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Nature

Measurements of Lifetimes of Excited States of Atoms by the Method of Delayed Coincidences

S. HERON, R. W. P. McWhirter, E. H. Rhoderick

Published Sep 1, 1954• 22 citations
Publisher
DOI
10.1038/174564a0

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An electronic method for improving the delayed coincidence method in the measurement of the lifetime of the. excited state of an atom is proposed. A gate circuit which used tunnel diodes was studied. For the tunnel diode 1 N 3219 the calculation led to a rise time of the order of 0.8 nsec. (tr-auth)

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physica status solidi (a)•Apr 16, 1992•2 citations

Measured Lifetime of the ( 3p54s ) P13 State of Argon

John L. Morack, Clifford E. Fairchild

A direct measurement of the natural lifetime for the ($3{p}^{5}4s$) $^{3}P_{1}$ state of argon has been made using a modified delayed-coincidence method. Argon atoms are repetitively excited by pulses of electrons. For each pulse, the decaying light signal is sampled for a time $\ensuremath{\Delta}t$ at some delay time ${t}_{1}$ after the excitation is terminated. The exponential decay is then reconstructed as the delay time is changed. Collision effects are not important in the pressure region (5.0\ifmmode\times\else\texttimes\fi{}${10}^{\ensuremath{-}6}$-2.0\ifmmode\times\else\texttimes\fi{}${10}^{\ensuremath{-}4}$ Torr) of the experiment and the effects due to cascading are eliminated by keeping the energy of the bombarding electrons low enough so that excitation of the $3{p}^{5}4p$ levels is negligible. The measured lifetime is dependent upon the argon pressure, and this effect is attributed to resonance trapping; a value of 21\ifmmode\pm\else\textpm\fi{}2 nsec is obtained for the natural lifetime by using the existing theories of resonance trapping to extrapolate the data to zero pressure.

Physical Review•Nov 5, 1967•18 citations
A direct measurement of the natural lifetime for the (3p54s3{p}^{5}4s3p54s) 3P1^{3}P_{1}3P1​ state of argon has been made using a modified delayed-coincidence method. Argon atoms are repetitively excited by pulses of electrons. For each pulse, the decaying light signal is sampled for a time $\ensuremath{\Delta}t$ at some delay time t1{t}_{1}t1​ after the excitation is terminated. The exponential decay is then reconstructed as the delay time is changed. Collision effects are not important in the pressure region (5.0\ifmmode\times\else\texttimes\fi{}${10}^{\ensuremath{-}6}$-2.0\ifmmode\times\else\texttimes\fi{}${10}^{\ensuremath{-}4}$ Torr) of the experiment and the effects due to cascading are eliminated by keeping the energy of the bombarding electrons low enough so that excitation of the 3p54p3{p}^{5}4p3p54p levels is negligible. The measured lifetime is dependent upon the argon pressure, and this effect is attributed to resonance trapping; a value of 21\ifmmode\pm\else\textpm\fi{}2 nsec is obtained for the natural lifetime by using the existing theories of resonance trapping to extrapolate the data to zero pressure.