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Journal of the Optical Society of America B

Optical bistability in a three-level lambda molecule with permanent dipole moments

Seyyed Hossein Asadpour, HAMID RAHIMPOUR SOLEIMANI

Published Nov 17, 2014• 11 citations
Publisher

Abstract

Optical bistability (OB) in a unidirectional ring cavity with a three-level Λ-type molecular system with nonzero permanent dipole moments is discussed. We found that in the (2+2)-transition processes, the permanent dipole moments induced new quantum coherence effects which lead to controlling the OB behavior of the system. Moreover, we showed that the group velocity can be switched from slow to fast or vice versa under specific conditions of difference in permanent dipole moments of the probe transition.

DOI
10.1364/josab.31.003123

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The optical bistability (OB) and multistability (OM) in chiral molecules are investigated by placing the sample into a unidirectional ring cavity. Because of broken mirror symmetry of the effective potential, the chiral molecules have a cyclic three-level Δ-configuration structure, in which one- and two-photon transitions can coexist. We find that the OB is achievable in this system on exact one-, two- and three-photon resonance conditions but absent in the three-level Λ-type system under the two-photon resonance. Moreover, the OM and the switching between OB and OM are also realized by choosing parameters properly. Interestingly, the left- and right-handed chiral molecules exhibit different bistable and multistable behaviors. It is shown that the threshold intensity of OB is strongly dependent on the percentage of the two enantiomers in the mixture. This provides an effective approach to probe molecular chirality and to determine enantiomer excess, which may find potential application in organic chemistry, pharmacology, biochemistry, etc..

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Abstract We have investigated the optical bistability and multistability behaviors in a three-level V-type system via both coherent and incoherent fields inside a unidirectional ring cavity. We find that the appearance and disappearance of optical bistability (OB)/optical multistability (OM) can easily be controlled by adjusting systemic parameters. Our scheme opens up a new possibility for realizing transition from OB to OM or vice versa for potential applications in information networks and processing with increased capacity.

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Electromagnetically induced transparency in a Λ-type molecular system with permanent dipole moments revisited

Niharika Singh, Q. V. Lawande, Richard D’Souza +1 more

Electromagnetically induced transparency (EIT) in a molecular three-level Λ system with permanent dipole moments and undergoing m- and n-photon transitions by pump and probe lasers is investigated. Analytical expressions are derived for probe absorption spectrum and dispersion for a medium of stationary as well as thermal molecules. Contrary to the earlier study by Zhou et al. [J. Chem. Phys. 131, 034105 (2009)], we observe no amplification in 2 + 2 photon process when the sign of the difference of the permanent moments of the excited and the ground levels is reversed. Reasons for these contrasting observations are discussed. Our study shows that the permanent moments essentially damp the laser-molecule Rabi frequency to result in narrower EIT line width and larger group velocity index. These effects are further enhanced when the order of the multi-photon process is increased. The importance of the virtual mechanism is discussed by considering the special case of 2 + 1 photon EIT.

The Journal of Chemical Physics•Sep 12, 2012•6 citations
Optical bistability (OB) in a unidirectional ring cavity with a three-level Λ-type molecular system with nonzero permanent dipole moments is discussed. We found that in the (2+2)-transition processes, the permanent dipole moments induced new quantum coherence effects which lead to controlling the OB behavior of the system. Moreover, we showed that the group velocity can be switched from slow to fast or vice versa under specific conditions of difference in permanent dipole moments of the probe transition.
The effect of permanent dipole moments on the optical bistability of weak probe light in a unidirectional ring cavity with a three-level molecule is investigated. It is found that the intensity threshold of optical bistability and optical multistability can be controlled by quantum coherence induced by permanent dipole moments. It is shown that switching from optical bistability to optical multistability and lasing without population inversion can be occurred by this coherence under different conditions.
The optical bistability (OB) and multistability (OM) in chiral molecules are investigated by placing the sample into a unidirectional ring cavity. Because of broken mirror symmetry of the effective potential, the chiral molecules have a cyclic three-level Δ-configuration structure, in which one- and two-photon transitions can coexist. We find that the OB is achievable in this system on exact one-, two- and three-photon resonance conditions but absent in the three-level Λ-type system under the two-photon resonance. Moreover, the OM and the switching between OB and OM are also realized by choosing parameters properly. Interestingly, the left- and right-handed chiral molecules exhibit different bistable and multistable behaviors. It is shown that the threshold intensity of OB is strongly dependent on the percentage of the two enantiomers in the mixture. This provides an effective approach to probe molecular chirality and to determine enantiomer excess, which may find potential application in organic chemistry, pharmacology, biochemistry, etc..
Electromagnetically induced transparency in a three-level Lambda-type molecular system with nonzero permanent dipole moments is investigated. It is shown that in the (2+2)-transition processes, when the sign of d(21), the difference in permanent dipole moments of the probe transition, is positive, perfect electromagnetically induced transparency with steep normal dispersion could be obtained under specific conditions. In contrast, when the sign of d(21) is negative, surprisingly gain without inversion with steep anomalous dispersion could be attained.
The steady-state optical bistability(OB) and optical multistability(OM) behavior in the quasi——type atomic system driven by a probe field and a coherent coupling field inside a unidirectional ring cavity are shown,and the effects of coupling-field detuning and coupling-field intensity on the OB and OM behavior are investigated. The transition from OB to OM or vice versa is found by varying the detuning of the coherent coupling field or by adjusting the intensity of the coupling field. The influence of the atomic cooperation parameter on the OM behavior is also discussed.
Abstract We have investigated the optical bistability and multistability behaviors in a three-level V-type system via both coherent and incoherent fields inside a unidirectional ring cavity. We find that the appearance and disappearance of optical bistability (OB)/optical multistability (OM) can easily be controlled by adjusting systemic parameters. Our scheme opens up a new possibility for realizing transition from OB to OM or vice versa for potential applications in information networks and processing with increased capacity.
Electromagnetically induced transparency (EIT) in a molecular three-level Λ system with permanent dipole moments and undergoing m- and n-photon transitions by pump and probe lasers is investigated. Analytical expressions are derived for probe absorption spectrum and dispersion for a medium of stationary as well as thermal molecules. Contrary to the earlier study by Zhou et al. [J. Chem. Phys. 131, 034105 (2009)], we observe no amplification in 2 + 2 photon process when the sign of the difference of the permanent moments of the excited and the ground levels is reversed. Reasons for these contrasting observations are discussed. Our study shows that the permanent moments essentially damp the laser-molecule Rabi frequency to result in narrower EIT line width and larger group velocity index. These effects are further enhanced when the order of the multi-photon process is increased. The importance of the virtual mechanism is discussed by considering the special case of 2 + 1 photon EIT.