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ACS Photonics

Optical Orbital Angular Momentum Detection Using Second-Order Nonlinear Optical Processes

Ju-Young Kim, Minhaeng Cho

Published Feb 5, 2026• 1 citation
Publisher

Abstract

Optical vortex beams (OVBs) carrying orbital angular momentum (OAM) offer access to an unbounded set of orthogonal states, enabling a dramatic increase in the information capacity for optical communication systems. However, practical OAM detection in telecommunication platforms remains challenging due to background noise, detector limitations at infrared communication wavelengths, and the destructive nature of conventional sampling methods. Here, we introduce an all-optical, nearly nondestructive OAM detection method based on sum-frequency generation (SFG) that overcomes these limitations by transferring the information on the OAM into a distinct frequency domain. In our scheme, two OVBs─one carrying OAM-encoded information and the other serving as a reference─are coupled within a beta-barium borate (BBO) crystal to generate an SFG signal. Our theoretical and experimental studies demonstrate that SFG efficiency is governed by the spatial overlap of the interacting vortex profiles, providing mode-selective and OAM-resolved detection. Crucially, as only a small fraction of the input photons undergo conversion into the nonlinear signal, the original beams remain functionally intact. Since detection is performed exclusively on the upconverted signal in a spectrally distinct visible wavelength region, the signal-to-noise ratio can be improved. Moreover, the SFG signal is generated only when specific OAM states and temporal overlap conditions are simultaneously satisfied, enabling ultrafast and conditionally gated access to the OAM information. This nonlinear selectivity offers enhanced physical-layer security and high-throughput capabilities. Together, our approach provides a robust and versatile platform for advanced OAM-based optical communications and high-capacity photonics applications.

DOI
10.1021/acsphotonics.5c02389

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Newton•Apr 24, 2026•1 citation
Optical vortex beams (OVBs) carrying orbital angular momentum (OAM) offer access to an unbounded set of orthogonal states, enabling a dramatic increase in the information capacity for optical communication systems. However, practical OAM detection in telecommunication platforms remains challenging due to background noise, detector limitations at infrared communication wavelengths, and the destructive nature of conventional sampling methods. Here, we introduce an all-optical, nearly nondestructive OAM detection method based on sum-frequency generation (SFG) that overcomes these limitations by transferring the information on the OAM into a distinct frequency domain. In our scheme, two OVBs─one carrying OAM-encoded information and the other serving as a reference─are coupled within a beta-barium borate (BBO) crystal to generate an SFG signal. Our theoretical and experimental studies demonstrate that SFG efficiency is governed by the spatial overlap of the interacting vortex profiles, providing mode-selective and OAM-resolved detection. Crucially, as only a small fraction of the input photons undergo conversion into the nonlinear signal, the original beams remain functionally intact. Since detection is performed exclusively on the upconverted signal in a spectrally distinct visible wavelength region, the signal-to-noise ratio can be improved. Moreover, the SFG signal is generated only when specific OAM states and temporal overlap conditions are simultaneously satisfied, enabling ultrafast and conditionally gated access to the OAM information. This nonlinear selectivity offers enhanced physical-layer security and high-throughput capabilities. Together, our approach provides a robust and versatile platform for advanced OAM-based optical communications and high-capacity photonics applications.
Methods to generate, manipulate, and measure optical and atomic fields with global or local angular momentum have a wide range of applications in both fundamental physics research and technology development. In optics, the engineering of angular momentum states of light can aid studies of orbital angular momentum (OAM) exchange between light and matter. The engineering of optical angular momentum states can also be used to increase the bandwidth of optical communications or serve as a means to distribute quantum keys, for example. Similar capabilities in Bose-Einstein condensates are being investigated to improve our understanding of superfluid dynamics, superconductivity, and turbulence, the last of which is widely considered to be one of most ubiquitous yet poorly understood subjects in physics. The first part of this two-part dissertation presents an analysis of techniques for measuring and manipulating quantized vortices in BECs. The second part of this dissertation presents theoretical and numerical analyses of new methods to engineer the OAM spectra of optical beams. The superfluid dynamics of a BEC are often well described by a nonlinear Schrodinger equation. The nonlinearity arises from interatomic scattering and enables BECs to support quantized vortices, which have quantized circulation and are fundamental structural elements of quantum turbulence. With the experimental tools to dynamically manipulate and measure quantized vortices, BECs are proving to be a useful medium for testing the theoretical predictions of quantum turbulence. In this dissertation we analyze a method for making minimally destructive in situ observations of quantized vortices in a BEC. Secondly, we numerically study a mechanism to imprint vortex dipoles in a BEC. With these advancements, more robust experiments of vortex dynamics and quantum turbulence will be within reach. A more complete understanding of quantum turbulence will enable principles of microscopic fluid flow to be related to the statistical properties of turbulence in a superfluid. In the second part of this dissertation we explore frequency mixing, a subset of nonlinear optical processes in which one or more input optical beam(s) are converted into one or more output beams with different optical frequencies. The ability of parametric nonlinear processes such as second harmonic generation or parametric amplification to manipulate the OAM spectra of optical beams is an active area of research. In a theoretical and numerical investigation, two complimentary methods for sculpting the OAM spectra are developed. The first method employs second harmonic generation with two non-collinear input beams to develop a broad spectrum of OAM states in an optical field. The second method utilizes parametric amplification with collinear input beams to develop an OAM-dependent gain or attenuation, termed dichroism for OAM, to effectively narrow the OAM spectrum of an optical beam. The theoretical principles developed in this dissertation enhance our understanding of how nonlinear processes can be used to engineer the OAM spectra of optical beams and could serve as methods to increase the bandwidth of an optical signal by multiplexing over a range of OAM states.
The bandwidth of any communication system, classical or quantum, is limited by the number of orthogonal states in which the information can be encoded. Quantum key distribution systems available commercially rely on the two-dimensional polarisation state of photons. Quantum computation has also been largely designed on the basis of qubits. However, a photon is endowed with other degrees of freedom, such as orbital angular momentum (OAM). OAM is an attractive basis to be used for quantum information because it is discrete and theoretically infinite-dimensional. This promises a higher information capacity per photon which can lead to more complex quantum computation protocols and more security and robustness for quantum cryptography. Entanglement of OAM naturally arises from spontaneous parametric down-conversion (SPDC). However, any practical experiment utilising the innately high-dimensional entanglement of the orbital angular momentum (OAM) state space of photons is subject to the modal capacity of the detection system. Only a finite subset of this space is accessible experimentally. Given such a constraint, we show that the number of measured, entangled OAM modes in photon pairs generated by SPDC can be increased by tuning the phase-matching conditions in the SPDC process. We achieve this by tuning the orientation angle of the nonlinear crystal generating the entangled photons.
Light carrying orbital angular momentum (OAM) has many applications ranging from optical manipulation, imaging and remote sensing, and optical communications, and can be used to perform fundamental studies in quantum mechanics and quantum information. Moreover, single photons with high-order OAM allow for increasing the amount of information carried per photon in quantum communication. This thesis describes the study of methods for the preparation and detection of OAM of light in high mode order by utilizing beam shaping techniques using spatial light modulators (SLMs). The quality of the generated high-order OAM mode is limited by optical aberrations which are induced by optical elements in realistic systems and propagation through realistic channels. In order to create and characterize the OAM modes with high quality, we investigate methods for aberration detection and correction using SLMs. These beam shaping techniques for the correction of optical aberrations allow us to generate and detect light carrying OAM with mode order ranging from l = 0 to l = 8 with good quality, and to generate high-quality superpositions of OAM modes with high mode order or in high dimensions. Furthermore, we observe low crosstalk and good levels of mode discrimination between different OAM modes of light. Our experimental setup can be applied in future studies to investigate and test different protocols in quantum information with high dimensional systems, such as high dimensional quantum state tomography.
This study presents an innovative scheme for detecting the orbital angular momentum (OAM) of vortex beams within an atomic ensemble. Leveraging a homogeneously broadened four-level atomic system driven by two orthogonal polarization probe beams, we demonstrate the selective generation of structured beams without the need for magnetic fields between the two ground states. Through detailed theoretical analysis and numerical simulations, we elucidate the phase-dependent behavior of atomic coherences induced by an OAM-carrying Laguerre–Gaussian optical probe beam. These findings enable the creation of petal-like structures within the probe beam, with the number of petals directly correlated to the OAM value. Our investigation underscores the potential of this OAM detection scheme as a highly sensitive and precise sensor, applicable across diverse domains such as telecommunication, microscopy, and optical metrology.
We explore the generation of orbital angular momentum (OAM) carrying mid-infrared Bessel-Gaussian beams through nonlinear interactions within a non-uniformly broadened 85 Rb atomic ensemble. Utilizing an efficient four-wave mixing (FWM) scheme driven by two strong control fields and a weak probe field, we achieve coherent emission at a wavelength of 5.23 µm. By employing the density matrix approach, we obtain an analytical expression for the nonlinear atomic coherence involved in the four-wave mixing process, elucidating how the Bessel-Gaussian profile of the probe field is transferred into the mid-infrared signal. Numerical simulations of Maxwell’s wave equation ensure the generation of phase-matched, non-diffracting Bessel-Gaussian beams, which can be precisely controlled by manipulating the spatial susceptibility of the atomic medium. Furthermore, this study demonstrates the potential of higher-order Bessel-Gaussian beams with OAM to significantly advance applications in high-speed communication, biomedical imaging, and optical manipulation, owing to their robust beam integrity and enhanced data transmission capabilities in the mid-infrared spectrum.
Orbital angular momentum (OAM) of photons provides a promising approach to enhance the capacity, robustness, and functionality of quantum communication systems in optical fibers. With many twist states available, OAM enables high-dimensional encoding, significantly increasing data rates and noise tolerance. This review explores sources, channels, and system architectures for OAM-based quantum communication in fibers. It compares free-space and integrated emitters, discussing in-fiber pair generation and mode conversion pathways that produce fiber-ready single photons and entangled states. For the channels, it details design principles and trade-offs for step-index and ring-core fibers that minimize intermodal coupling and reviews milestones in kilometer-scale single-photon transmission and high-dimensional entanglement transport. On the system side, the review examines coupling, multiplexing, and detection techniques—including mode (de)multiplexers, lanterns, and programmable sorters—and discusses transmission-matrix-based control methods to mitigate dispersion and bending effects. The review concludes with practical guidance and open challenges, such as improving mode selectivity and stability under real-world conditions; developing compact, efficient detectors for many modes; and integrating co-designed error correction schemes. These directions aim to bridge laboratory demonstrations with the deployment of scalable, high-dimensional fiber networks that harness OAM to significantly boost capacity, resilience, and functionality.