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Physical Review A

Optical polarization modulation by competing atomic coherence effects in a degenerate four-level Yb atomic system

Sung Jong Park, Chang Yong Park, Tai Hyun Yoon

Published Jun 28, 2005• 12 citations
Publisher

Abstract

A scheme of optical polarization modulation of a linearly polarized infrared probe field is studied in a degenerate four-level Yb atomic system. We have observed an anomalous transmission spectra of two circular polarization components of the probe field exhibiting an enhanced two-photon absorption and a three-photon gain with comparable magnitude, leading to the lossless transmission and enhanced circular dichroism. We carried out a proof-of-principle experiment of fast optical polarization modulation in such a system by modulating the polarization state of the coupling field. The observed enhanced two-photon absorption and three-photon gain of the probe field are due to the result of competing atomic coherence effects.

DOI
10.1103/physreva.71.063819

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A scheme of optical polarization modulation of a linearly polarized infrared probe field is studied in a degenerate four-level Yb atomic system. We have observed an anomalous transmission spectra of two circular polarization components of the probe field exhibiting an enhanced two-photon absorption and a three-photon gain with comparable magnitude, leading to the lossless transmission and enhanced circular dichroism. We carried out a proof-of-principle experiment of fast optical polarization modulation in such a system by modulating the polarization state of the coupling field. The observed enhanced two-photon absorption and three-photon gain of the probe field are due to the result of competing atomic coherence effects.
When a four-level Y\mathsf{Y}Y-type atom with two highest nearly degenerate lying levels interacts with the same vacuum radiation field, its excited levels have vacuum-induced coherence due to the quantum interference between the spontaneous decay channels. We consider the effects of the vacuum-induced coherence on the electromagnetically induced transparency against single- and two-photon absorption in the atomic system. We find that the vacuum-induced coherence can lead to probe gain without incoherent pumping. On the other hand, the coherence can suppress the two-photon transparency, even in some cases where it can enhance the two-photon absorption. Another important result is the finding of the crucial role played by the relative phase between the probe and coupling fields: the two-photon transparency and the probe gain spectra can be modulated by this phase.
When the transitions connected by two nearly degenerate ground levels with an intermediate level in a four-level inverted Y-type atom interact with the same vacuum radiation field,which will lead to the quantum interference and create the vacuum-induced coherence.We find that the vacuuminduced coherence can suppress the single-and two-photon transparency at resonance and lead to single-photon probe gain at other frequency.Meanwhile,it is shown that the single-and two-photon absorption spectra can be drastically modulated by the relative phase between the probe and coupling fields.
We report the observation of laser-induced birefringence (LIB) in a wavelength-mismatched cascade system ($J=0\ensuremath{\leftrightarrow}J=1\ensuremath{\leftrightarrow}J=0$ transitions) of inhomogeneously broadened ytterbium atoms with strong pump and probe fields. We investigate the transmission spectrum of two circular polarization (${\ensuremath{\sigma}}_{p}^{+}$ and ${\ensuremath{\sigma}}_{p}^{\ensuremath{-}}$) components of strong probe field at fixed frequency, depending on the detuning of a circularly polarized $({\ensuremath{\sigma}}_{c}^{\ensuremath{-}})$ coupling field from two-photon resonance. We find that the ${\ensuremath{\sigma}}_{p}^{+}$ $({\ensuremath{\sigma}}_{p}^{\ensuremath{-}})$ polarized component exhibits a narrow electromagnetically induced absorption (transparency) spectrum. Numerical solutions of density matrix equations show qualitative agreement with experimental results. A Doppler-free dispersive LIB signal is obtained by detecting the Stokes parameter of the probe field, enabling us to stabilize the frequency of the coupling laser without frequency modulation.
Abstract We have studied the rotation of an elliptically polarized light propagating through thermal rubidium vapor with efficient four-wave mixing (FWM) and cross-phase modulation (XPM). These nonlinear processes are enhanced by Zeeman coherence within the degenerate sub-levels of the two-level atomic system. The elliptically polarized light with small ellipticity is considered as the superposition of a strong-linearly-polarized pump beam and a weak-orthogonal-polarized probe beam. The interference of the probe and the newly generated light field due to degenerate FWM and their gain in the medium due to a large XPM induced by the pump beam leads to the rotation of the elliptical polarized light. A theoretical analysis of the probe propagation through the nonlinear medium was used to explain the experimental observation and the fitting of the experimental data gives the estimates of the third-order non-linear susceptibilities associated with FWM and XPM. Our study can provide useful parameters for the generation of efficient squeezed vacuum states and squeezed polarization states of light. Furthermore our study finds application in controlling the diffraction of a linearly-polarized light beam traversing the medium.
Abstract We present a theoretical study of four-wave mixing (FWM) in a degenerate two-level atomic system subject to a magnetic field whose Zeeman sublevels constitute a tripod-type atomic system, which is driven by a linearly polarized field, and coupled and probed by two sets of left and right circularly polarized fields. The optical effects of coherent hole burning (CHB) and electromagnetically induced transparency (EIT) are involved in the coherent system, among which the CHB has much larger response for the FWM than the EITs. Three situations of CHB are involved, and they are the solitary CHB, overlapped CHBs, and an overlap between CHB and EIT. The overlapped CHBs have the greatest magnitude of FWM signal among the three situations. Whereas, for the overlapped CHB and EIT, it has the smallest FWM magnitude, which is no more than one tenth of the former. While for the single CHB, the FWM magnitude is half of that of the overlapped CHBs. It is noted that, in the overlap between CHB and EIT, dual EIAs can be obtained, whose FWM signal also has an enhancement in comparison to no EIA.
Abstract This paper describes the first observation of polarization-selective four-wave mixing signals in conventional coupling-probe spectroscopy, specifically, saturation absorption spectroscopy in 85Rb atoms. The four-wave mixing signal is induced by two counter-propagating laser beams in a degenerate multi-level atomic system, involving the Fg=3→Fe=2,3F_g=3 \rightarrow F_e =2,3Fg​=3→Fe​=2,3 F g = 3 → F e = 2 , 3 , and 4 transitions of the 85Rb D2 line. Consequently, the four-wave mixing signals copropagating along the probe beam induce polarization rotation of a linearly polarized probe beam. To distinguish these four-wave mixing signals from the resulting probe beam, we detect the polarization components orthogonal to the polarization direction of the input probe beam, depending on the linear polarization angles between the probe and coupling beams. The experimental findings demonstrate excellent agreement with theoretical results.