L. Ginzton Laboratory, Stanford University, Stanford, California 94305, USA(Dated: March 2011)Off-resonant coupling between a quantum dot and a photonic resonator is a phenomenon uniqueto solid state cavity quantum electrodynamics. We theoretically show that the spectral lineshapeof the emission of a cavity off-resonantly coupled to a quantum dot under bichromatic resonantexcitation can be used to observe signatures of the dressing of the quantum dot. This incoherentchannel provides a convenient means of observing the effects of coherent interaction between thequantum dot and the resonant light field at a wavelength that is spectrally detuned from both.I. INTRODUCTION
Chip-based cavity quantum electrodynamics (QED) devices consisting of a self-assembled InAs quantum dot (QD) coupled to a high quality factor GaAs microdisk cavity are coherently probed through their optical channel using a fiber taper waveguide. We highlight one particularly important aspect of this all-fiber measurement setup, which is the accuracy to which the optical coupling level and optical losses are known relative to typical free-space excitation techniques. This allows for precise knowledge of the intracavity photon number and measurement of absolute transmitted and reflected signals. Resonant optical spectroscopy of the system under both weak and strong driving conditions are presented, which when compared with a quantum master equation model of the system allows for determination of the coherent coupling rate between QD exciton and optical cavity mode, the different levels of elastic and inelastic dephasing of the exciton state, and the position and orientation of the QD within the cavity. Pump-probe measurements are also performed in which a far off-resonant red-detuned control laser beam is introduced into the cavity. Rather than producing a measurable ac Stark shift in the exciton line of the QD, we find that this control beam induces a saturation of the resonant system response. The broad photoluminescence spectrum resulting from the presence of the control beam in the cavity points to sub-band-gap absorption in the semiconductor, and the resulting free-carrier generation, as the likely source of system saturation.
A single quantum dot embedded in a photonic crystal defect cavity allows for the investigation of cavity quantum electrodynamics effects in a solid-state environment. We present experiments demonstrating the quantum nature of this fundamental system in the strong coupling regime. Photon correlation measurements are used to characterize the fundamental properties of this unique system: through these experiments, we identify an unexpected, efficient sustaining mechanism that ensures strong cavity emission and is quantum correlated with the exciton resonance, even when all the quantum dot resonances are far detuned from the cavity mode.
In this work we present an extensive experimental and theoretical investigation of different regimes of strong field light–matter interaction for cavity-driven quantum dot (QD) cavity systems. The electric field enhancement inside a high-Q micropillar cavity facilitates exceptionally strong interaction with few cavity photons, enabling the simultaneous investigation for a wide range of QD-laser detuning. In case of a resonant drive, the formation of dressed states and a Mollow triplet sideband splitting of up to 45 μ eV is measured for a mean cavity photon number . In the asymptotic limit of the linear AC Stark effect we systematically investigate the power and detuning dependence of more than 400 QDs. Some QD-cavity systems exhibit an unexpected anomalous Stark shift, which can be explained by an extended dressed 4-level QD model. We provide a detailed analysis of the QD-cavity systems properties enabling this novel effect. The experimental results are successfully reproduced using a polaron master equation approach for the QD-cavity system, which includes the driving laser field, exciton-cavity and exciton-phonon interactions.
A lot of experimental and theoretical studies of a system in cavity quantum electrodynamics (cavity QED), which consists of two spatially separated quantum emitters strongly coupled to a single optical cavity mode, have recently attracted much interest in the quantum optics community for various quantum information applications. Here, we propose a method for high-order harmonic generation in a photonic crystal microcavity coupled to single semiconductor quantum dots (QDs). The system is coherently driven by a bichromatic laser consisting of the control and signal fields at low input power (a few nanowatts) and the cavity output power via the cavity loss channel is monitored. Via numerical simulations, we thoroughly explore the difference of the generated high-order harmonic spectra between two QDs, one QD, and zero QDs in microcavity. The results clearly indicate that harmonic generation can be significantly enhanced via collective coherent coupling in the case of two spatially separated QDs coupled to the same photonic crystal microcavity mode. In addition, we present a study of the carrier-envelope phase (CEP) effect on high-order harmonic spectra, which may provide the insight of CEP effect in a new regime. Beyond this, our obtained results also apply to other classes of single-mode cavity-QED setup incorporating two-level atoms or comparable solid-state emitters.