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Chinese Physics Letters

Correlation of Exciton and Biexciton from a Single InAs Quantum Dot

Yu-Long Li, Geng Chen, Jian‐Shun Tang, Chuan‐Feng Li

Published Sep 1, 2012• 2 citations
Publisher

Abstract

The peaks of exciton and biexciton from the single quantum dot (QD) micro-photoluminescence spectra are identified by observing the intensity of those peaks in relation to increasing excitation power. In order to further verify the properties of the exciton and biexciton, we perform auto- and cross correlation measurements. Using the former, we confirm the antibunching property of the signal light emitted from the single QD. Using cross correlation measurement, we verify that the exciton and biexciton emissions originate from the same QD and they are strongly correlated with each other. Lastly, we analyze the behavior of the cross correlation function in both the cases of saturated and unsaturated excitation of the QD.

DOI
10.1088/0256-307x/29/9/094201

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We report photon correlation measurements that reveal unique signatures of biexciton and charged exciton emissions in a single self-assembled InAs quantum dot. Biexciton emission exhibits both bunching and antibunching under continuous-wave excitation and only antibunching under pulsed excitation. Cross correlation between biexciton and single-exciton emissions reveals highly asymmetric features due to cascaded emission. Under our excitation conditions, no polarization correlations between the exciton and biexciton emissions were observed.
Single InAs quantum dot (QD) sample was grown by molecular-beam epitaxy (MBE). The Photoluminescences (PL) of the exciton and biexciton in a single QD were measured at 5 K. The PL intensity as a function of the laser excitation power, the fine structure splittings of the exciton and biexciton, and the corresponding linearly polarized emissions were analyzed. By means of Hanbury-Brown and Twiss (HBT) setup, the photon correlation between the PL of exciton and biexciton were measured, which is gave an evidence of the quantum cascade emissions between biexciton and exciton PL.
We report the observation of antibunched emission from single self-assembled InAs quantum dots under various conditions. We have measured the correlation function of the photon emission pertaining to single emission lines from single quantum dots under continuous and pulsed laser excitation, as well as under continuous white light excitation. The measurements were performed under different excitation intensities at liquid helium temperatures on two samples with distinct structures. At higher temperatures (30 K), an antibunching dip was still observed. We have also observed antibunching on a second emission line in the quantum dot spectrum, attributed to the biexciton, demonstrating the possibility of generating photon pairs with a single quantum dot. Polarization correlations on the biexciton and exciton line were also measured in an attempt to generate entangled photon pairs.
We report correlation and cross-correlation measurements of photons emitted under continuous wave excitation by a single II–VI quantum dot (QD) grown by molecular-beam epitaxy. A standard technique of microphotoluminescence combined with an ultrafast photon correlation setup allowed us to see an antibunching effect on photons emitted by excitons recombining in a single CdTe∕ZnTe QD, as well as cross correlation within the biexciton (X2)-exciton (X) radiative cascade from the same dot. Fast microchannel plate photomultipliers and a time-correlated single photon module gave us an overall temporal resolution of 140ps better than the typical exciton lifetime in II–VI QDs of about 250ps.
We investigate the influence of multiple excitons on the photon emission properties of a quantum dot (QD)-cavity system via the master equation for the density matrix. We show that in the intermediate to strong coupling regimes, the multiple excitons lead to the suppressed QD emissions as well as the absence of anti-crossing near zero detuning, arising from the interaction between the multiple excitons and cavity. Furthermore, we analyze the role of the cavity-biexciton detuning in the photon emission properties of cavity and exciton through the second-order correlation function. The small cavity-biexciton detuning yields the significant Purcell effect and the high probability of single photon emissions. The proposed model offers the fundamental approach in developing efficient single-photon emitting devices.