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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Nonlinear properties of quasi-optic open resonator with a layer of Crvsolution in heavy alcohol under the conditions of magnetic resonance

Alexey A. Vertiy, Sergiy P. Gavrilov

Published Feb 1, 1991• 0 citations
Publisher

Abstract

A quasi-optic resonator with a paramagnetic plane-parallel layer is considered. Stationary and non-stationary excitations of fields in such open resonator by a plane linearly polarized electromagnetic wave are studied. The dependences of the OR transmission coefficient as a nonlinear function on the magnetic component of the exciting electromagnetic field and time have been calculated assuming that magnetic susceptibility in paramagnetic is connected with the amplitude of a radio-frequency magnetic field as a nonlinear function determined from the Bloch''s equations. Bistability hysteretic phenomena and unstable operating regimes of the structure in question have been found.

DOI
10.1117/12.24453

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A quasi-optic resonator with a paramagnetic plane-parallel layer is considered. Stationary and non-stationary excitations of fields in such open resonator by a plane linearly polarized electromagnetic wave are studied. The dependences of the OR transmission coefficient as a nonlinear function on the magnetic component of the exciting electromagnetic field and time have been calculated assuming that magnetic susceptibility in paramagnetic is connected with the amplitude of a radio-frequency magnetic field as a nonlinear function determined from the Bloch''s equations. Bistability hysteretic phenomena and unstable operating regimes of the structure in question have been found.
Experimental investigations of nonlinear characteristics of the transfer coefficient (G) and bistability phenomena in a quasioptical resonator with the ruby layer saturated under the electron spin resonance conditions (ESR) are presented. Experiments have been carried out on the special radiophysical complex BURAN /1/ at the electromagnetic wave frequency ν = 75⋅109H3 and in the temperature range T = 0.9 K + 4 K and with the static magnetic field H<6 T. A two-mirror half-symmetric open resonator has the mirror aperture about 2a=8λ, the radius of a spherical mirror R = 15λ , the quality factor Q ≈8⋅103 and operates on the spectral mode TEM0011. A ruby layer (thickness h = λ/4) is placed near the plane mirror.
The results of the analysis of the stability of stationary solutions of wave equations describing a behavior of the nonlinear Fabry-Perot interferometer with a saturated paramagnetic filling are presented in this paper. The cases when paramagnetic medium is characterized by a homogeneously and non-homogeneously broadened line of the magnetic resonance have been considered. The analysis of the stability has been conducted using the two-layer Newton- Kantorovich method. Some characteristics of the electrodynamic structure under consideration have been calculated under conditions of high and low quality of the resonance structure and the absence of frequency deviation and magnetic field. These are transmission and absorption coefficients. Areas of unstable behavior of these characteristics of the resonance structure have been found.
The operation principle of the optical transistor is based on the optical bistability phenomenon and inversionless (differential) amplification in the passive Fabry-Perot resonator (OR), filled with a substance having non-linear adsorption or refraction. In the millimeter wave range such resonator with a paramagnetic saturated by the UHF field under the ESR conditions is used to reach the similar purposes. In the paper the results of experimental and theoretical investigations of the non-linear OR (quasi-optical ESR-cell) with the ruby layer in 4-millimeter wave range at the temperatures T
In this work a theoretical study of the interaction between a light beam and an anisotropic nonlinear interferometer has been considered and methods to control the transmission of the microcavity using optical and magnetic fields have been developed. It has been demonstrated that anisotrophy of intracavity media determines the differences in transmission functions for various polarization modes and produces polarization instability. Varying spectroscopic parameters of the resonant medium and parameters of the anisotropic element, different types of intensity self-oscillations for different polarization modes can be obtained. To control the characteristics of nonlinear interferometer, it is proposed to use an additional light beam whose frequency is tuned into the absorption band from the excited level. The propagation characteristics of periodic magento-optical and dielectric multilayer films made of alternating layers of these materials having a symmetric periodicity with the center of the structure under a magnetic field is analyzed. The magnetic induction on this type of materials is temperature dependent and modifies the transmission and reflection characteristics of these structures. This kinds of structures, gives us the possibilities for an additional controlling of the characteristics of nonlinear interferometer.
For atomic media with resonant Doppler-broadened transitions of J=0 to J'=1 or J=1 to J'=0 type and taking into account the relaxation due to depolarizing collisions a theory of nonlinear magneto-optic polarization phenomena is developed. The theory is valid in the case of both arbitrary resonance linearly-polarized radiation intensity and arbitrary external magnetic field spatial orientation. The Faraday and Voigt geometries are analysed in detail, and in the case of the Faraday geometry the effect is considered of a noncompensated magnetic field transverse component on the shape of a dependence relating the radiation polarization plane rotation angle to a magnetic field longitudinal component. In the case of the Voigt geometry an essential effect is found of the angle between the radiation initial polarization and transverse magnetic field vectors on the character of the dependence relating the radiation polarization plane rotation angle to the transverse magnetic field magnitude.
An investigation is made of the change in the magnetic properties of a diamagnetic molecule (atom) induced by a resonance optical radiation field. Calculations are made for the 0→1 molecular transition in the presence of an external magnetostatic field. Expressions are derived for the magnetization and the magnetic susceptibility of the molecule, which depend nonlinearly on the light wave intensity, in the case of longitudinal and transverse directions of the external magnetic field with respect to the direction of propagation of the radiation. It is shown that the field-induced nonlinear magnetic susceptibility of a diamagnetic substance can change sign and increase considerably (by several orders of magnitude compared with the linear diamagnetic susceptibility). The field-induced nonlinear magnetization of the substance does not depend on its magnetic properties and is the same for diamagnetic and paramagnetic substances.