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Physical Review A

Managing orbital angular momentum in second-harmonic generation

Simin Li, Ling‐Jun Kong, Zhi‐Cheng Ren, Yongnan Li, Chenghou Tu, Hui‐Tian Wang

Published Sep 3, 2013• 48 citations
Publisher

Abstract

We propose a convenient approach for managing orbital angular momentum (OAM) of second-harmonic photons generated by a quadratic nonlinear interaction under noncolinear type-I phase matching condition. Since the OAMs of two fundamental photons can be flexibly controlled by using computer-generated holograms, we were able to realize arbitrary combination of both OAMs and experimentally confirm the OAM conservation selection rule ${\ensuremath{\ell}}_{2\ensuremath{\omega}}={\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}}+{\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}\ensuremath{'}}$ in general cases. In particular, our approach could be used to generate the second-harmonic photon states with fractional and odd-order OAMs.

DOI
10.1103/physreva.88.035801

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We propose a convenient approach for managing orbital angular momentum (OAM) of second-harmonic photons generated by a quadratic nonlinear interaction under noncolinear type-I phase matching condition. Since the OAMs of two fundamental photons can be flexibly controlled by using computer-generated holograms, we were able to realize arbitrary combination of both OAMs and experimentally confirm the OAM conservation selection rule \ensuremathℓ2\ensuremathω=\ensuremathℓ\ensuremathω\ensuremath′+\ensuremathℓ\ensuremathω\ensuremath′\ensuremath′{\ensuremath{\ell}}_{2\ensuremath{\omega}}={\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}}+{\ensuremath{\ell}}_{\ensuremath{\omega}}^{\ensuremath{'}\ensuremath{'}}\ensuremathℓ2\ensuremathω​=\ensuremathℓ\ensuremathω\ensuremath′​+\ensuremathℓ\ensuremathω\ensuremath′\ensuremath′​ in general cases. In particular, our approach could be used to generate the second-harmonic photon states with fractional and odd-order OAMs.
Nonlinear interaction between orbital angular momentum (OAM) modes has interesting effects and tremendous applications in both classical and quantum realms. Here we propose a strategy of using perfect vortices, which not only overcomes the spatial mode matching problem of nondegenerate OAM modes, but also reveals the OAM-only influence on the momentum matching by tuning the OAMs of the fundamental wave. We use perfect vortices of degenerate and nondegenerate OAM modes to clearly demonstrate the flexible control of OAM modes on nonlinear interaction by carefully exploring second-harmonic generation (SHG) in periodically poled crystal. We generate second-harmonic perfect vortices with the OAM order up to 40. Based on the observed phase-matching temperature shift caused by OAMs, we also use the SHG nonlinear process to distinctly confirm the OAM-only-induced subluminal effect. Our results pave the way toward unveiling the underlying physics behind nonlinear process of OAM modes and building high-capacity quantum links between systems operating at various wavelengths. The inverse process of SHG we developed, perfect-vortex-based spontaneous parametric down-conversion, may provide a promising solution for high-dimensional OAM entangled source.
Orbital angular momentum (OAM)-entangled states produced by spontaneous parametric down-conversion (SPDC) are considered ideal for realizing high-dimensional entangled states, which have several advantages for quantum technologies. However, the limited sensitivity of current two-photon OAM detectors is a major roadblock not only for realizing such technologies but also for resolving foundational questions, such as OAM conservation in SPDC. The current theoretical understanding is that OAM is not conserved in Type-II SPDC but is conserved in Type-I. Experimentally, although non-conservation in TypeII has not been demonstrated, conservation in Type-I has been reported frequently and has become an underlying assumption for techniques generating high-dimensional OAM entangled states. In this work, we experimentally demonstrate a high-sensitivity two-photon OAM detector, using which, contrary to the current understanding, we report non-conservation of OAM in Type-I SPDC. We attribute this to a spatial walk-off effect and prove it using a framework free of standard phase-matching approximations.
We experimentally demonstrate multiple copies of optical orbital angular momentum (OAM) states through quasi-phase-matched (QPM) second-harmonic (SH) generation in a 2D periodically poled LiTaO3 (PPLT) crystal. Since the QPM condition is satisfied by involving different reciprocal vectors in the 2D PPLT crystal, collinear and noncollinear SH beams carrying OAMs of l2 are simultaneously generated by the input fundamental beam with an OAM of l1. The OAM conservation law (i.e., l2 = 2l1) holds well in the experiment, which can tolerate certain phase-mismatch between the interacting waves. Our results provide an efficient way to obtain multiple copies of the wavelength-converted OAM states, which can be used to enhance the capacity in optical communications.
The bandwidth of any communication system, classical or quantum, is limited by the number of orthogonal states in which the information can be encoded. Quantum key distribution systems available commercially rely on the two-dimensional polarisation state of photons. Quantum computation has also been largely designed on the basis of qubits. However, a photon is endowed with other degrees of freedom, such as orbital angular momentum (OAM). OAM is an attractive basis to be used for quantum information because it is discrete and theoretically infinite-dimensional. This promises a higher information capacity per photon which can lead to more complex quantum computation protocols and more security and robustness for quantum cryptography. Entanglement of OAM naturally arises from spontaneous parametric down-conversion (SPDC). However, any practical experiment utilising the innately high-dimensional entanglement of the orbital angular momentum (OAM) state space of photons is subject to the modal capacity of the detection system. Only a finite subset of this space is accessible experimentally. Given such a constraint, we show that the number of measured, entangled OAM modes in photon pairs generated by SPDC can be increased by tuning the phase-matching conditions in the SPDC process. We achieve this by tuning the orientation angle of the nonlinear crystal generating the entangled photons.
Optical spin–orbit interaction (SOI), which can be used to simultaneously control the spin and orbital angular momentum of light, is important for both classical and quantum information applications. In linear and nonlinear optics, the SOI of light has been extensively explored in both artificial structures and conventional optical crystals. However, optical SOI in quantum nonlinear optical processes, such as spontaneous parametric downconversion (SPDC), has not been studied before. Here, we experimentally demonstrate that optical SOI in the SPDC process can be realized through a nonlinear crystal with threefold rotational symmetry. Two-photon quantum states with controlled angular momentum can be generated through the symmetry selection rules in nonlinear optics and the SOI of the pump wave. The proposed methodology may facilitate the generation and control of spin and orbital angular momentum of entangled photons.
Using orbital angular momentum (OAM) conservation in second-order nonlinear interaction processes, we create a classical to quantum optical network link in the OAM degrees of freedom of light via sum frequency generation, followed by spontaneous parametric down-conversion. Coherent OAM-carrying beams at 1550 nm are up-converted to 525.5-nm OAM-carrying beams in the first crystal, and are used to pump a second crystal to generate non-degenerate OAM entangled photon pairs at 795 nm and 1550 nm. By switching the OAM carried by the classical part, OAM correlation in the quantum part is shifted. High-level OAM entanglements in two-dimensional subspaces are verified.