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Conference on Lasers and Electro-Optics

Coupling of Nitrogen-Vacancy Centers to Photonic Crystal Resonators in Monocrystalline Diamond

Andrei Faraon, Zhihong Huang, Víctor M. Acosta, Charles Santori, Raymond G. Beausoleil

Published Jan 1, 2012• 23 citations
Publisher

Abstract

The zero-phonon transition rate for nitrogen-vacancy centers is enhanced by coupling to photonic crystal resonators fabricated in monocrystalline diamond. Autocorrelation measurements on the spectrally filtered zero-phonon line demonstrate coupling of a single emitter.
DOI
10.1364/qels.2012.qm3c.5

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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)•May 1, 2013•1 citation
The zero-phonon transition rate of a nitrogen-vacancy center is enhanced by a factor of ∼70 by coupling to a photonic crystal resonator fabricated in monocrystalline diamond using standard semiconductor fabrication techniques. Photon correlation measurements on the spectrally filtered zero-phonon line show antibunching, a signature that the collected photoluminescence is emitted primarily by a single nitrogen-vacancy center. The linewidth of the coupled nitrogen-vacancy center and the spectral diffusion are characterized using high-resolution photoluminescence and photoluminescence excitation spectroscopy.
The realization of efficient optical interfaces for solid-state atom-like systems is an important problem in quantum science with potential applications in quantum communications and quantum information processing. We describe and demonstrate a technique for coupling single nitrogen vacancy (NV) centers to suspended diamond photonic crystal cavities with quality factors up to 6000. Specifically, we present an enhancement of the NV center's zero-phonon line fluorescence by a factor of ~ 7 in low-temperature measurements.
Nitrogen–vacancy centers in diamond have outstanding quantum optical properties that enable applications in information processing and sensing. As with most solid-state systems for quantum photonic applications, the great promise lies in the capability to embed them in an on-chip optical network. Here we present basic integrated devices composed of diamond micro-ring resonators coupled to waveguides that are terminated with grating out-couplers. Strong enhancement is observed for the zero-phonon line of nitrogen–vacancy centers coupled to the ring resonance. The zero-phonon line is efficiently coupled from the ring into the waveguide and then scattered out of plane by the grating out-couplers.
Summary form only given. Deterministic coupling of a single emitter to a photonic crystal cavity is an important step towards the realization of integrated solid-state devices for quantum photonics. As single emitters, color centers in diamond, e.g. the Nitrogen-Vacancy (NV) center or the Silicon-Vacancy (SiV) center have attracted significant interest due to their extraordinary properties like long spin-coherence times or narrowband and bright single photon emission, respectively. For the realization of recent proposals like cavity-enhanced spin measurements or cavity-enhanced single photon sources, it is necessary to couple single color centers to a cavity with small mode volume and high quality factor. Photonic crystal cavities directly fabricated within a monocrystalline diamond membrane are well suited for this task, as they offer tiny mode volumes for efficient emitter-cavity coupling as well as scalable architectures for integrated photonic devices.In order to achieve controlled coupling of a color center to a photonic crystal cavity, several challenges have to be tackled, e.g. exact emitter positioning and alignment of its dipole moment with the cavity electric field as well as the ability for cavity tuning. For deterministic emitter-cavity positioning, two different routes can be pursued: In the first approach, a single emitter is localized within the diamond, its dipole orientation is determined and the cavity is subsequently structured around it. In the second approach, the cavity is fabricated first and a single color center is created within the cavity, e.g. via ion implantion or creation of vacancies. Here we present strategies to realize both methods for deterministic emitter-cavity coupling. For the first approach, we use a monocrystalline diamond film containing single SiV centers. Figure 1a) shows a fluorescence scan of a single SiV center with position markers next to it. The position markers are subsequently used to structure a photonic crystal cavity around the color center using focused ion beam milling [1]. Figures 1b) and c) show SEMimages before and after the cavity fabrication. The photonic crystal lattice constant a ≈ 283nm is chosen such that the cavity modes are red shifted with respect to the SiV emission lines. Using an oxidation tuning method, the cavity modes are tuned into resonance with the zero-phonon line at 740nm of a single SiV center (see Fig. 1d)). On resonance, we measure an intensity enhancement by a factor of 3.8 compared to the off-resonant case.