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Physical Review Letters

High Contrast Ramsey Fringes with Coherent-Population-Trapping Pulses in a Double Lambda Atomic System

T. Zanon-Willette, Stéphane Guérandel, Emeric de Clercq, David Holleville, N. Dimarcq, Andr  Clairon

Published May 17, 2005• 268 citations
Publisher

Abstract

We report the observation of Raman-Ramsey fringes using a double lambda scheme creating coherent population trapping in an atomic ensemble combined with pulsed optical radiations. The observation was made in a Cs vapor mixed with N2 buffer gas in a closed cell. The double lambda scheme is created with lin perpendicular lin polarized laser beams leading to higher contrast than the usual simple lambda scheme. The pulsed trapping technique leads to narrow fringe widths scaling as 1/(2T) with high contrasts which are no longer limited by the saturation effect. This technique operates in a different way from the classical Ramsey sequence: the signal is done by applying a long trapping pulse to prepare the atomic state superposition, and fringe detection is accomplished by optical transmission during a short second trapping pulse without any perturbation of the dark state.

DOI
10.1103/physrevlett.94.193002

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We report the observation of Raman-Ramsey fringes using a double lambda scheme creating coherent population trapping in an atomic ensemble combined with pulsed optical radiations. The observation was made in a Cs vapor mixed with N2 buffer gas in a closed cell. The double lambda scheme is created with lin perpendicular lin polarized laser beams leading to higher contrast than the usual simple lambda scheme. The pulsed trapping technique leads to narrow fringe widths scaling as 1/(2T) with high contrasts which are no longer limited by the saturation effect. This technique operates in a different way from the classical Ramsey sequence: the signal is done by applying a long trapping pulse to prepare the atomic state superposition, and fringe detection is accomplished by optical transmission during a short second trapping pulse without any perturbation of the dark state.
The Ramsey method has been applied by means of optical coherent population trapping (CPT) pulses through a cesium vapor cell with N/sub 2/ buffer gas at room temperature, using two phase-locked lasers. With this method, CPT resonance spectral widths are no longer limited by optical saturation and collision effects, but only depend on free evolution time between the two pulses. A fringe width below 100 Hz is reported. Experimental Raman-Ramsey fringes are analyzed using the classical wavefunction formalism.
We report the results of experimental investigation of the Raman – Ramsey method of pulsed excitation of coherent population trapping (CPT) resonances in a rubidium vapour cell filled with a mixture of Ar and Ne buffer gases. For the development of compact quantum microwave frequency standards, this method is an alternative to the pulsed optical pumping method recently implemented using the same rubidium cell. Both methods have advantages over the traditional double radio-optical resonance technique, the main of which is the substantial suppression of the light shift of the clock transition frequency, since the evolution of the coherence of atomic states forming the clock transition occurs in the absence of laser radiation in the cell. The narrow (110 – 240 Hz) Raman – Ramsey resonances are obtained using the scheme of pulsed excitation of CPT resonances on the D 1 lines of the 87 Rb atom with the same linear (lin||lin) polarisations of the bichromatic laser radiation components. The process of optimising the central fringe linewidth, its contrast, and the linewidth-to-contrast ratio is described. The magnetic dependence of the Raman – Ramsey line central fringe linewidth is experimentally investigated.
The linewidth of CPT atomic resonances observed in a vapor cell are usually limited by optical saturation and collisions due to buffer gas. We have applied here the Ramsey method with optical CPT pulses generated by a phase-locked device. Fringes are then produced giving narrow atomic signals only dependent on interrogation time between the two pulses. The possibility to obtain narrow fringe widths below 100 Hz with short or long pulses is shown experimentally and analysed using the classical Schrodinger state representation.
High contrast transparent Ramsey fringes are observed using double microwave pulses interaction with the prepared atomic coherent state in a warm 87 Rb vapor with mixture buffer gases in a closed cell.The Ramsey fringes are generated by the pulsed technique, a strong coupling light pulse and a weak signal light pulse are applied to prepare the atomic coherent state, followed by the application of double microwave pulses to interact with the atomic coherent state.Afterwards, the light pulses are applied again with weaker intensity and detecting the signal transmission is delected.The central line of the transparent Ramsey fringes has narrow linewidth of 125 Hz and high contrast of 21%.The light shift is dramatically reduced since the interrogating process is not involved the light field, and the cavity pulling effect is negligible due to the low Q requirement, which is promising for building small, compact, and stable atomic clocks.
We report on the detection of high-contrast and narrow Coherent Population Trapping (CPT) Ramsey fringes in a Cs vapor cell using a simple-architecture laser system. The latter allows the combination of push-pull optical pumping (PPOP) and a temporal Ramsey-like pulsed interrogation. An originality of the optics package is the use of a single Mach-Zehnder electro-optic modulator (MZ EOM) both for optical sidebands generation and light switch for pulsed interaction. Typical Ramsey fringes with a linewidth of 166 Hz and a contrast of 33 % are detected in a cm-scale buffer-gas filled Cs vapor cell. This technique could be interesting for the development of high-performance and low power consumption compact vapor cell clocks based on CPT.
We demonstrate a high-performance coherent-population-trapping (CPT) Cs vapor cell atomic clock using the push-pull optical pumping technique in the pulsed regime, allowing the detection of high-contrast and narrow Ramsey-CPT fringes. The impact of several experimental parameters onto the clock resonance and short-term fractional frequency stability, including the laser power, the cell temperature, and the Ramsey sequence parameters, has been investigated. We observe and explain the existence of a slight dependence on laser power of the central Ramsey-CPT fringe line-width in the pulsed regime. We report also that the central fringe line-width is commonly narrower than the expected Ramsey line-width given by 1/(2TR), with TR the free-evolution time, for short values of TR. The clock demonstrates a short-term fractional frequency stability at the level of 2.3×10−13 τ−1/2 up to 100 s averaging time, mainly limited by the laser amplitude modulation noise. Comparable performances are obtained in the conventional continuous wave regime, with the use of an additional laser power stabilization setup. The pulsed interaction allows to reduce significantly the clock frequency sensitivity to laser power variations, especially for high values of TR. This pulsed CPT clock, ranking among the best microwave vapor cell atomic frequency standards, could find applications in telecommunication, instrumentation, defense or satellite-based navigation systems.