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Japanese Journal of Applied Physics

Frequency Detuning and Stabilization of a Diode Laser Using the Zeeman Shift of the Saturated Absorption Signal of Rubidium Atoms

Ho Seong Lee, Sung Hoon Yang, Young Bum Kim, Sang Eon Park, Hyuck Cho, Jong Dae Park

Published Jan 1, 1996• 13 citations
Publisher

Abstract

We observed saturated absorption spectra of the 87Rb atom under a magnetic field of several millitesla with a diode laser oscillating at 780 nm. The spectra were compared with the theoretical ones obtained on the basis of Nakayama's four-level model. We numerically computed Zeeman splittings of the 52 P 3/2 excited state of the atom. As the magnetic field increased to 5 mT, the absorption peak of the F=2→F'=3 transition shifted almost linearly up to about 62 MHz. The shift direction was reversed by changing the polarization combination of the pump and probe lasers. The measured frequency stability, when the laser was locked at the absorption peak, was better than σy(τ)= 1 ×10-11τ-1/2 for the sampling time of 0.01 s≤τ≤10 s.

DOI
10.1143/jjap.35.276

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We observed saturated absorption spectra of the 87Rb atom under a magnetic field of several millitesla with a diode laser oscillating at 780 nm. The spectra were compared with the theoretical ones obtained on the basis of Nakayama's four-level model. We numerically computed Zeeman splittings of the 52 P 3/2 excited state of the atom. As the magnetic field increased to 5 mT, the absorption peak of the F=2→F'=3 transition shifted almost linearly up to about 62 MHz. The shift direction was reversed by changing the polarization combination of the pump and probe lasers. The measured frequency stability, when the laser was locked at the absorption peak, was better than σy(τ)= 1 ×10-11τ-1/2 for the sampling time of 0.01 s≤τ≤10 s.
Zeeman split takes place for the hyperfine level structure of neutral atoms where magnetic field exists. In addition, being excited by right circularly polarized light and left circularly polarized light, atoms obey different transition rules. So, the absorption peak between the hyperfine Zeeman level shifts with respect to the absorption peak without magnetic field. Accordingly, the authors demonstrated a kind of simple and flexible method to stabilize the frequency of diode laser. The linewidth of diode laser was reduced to less than 1 MHz using this method. Through analyzing the experiment results, the authors found that when the sum of both shifts of the hyperfine level of atoms excited by right circularly polarized light and left circularly polarized light was equal to the FWHM (Full Width at Half Maximum) of the saturated absorption peak, the laser frequency was stabilized best.
Recently a new type of spectroscopy using Zeeman shift has been developed, which aims for a large recapture range by making a dispersive-like signal obtained from the subtraction of two different circularly polarized Doppler-broadened absorption signals in the presence of a magnetic field (order of 100 G). We would like to propose another method for stabilizing a diode laser frequency onto an atomic frequency with a small tunable range in the presence of small longitudinal magnetic field (order of Gauss). A solid state diode laser is preferred as it is a good light source. Our technique has the advantages of cancellation of frequency fluctuation over side-locking and no need for phase-sensitive detection and frequency modulation over peak-locking. A subtracted SAS signal and the blocking signal are displayed on one photodiode.
We report on the observation of a Zeeman shift (order of 100 MHz) of the Doppler-broadened D2 transition of both 85Rb and 87Rb isotopes via transmission through a 400 nm diameter optical nanofiber in the presence of a DC magnetic field. Linearly-polarized light propagating in the nanofiber is analyzed as a superposition of two orthogonally circularly polarized orientations, σ+ and σ-. In the absence of the magnetic field, the absorption of these polarizations by the atomic vapor, via the evanescent field at the waist of the nanofiber, is degenerate. When a weak magnetic field is applied parallel to the propagating light, this degeneracy is lifted and relative shifts in the resonance frequencies are detected. Typical linear shift rates of 1.6 MHz/G and -2.0 MHz/G were observed. We also demonstrate a dichroic atomic vapor laser lock line shape by monitoring the real-time subtraction of the two magnetically-shifted absorption spectra. This is particularly interesting for magneto-optical experiments as it could be directly implemented for diode laser frequencystabilization.
High-resolution saturated absorption spectroscopy of the 85RbD1 line has been used for observation of the Zeeman effect by use of a diode laser with a narrow linewidth. Experimental results were compared with both Breit–Rabi theory related to shifted resonant frequencies and Nakayama's single-cycle optical pumping theory related to signal magnitudes of signal [J. Opt. Soc. Am. B2, 1431 (1985)]. A comparison of our results with those of Bowie [J. Opt. Soc. Am. B12, 1839 (1995)], who used perturbation theory to obtain the energy-level shifts, yielded experimental results that differ significantly in some respects.
We demonstrate a robust method of stabilizing a diode laser frequency to an atomic transition. This technique employs the Zeeman shift to generate an antisymmetric signal about a Doppler-broadened atomic resonance, and therefore offers a large recapture range as well as high stability. The frequency of a 780-nm diode laser, stabilized to such a signal in Rb, drifted less than 0.5 MHz peak-peak (1 part in 10(9)) in 38 h. This tunable frequency lock can be constructed inexpensively, requires little laser power, rarely loses lock, and can be extended to other wavelengths by use of different atomic species.