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Superconducting Nanowire Single-Photon Detectors based on TaN Thin Films

Mathematisch-Naturwissenschaftliche Fakult, Adrian Aeschbacher

Published Jan 1, 2011• 0 citations
OpenAlex

Abstract

Superconducting Nanowire Single Photon Detectors (SNSPD) are very fast, low noise devices, that detect single photons over a broad spectral range with practical quantum efficiency. The quantum efficiency drops at a certain deposited energy abruptly, the so called cutoff energy or the corresponding cutoff wavelength. The most common material to fabricate these nanowires is niobium nitride (NbN). A promising material, that has not been used for this purpose before is tantalum nitride (TaN). Many material properties of TaN and NbN are similar, but TaN has a smaller energy gap. This should make the device more sensitive to photons with lower energies. In this thesis, SNSPDs made of NbN and TaN were characterized, the quantum efficiencies were measured and the cutoff criteria were determined and compared. With the use of TaN the cutoff wavelength could be increased significantly. Measurements of quantum efficiency and dark-count rates at several temperatures and operation conditions are presented and discussed. Furthermore, the cutoff criteria are determined and compared between the materials mentioned as well as the experimental results are compared to the theoretical predictions of the detection model.

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Superconducting Nanowire Single Photon Detectors (SNSPD) are very fast, low noise devices, that detect single photons over a broad spectral range with practical quantum efficiency. The quantum efficiency drops at a certain deposited energy abruptly, the so called cutoff energy or the corresponding cutoff wavelength. The most common material to fabricate these nanowires is niobium nitride (NbN). A promising material, that has not been used for this purpose before is tantalum nitride (TaN). Many material properties of TaN and NbN are similar, but TaN has a smaller energy gap. This should make the device more sensitive to photons with lower energies. In this thesis, SNSPDs made of NbN and TaN were characterized, the quantum efficiencies were measured and the cutoff criteria were determined and compared. With the use of TaN the cutoff wavelength could be increased significantly. Measurements of quantum efficiency and dark-count rates at several temperatures and operation conditions are presented and discussed. Furthermore, the cutoff criteria are determined and compared between the materials mentioned as well as the experimental results are compared to the theoretical predictions of the detection model.
Materials with a small superconducting energy gap are expected to favor a high detection efficiency of low-energy photons in superconducting nanowire single-photon detectors. We developed a TaN detector with smaller gap and lower density of states at the Fermi energy than in comparable NbN devices, while other relevant parameters remain essentially unchanged. The observed reduction of the minimum photon energy required for direct detection is in line with model predictions of ≈1/3 as compared to NbN.
Superconducting nanowire single photon detectors (SNSPD) offer excellent performance for infrared single photon detection, combining high efficiency, low timing jitter, low dark count rates and high photon counting rates. Promising application areas for SNSPDs include quantum key distribution, space-to-ground communications and single photon remote sensing [1]. SNSPDs are typically made with ultrathin niobium nitride (NbN) films with thickness 4 nm and a superconducting transition temperature above 9 K. NbN offers high performance in the near infrared but their sensitivity drops at wavelengths beyond 2 um. There is growing interest in potential photon counting applications in the mid infrared domain (for example remote sensing of greenhouse gases in the atmosphere [2]). One way to overcome the wavelength limit in NbN SNSPDs is to use films with a lower superconducting energy gap [3]. Here we report on the study of SNSPDs fabricated with thin films of titanium nitride (TiN). We compare TiN films deposited by atomic layer deposition (ALD) and by magnetron sputtering. The TiN films range in thickness from 5 to 60 nm, with superconducting transition temperatures from ~1 K to 3.5 K. We have analyzed the films via transmission electron microscopy and variable angle spectroscopic ellipsometry. We characterize TiN SNSPDs performance from near to mid-infrared at wavelengths (1-4 um) with fast optical parametric oscillator (OPO) source. We compare the performance of TiN SNSPDs to devices based on other lower gap materials: MoSi, NbTiN, WSi. [1] Natarajan et al Superconductor Science and Technology 25 063001 (2012) [2] Abshire et al Laser Applications to Chemical, Security and Environmental Analysis, (Optical Society of America, 2008) paper LMA4 [3] Verma et al Applied Physics Letters 105 022602 (2014)
Materials with a small superconducting energy gap are expected to favor a high detection efficiency of low-energy photons in superconducting nanowire single-photon detectors. We developed a TaN detector with smaller gap and lower density of states at the Fermi energy than in comparable NbN devices, while other relevant parameters remain essentially unchanged. The observed reduction of the minimum photon energy required for direct detection is in line with model predictions of ≈1/3 as compared to NbN.
Superconducting nanowire single-photon detectors (SNSPDs) are nanodevices usually made from thin niobium nitride (NbN) films. Operated at liquid helium temperature, they can exhibit high detection efficiency with low dark-counts associated with a fast response time and a low timing jitter. Covering a broad detection range from ultraviolet to mid-infrared, SNSPDs are a very attractive alternative to silicon or gallium arsenide based semiconductor detectors for fiber based telecommunication when single-photon sensitivity and high counting rates are necessary. \nEfficient packaging and fiber coupling of a SNSPD is in itself a real challenge and is often a limiting factor in reaching high system quantum efficiency. Our approach makes use of a controlled expansion alloy which has been adequately heat treated to enhance its characteristics for cryogenic operation. This insures the integrity of the optical coupling at cryogenic temperatures while done at room temperature. It also provides a good attenuation for electromagnetic interference due to the high relative permeability of the nickel-iron alloy. The small form factor of this pigtailed optical fiber package makes it versatile and could be easily integrated with a commercial cryogen-free system or simply dipped into a standard helium transport Dewar. We report on our theoretical and experimental methodology to evaluate the optical coupling quality and present the optoelectronic characterization of two devices packaged in this way. Electrical simulation is studied to understand the speed limitation factor inherent to these devices and preliminary speed and jitter measurements are reported.
The spectral detection efficiency and the dark count rate of superconducting nanowire single-photon detectors (SNSPD) have been studied systematically on detectors made from thin NbN films with different chemical compositions. Reduction of the nitrogen content in the 4 nm thick NbN films results in a decrease of the dark count rates more than two orders of magnitude and in a red shift of the cut-off wavelength of the hot-spot SNSPD response. The observed phenomena are explained by an improvement of uniformity of NbN films that has been confirmed by a decrease of resistivity and an increase of the ratio of the measured critical current to the depairing current. The latter factor is considered as the most crucial for both the cut-off wavelength and the dark count rates of SNSPD. Based on our results we propose a set of criteria for material properties to optimize SNSPD in the infrared spectral region.
We have developed a practical superconducting nanowire single photon detector (SNSPD) system with our superconducting thin films and devices fabrication, optical coupling packaging, and cryogenic technology. The SNSPD devices were fabricated from high-quality niobium nitride (NbN) ultra-thin films that were epitaxially grown on single-crystal MgO substrates, and optical cavity structure were applied for improvement of photo absorption efficiency. The SNSPD system was developed based on a compact Gifford-McMahon (GM) cryocooler, in which SNSPD can operate continuously at temperature of 2.9 K +/- 10 mK with low power consumption without any liquid cryogens. The system detection efficiencies at 1550 nm wavelength (at a 100 Hz dark count rate) were found to be 2.6% for device without optical cavity and 21% for device with optical cavity. The response speed of devices showed maximally 200 MHz with 5 × 5 mm square device, and timing jitter of 100 ps full width at a half maximum (FWHM) was observed.