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Applied Physics Letters

Multiple copies of orbital angular momentum states through second-harmonic generation in a two-dimensional periodically poled LiTaO3 crystal

Xinyuan Fang, Dunzhao Wei, Dongmei Liu, Weihao Zhong, Rui Ni, Zhenhua Chen, Xiaopeng Hu, Yong Zhang, Shining N. Zhu, Min Xiao

Published Oct 19, 2015• 33 citations
Publisher

Abstract

We experimentally demonstrate multiple copies of optical orbital angular momentum (OAM) states through quasi-phase-matched (QPM) second-harmonic (SH) generation in a 2D periodically poled LiTaO3 (PPLT) crystal. Since the QPM condition is satisfied by involving different reciprocal vectors in the 2D PPLT crystal, collinear and noncollinear SH beams carrying OAMs of l2 are simultaneously generated by the input fundamental beam with an OAM of l1. The OAM conservation law (i.e., l2 = 2l1) holds well in the experiment, which can tolerate certain phase-mismatch between the interacting waves. Our results provide an efficient way to obtain multiple copies of the wavelength-converted OAM states, which can be used to enhance the capacity in optical communications.

DOI
10.1063/1.4934488

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ACS Photonics•Feb 5, 2026•1 citation
We experimentally demonstrate multiple copies of optical orbital angular momentum (OAM) states through quasi-phase-matched (QPM) second-harmonic (SH) generation in a 2D periodically poled LiTaO3 (PPLT) crystal. Since the QPM condition is satisfied by involving different reciprocal vectors in the 2D PPLT crystal, collinear and noncollinear SH beams carrying OAMs of l2 are simultaneously generated by the input fundamental beam with an OAM of l1. The OAM conservation law (i.e., l2 = 2l1) holds well in the experiment, which can tolerate certain phase-mismatch between the interacting waves. Our results provide an efficient way to obtain multiple copies of the wavelength-converted OAM states, which can be used to enhance the capacity in optical communications.
We report that the optical orbital angular momentum (OAM) is conserved in the two-step cascaded nonlinear processes through quasi-phase-matched (QPM) in a dual-structure periodically poled LiTaO!(PPLT) crystal. Because of the different reciprocal vectors provided by the different structures in the crystal, collinear second harmonic (SH) beam with an OAM of l2 and third harmonic (TH) beam with an OAM of l3 are simultaneously generated by the input fundamental beam with an OAM of l1. The OAM conversion law (l2 = 2l1, l3 = 3l1) holds well in this nonlinear process. Our results provide an effective way to obtain three beams (fundamental beam, SH beam, TH beam) with different OAMs at the same time, which can be used to enhance the capacity of optical communication.
Nonlinear interaction between orbital angular momentum (OAM) modes has interesting effects and tremendous applications in both classical and quantum realms. Here we propose a strategy of using perfect vortices, which not only overcomes the spatial mode matching problem of nondegenerate OAM modes, but also reveals the OAM-only influence on the momentum matching by tuning the OAMs of the fundamental wave. We use perfect vortices of degenerate and nondegenerate OAM modes to clearly demonstrate the flexible control of OAM modes on nonlinear interaction by carefully exploring second-harmonic generation (SHG) in periodically poled crystal. We generate second-harmonic perfect vortices with the OAM order up to 40. Based on the observed phase-matching temperature shift caused by OAMs, we also use the SHG nonlinear process to distinctly confirm the OAM-only-induced subluminal effect. Our results pave the way toward unveiling the underlying physics behind nonlinear process of OAM modes and building high-capacity quantum links between systems operating at various wavelengths. The inverse process of SHG we developed, perfect-vortex-based spontaneous parametric down-conversion, may provide a promising solution for high-dimensional OAM entangled source.
We demonstrate energy exchange between two orthogonally polarized optical waves as a consequence of a two-color multistep parametric interaction. The energy exchange results from cascading of two quasi-phase-matched (QPM) second-harmonic parametric processes, and it is intrinsically instantaneous. The effect is observed when both the type-I (ooe) second-harmonic generation process and higher QPM order type-0 (eee) second-harmonic generation processes are phase-matched simultaneously in a congruent periodically-poled lithium niobate crystal. The two second-harmonic generation processes share a common second-harmonic wave which couple the two cross-polarized fundamental components and facilitate an energy flow between them. We demonstrate a good agreement between the experimental data and the results of numerical simulations.
We propose a convenient approach for managing orbital angular momentum (OAM) of second-harmonic photons generated by a quadratic nonlinear interaction under noncolinear type-I phase matching condition. Since the OAMs of two fundamental photons can be flexibly controlled by using computer-generated holograms, we were able to realize arbitrary combination of both OAMs and experimentally confirm the OAM conservation selection rule ${\ensuremath{\ell}}_{2\ensuremath{\omega}}={\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}}+{\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}\ensuremath{'}}$ in general cases. In particular, our approach could be used to generate the second-harmonic photon states with fractional and odd-order OAMs.
We experimentally demonstrate wavelength broadcast based on simultaneous Type I quasi-phase-matched (QPM) broadband sum-frequency generation (SFG) and second-harmonic generation (SHG) in 5 mol.% MgO-doped periodically poled lithium niobate (MgO:PPLN). One signal has been synchronously converted into seven different wavelengths using two pumps at a 1.5 microm band via quadratic cascaded nonlinear wavelength conversion. By selecting different pump regions, i.e., selecting different cascaded chi((2)):chi((2)) interactions, the flexible wavelength conversions with shifting from one signal to single, double, and triple channels were also demonstrated.
Optical vortex beams (OVBs) carrying orbital angular momentum (OAM) offer access to an unbounded set of orthogonal states, enabling a dramatic increase in the information capacity for optical communication systems. However, practical OAM detection in telecommunication platforms remains challenging due to background noise, detector limitations at infrared communication wavelengths, and the destructive nature of conventional sampling methods. Here, we introduce an all-optical, nearly nondestructive OAM detection method based on sum-frequency generation (SFG) that overcomes these limitations by transferring the information on the OAM into a distinct frequency domain. In our scheme, two OVBs─one carrying OAM-encoded information and the other serving as a reference─are coupled within a beta-barium borate (BBO) crystal to generate an SFG signal. Our theoretical and experimental studies demonstrate that SFG efficiency is governed by the spatial overlap of the interacting vortex profiles, providing mode-selective and OAM-resolved detection. Crucially, as only a small fraction of the input photons undergo conversion into the nonlinear signal, the original beams remain functionally intact. Since detection is performed exclusively on the upconverted signal in a spectrally distinct visible wavelength region, the signal-to-noise ratio can be improved. Moreover, the SFG signal is generated only when specific OAM states and temporal overlap conditions are simultaneously satisfied, enabling ultrafast and conditionally gated access to the OAM information. This nonlinear selectivity offers enhanced physical-layer security and high-throughput capabilities. Together, our approach provides a robust and versatile platform for advanced OAM-based optical communications and high-capacity photonics applications.