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Laser Physics Letters

Incoherent backward photon echo in ruby upon excitation through an optical fiber

В. В. Самарцев, Шегеда Анатолий Михайлович, A. V. Shkalikov, Каримуллин Камиль Равкатович, Tatiana G. Mitrofanova, В. А. Зуйков

Published Apr 4, 2007• 19 citations
Publisher

Abstract

The results of an experimental investigation of the incoherent photon echo in ruby (with Cr3+ concentration equal to 0.16 wt%) at T=1.7 K are presented. Optical fiber with length 3 m and diameter 100 μm was used for delivery of the first exciting pulse to a sample. The dependence of the IPE intensity on the excitation wavelength within the width of R1 absorption line was studied. The IPE decay curve was obtained and the phase relaxation time was found to be equal to 98 ns.

DOI
10.1002/lapl.200710026

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This paper is about the possibilities of optically dense impurity media spectroscopy by means of the incoherent photon echo. The theoretical model of the phenomenon is given. The results of experiment on incoherent photon echo in a crystal of ruby at liquid helium temperature are presented. Fiber optical delay line was used to make an incoherence of the excitation radiation. The dependence of the incoherent echo intensity on the excitation wavelength was studied. The echo decay curve was obtained and the phase relaxation time was found to be equal to 98 ns.

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The possibility of using incoherent photon echo in spectroscopy of optically dense impurity media is considered. A theoretical approach to description of this phenomenon is presented. The experimental data on incoherent photon echo in ruby at liquid-helium temperature, with transport of an excitation pulse through a fiber, are reported. The spectral dependence of the echo intensity is studied. The decay curve for an incoherent echo signal is investigated, and the phase relaxation time is found to be 98 ns.

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The signals of photon echo (PE) are investigated firstly in a ruby crystal doped only by the 53 Cr isotope ions in a concentration of 0.03 – 0,05 wt%. The optical experiments were performed in backward regime at the wavelength of 693.4 nm both with a low magnetic field (200 G) and without it. Since the 53 Cr isotope ions have hyperfine structure of levels the special attention was paid to the study of the stimulated photon echo and primarily to the investigation of its decay kinetics. It is established that this decay has a form which is typical to the signals of long-lived PE. But in contrast to the long-lived PE the decay time in our case is less than the lifetime of the excited 2E(Ē) state. The signals of primary photon echo and stimulated photon echo at a low longitudinal magnetic field and their decay curves are investigated. We observed the beats of temporal shape of these signals with a period of several tens of nanoseconds. Theoretical analysis shows that they are due to the hyperfine interaction of valence electrons of 53 Cr isotope ions with their own nuclei. The obtained decay curves allow us to estimate the phase relaxation time at the presence of a magnetic field. It proves to be equal to 98 ns. The spectrum of stimulated photon echo signal in the doped ruby exposed to a magnetic field is measured.

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Accumulated Photon-Echo Measurements In Ruby under Hydrostatic Pressure

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Photon-echo techniques are widely applied nowadays to study optically active ions in solids. The first photon echoes were observed for the R1 transition in ruby (Al2O3: Cr3+) by Kurnit et al1 using the high-power pulses of a ruby laser. Very recently,2 phase relaxation of both the R1 and R2 transitions in ruby was studied at 1.5 K and ambient pressure. Here, use was ma.de of the technique of accun1ulated photon echo,3 which despite the low average laser power offers greatly enhanced detection sensitivity by virtue of the high repetition rate.

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Reverse Photon Echo as a Method of Investigation of Resonant Medium Parameters

В. А. Зуйков, В. В. Самарцев

The possibilities of the reverse photon echo for obtaining information about the relaxation times and the electrical dipole momentum of the resonant transition are investigated experimentally in ruby (resonant transition 4A2–2E(Ē)). A new method based on the many-pulse excitation of the resonant system by a single travelling wave and by a sequence of standing waves, is proposed. As a result, this system irradiates a series of reverse echo signals, from the decay of their intensities it is possible to define the relaxation times in a single series. These relaxation times are measured at different values of the permanent magnetic field. The different apparatus solutions of these experimental problems are discussed.

physica status solidi (a)•Oct 16, 1982•15 citations
The results of an experimental investigation of the incoherent photon echo in ruby (with Cr3+ concentration equal to 0.16 wt%) at T=1.7 K are presented. Optical fiber with length 3 m and diameter 100 μm was used for delivery of the first exciting pulse to a sample. The dependence of the IPE intensity on the excitation wavelength within the width of R1 absorption line was studied. The IPE decay curve was obtained and the phase relaxation time was found to be equal to 98 ns.
This paper is about the possibilities of optically dense impurity media spectroscopy by means of the incoherent photon echo. The theoretical model of the phenomenon is given. The results of experiment on incoherent photon echo in a crystal of ruby at liquid helium temperature are presented. Fiber optical delay line was used to make an incoherence of the excitation radiation. The dependence of the incoherent echo intensity on the excitation wavelength was studied. The echo decay curve was obtained and the phase relaxation time was found to be equal to 98 ns.
The possibility of using incoherent photon echo in spectroscopy of optically dense impurity media is considered. A theoretical approach to description of this phenomenon is presented. The experimental data on incoherent photon echo in ruby at liquid-helium temperature, with transport of an excitation pulse through a fiber, are reported. The spectral dependence of the echo intensity is studied. The decay curve for an incoherent echo signal is investigated, and the phase relaxation time is found to be 98 ns.
A detailed experimental study is reported of the decay of circularly polarized photon echoes as a function of Cr concentration in samples ranging from 0.006 to 1.2 wt.% Cr2{\mathrm{Cr}}_{2}Cr2​O3{\mathrm{O}}_{3}O3​ in Al2{\mathrm{Al}}_{2}Al2​O3{\mathrm{O}}_{3}O3​. The decay is found to be independent of temperature in the liquid-helium range and generally depends on the pulse separation $\ensuremath{\tau}$ as $\mathrm{exp}(\ensuremath{-}K{\ensuremath{\tau}}^{\frac{1}{2}})$ with the decay constant KKK proportional to the square root of the Cr concentration. The measured decay is independent of external magnetic field in the range 1.5-6 kG except at 1.06 kG, where modified decays are observed. A theoretical analysis is made of photon-echo decay in terms of spin flips of echo ions resulting from Cr-Cr magnetic interactions and yields good agreement with the observed decays. Spectral diffusion, modified for photon echoes, is shown not to be an important effect. However, anomalously slow decay is observed in some samples when the laser is tuned to the long-wavelength tail of the sample absorption line and the spectral-diffusion mechanism may apply here. The photon-echo-decay measurements are compared with spin-resonance and available spin-echo data in ruby. Also, it is inferred that resonant optical energy transfer is not an important photon-echo-decay mechanism even in the darkest sample studied.
The signals of photon echo (PE) are investigated firstly in a ruby crystal doped only by the 53 Cr isotope ions in a concentration of 0.03 – 0,05 wt%. The optical experiments were performed in backward regime at the wavelength of 693.4 nm both with a low magnetic field (200 G) and without it. Since the 53 Cr isotope ions have hyperfine structure of levels the special attention was paid to the study of the stimulated photon echo and primarily to the investigation of its decay kinetics. It is established that this decay has a form which is typical to the signals of long-lived PE. But in contrast to the long-lived PE the decay time in our case is less than the lifetime of the excited 2E(Ē) state. The signals of primary photon echo and stimulated photon echo at a low longitudinal magnetic field and their decay curves are investigated. We observed the beats of temporal shape of these signals with a period of several tens of nanoseconds. Theoretical analysis shows that they are due to the hyperfine interaction of valence electrons of 53 Cr isotope ions with their own nuclei. The obtained decay curves allow us to estimate the phase relaxation time at the presence of a magnetic field. It proves to be equal to 98 ns. The spectrum of stimulated photon echo signal in the doped ruby exposed to a magnetic field is measured.
Photon-echo techniques are widely applied nowadays to study optically active ions in solids. The first photon echoes were observed for the R1 transition in ruby (Al2O3: Cr3+) by Kurnit et al1 using the high-power pulses of a ruby laser. Very recently,2 phase relaxation of both the R1 and R2 transitions in ruby was studied at 1.5 K and ambient pressure. Here, use was ma.de of the technique of accun1ulated photon echo,3 which despite the low average laser power offers greatly enhanced detection sensitivity by virtue of the high repetition rate.
The possibilities of the reverse photon echo for obtaining information about the relaxation times and the electrical dipole momentum of the resonant transition are investigated experimentally in ruby (resonant transition 4A2–2E(Ē)). A new method based on the many-pulse excitation of the resonant system by a single travelling wave and by a sequence of standing waves, is proposed. As a result, this system irradiates a series of reverse echo signals, from the decay of their intensities it is possible to define the relaxation times in a single series. These relaxation times are measured at different values of the permanent magnetic field. The different apparatus solutions of these experimental problems are discussed.