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Quantum Electronics

Resonances of coherent population trapping in samarium vapours

N. Kolachevsky, Alexey V. Akimov, Nikolai A. Kiselev, А. А. Папченко, Vadim N Sorokin, S. I. Kanorskii

Published Jan 31, 2001• 15 citations
Publisher

Abstract

Resonances of coherent population trapping were detected in atomic vapours of the rare-earth element samarium. The coherent population trapping was produced by two external-cavity diode lasers (672 and 686 nm) in a Λ-system formed by the three levels of 154 Sm: the 4 f 6 6 s 2 ( 7 F 0 ) ground state, the first fine-structure 4 f 6 6 s 2 ( 7 F 1 ) sublevel of the ground state and the 4 f 6 ( 7 F )6 s 6 p ( 3 P o ) 9 F o 1 upper level. The dependence of the spectral shapes and resonance contrasts on the polarisation of the laser beams and the direction of the applied magnetic field was studied. The obtained results were analysed.

DOI
10.1070/qe2001v031n01abeh001892

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Resonances of coherent population trapping were detected in atomic vapours of the rare-earth element samarium. The coherent population trapping was produced by two external-cavity diode lasers (672 and 686 nm) in a Λ-system formed by the three levels of 154 Sm: the 4 f 6 6 s 2 ( 7 F 0 ) ground state, the first fine-structure 4 f 6 6 s 2 ( 7 F 1 ) sublevel of the ground state and the 4 f 6 ( 7 F )6 s 6 p ( 3 P o ) 9 F o 1 upper level. The dependence of the spectral shapes and resonance contrasts on the polarisation of the laser beams and the direction of the applied magnetic field was studied. The obtained results were analysed.
We have detected and analyzed narrow, high contrast coherent population trapping resonances, which appear in transmission of the probe monochromatic light beam under action of the counterpropagating two-frequency laser radiation, on example of the nonclosed three level Λ-system formed by spectral components of the Doppler broadened D2 line of cesium atoms (in the cell with the rarefied Cs vapor). These nontrivial resonances are determined directly by the trapped atomic population on the definite lower level of the Λ-system and may be used in atomic frequency standards, sensitive magnetometers and in ultrahigh resolution laser spectroscopy of atoms and molecules.
A universal theory for calculating coherent population trapping resonances in multilevel atoms is suggested. The theory allows arbitrary schemes of multilevel atoms and their excitations to be calculated taking into account the influence of relaxation effects in atoms, applied magnetic field, and the Doppler effect. The experimental data obtained by high-precision diode spectroscopy of coherent dark resonances in samarium vapor are systematically analyzed using the suggested theory. In the absence of a magnetic field, the model of samarium is based on consideration of a degenerate Λ system of the 4f 66s 2(7 F 0) ↔ 4f 6(7 F)6s6p(3 P 0)9 F 1 0 ↔4f 66s 2(7 F 1) active transitions. If the fourth 4f 66s 2(7 F 2) level is taken into account, this Λ system becomes open. Numerical simulation of coherent population trapping resonances shows that the open character of the system decreases the contrast of resonance curves in absorption spectra without changing resonance widths. The system under applied external longitudinal and transverse magnetic fields is correctly described by 7-and 12-level models of atomic transitions, respectively.
A theoretical model of the coherent population trapping (CPT) in multilevel samarium atom and its comparison with experimental spectroscopic data are presented. Theoretical model describes a degenerated (Lambda) -system in Sm atom formed of the transitions 4f66s2(7F0) mutually implies 4f6(7F)6s6p(3Po)9Fo1 mutually implies 4f66s2(7F1) and includes also a fourth level 4f66s2(7F2), which complements the model making it an open system. An open character of the system reduces the contrast of the resonance curves in the CPT- spectra, but does not change the width of the CPT resonance. Numerical modeling of the CPT resonances in Sm atom was carried out for the case of applied longitudinal and transverse magnetic fields in 7- and 12-level models, as well.
The dependence of the shape of resonances of coherent population trapping (CPT) on magnetic sublevels of thallium atoms, forming a generalized Λ-system with the magnetic sublevels of the fine-structure levels as lower ones, on the polarization of the radiation fields has been numerically studied. The cases of linear, elliptical, and circular polarizations have been considered. The shape and the number of CPT resonances for different polarizations have been compared. It has been concluded that the electromagnetically induced transparency can be changed by changing the polarization properties of the laser radiation. The possibility to decrease the number of observed resonances may be useful in high-resolution spectroscopy.
At the conditions of two-photon resonance the effect of coherent population trapping (CPT) can take place. The CPT may be observed as in absorption so in resonance fluorescence. The CPT is widely applied in high resolution spectroscopy, laser cooling, atomic optics and so on. Earlier the peculiarities of CPT resonances on fine structure levels of an atom have been considered on example of thallium atoms. It was shown that the form and number of resonances are influenced by geometry of experiment and initial conditions (initial level populations). As the investigations of CPT on fine structure levels are the object of interest last years, we have considered the numerical analysis of dependence the form of CPT resonances on fine structure levels of T1 atoms as lower levels of Λ-system on polarization of radiation fields. The cases of elliptical, linear and circular polarization have been considered.
Specific features of the coherent population trapping effect are considered in the generalized Λ system whose lower levels are the magnetic sublevels of the fine structure levels of the thallium atom. Numerical experiments were performed aimed at examination of the coherent population trapping for the case of nontrivial, but feasible, initial populations of the upper metastable fine structure level. Such populations may be obtained, for example, due to the photodissociation of TlBr molecules. The possibility of reducing the number of resonances of the coherent population trapping in a multilevel system, which may be useful for high-resolution spectroscopy, is demonstrated. It is shown that the magnitude and shape of the resonances can be controlled by varying the orientation of the polarization vectors of the light field components with respect to each other and to a magnetic field. In addition, studying the shape of the coherent population trapping resonances for the atoms obtained by photodissociation of molecules may provide information about these molecules.