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Journal of Physics B Atomic and Molecular Physics

Conservation of angular momentum for light propagating in a transparent anisotropic medium

George Moe, W. Happer

Published May 11, 1977• 18 citations
Publisher

Abstract

When light propagates through a transparent medium, both the orbital and spin angular momenta of the light may change. It is shown by explicit calculation that the change in the angular momentum of the light is exactly equal and opposite to the change in the internal angular momentum of the atoms in the transparent medium. The centre-of-mass motion of the atoms does not play any significant role in this interchange of angular momentum.

DOI
10.1088/0022-3700/10/7/009

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When light propagates through a transparent medium, both the orbital and spin angular momenta of the light may change. It is shown by explicit calculation that the change in the angular momentum of the light is exactly equal and opposite to the change in the internal angular momentum of the atoms in the transparent medium. The centre-of-mass motion of the atoms does not play any significant role in this interchange of angular momentum.
We consider the propagation of slow light with an orbital angular momentum (OAM) in a moving atomic medium. We have derived a general equation of motion and applied it in analyzing propagation of slow light with an OAM in a rotating medium, such as a vortex lattice. We have shown that the OAM of slow light manifests itself in a rotation of the polarization plane of linearly polarized light. To extract a pure rotational phase shift, we suggest to measure a difference in the angle of the polarization plane rotation by two consecutive light beams with opposite OAM. The differential angle $\ensuremath{\Delta}{\ensuremath{\alpha}}_{l}$ is proportional to the rotation frequency of the medium ${\ensuremath{\omega}}_{\text{rot}}$ and the winding number lll of light, and is inversely proportional to the group velocity of light. For slow light the angle $\ensuremath{\Delta}{\ensuremath{\alpha}}_{l}$ should be large enough to be detectable. The effect can be used as a tool for measuring the rotation frequency ${\ensuremath{\omega}}_{\text{rot}}$ of the medium.
The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.
In the interaction of molecules with light endowed with orbital angular momentum, an exchange of orbital angular momentum in an electric dipole transition occurs only between the light and the center of mass motion; i.e., internal "electronic-type" motion does not participate in any exchange of orbital angular momentum in a dipole transition. A quadrupole transition is the lowest electric multipolar process in which an exchange of orbital angular momentum can occur between the light, the internal motion, and the center of mass motion. This rules out experiments seeking to observe exchange of orbital angular momentum between light beams and the internal motion in electric dipole transitions.
Light contains both spin and orbital angular momentum. Despite contributing equally to the total photonic angular momentum, these components derive from quite different parts of the electromagnetic field profile, namely its polarization and spatial variation, respectively, and therefore do not always share equal influence in light–matter interactions. With the growing interest in utilizing light’s orbital angular momentum to practice added control in the study of atomic systems, it becomes increasingly important for students and researchers to understand the subtlety involved in these interactions. In this article, we present a review of the fundamental concepts and recent experiments related to the interaction of beams containing orbital angular momentum with atoms. An emphasis is placed on understanding light’s angular momentum from the perspective of both classical waves and individual photons. We then review the application of these beams in recent experiments, namely single- and few-photon transitions, strong-field ionization, and high-harmonic generation, highlighting the role of light’s orbital angular momentum and the atom’s location within the beam profile within each case.
Anisotropy of angular momenta: ideas and methods The fundamental idea forming the basis of early quantum theory was the quantization of the angular momentum of the atom, which, at a later stage, assumed the form of the Bohr–Sommerfeld quantization rule [360], namely ∲ pdq = n ℏ where p and q are the generalized momentum and coordinate. This concept has retained its physical meaning in modern-day quantum mechanics [371, 372]. In the course of the further development of quantum mechanical concepts it became increasingly clear that in the theory of atoms and molecules the angular momentum is a ‘dominant’ notion, the fundamental significance of which is in no small degree connected with its dimension of action, which coincides with that of Planck's constant ℏ. In the interaction between particles and a directed beam of photons the angular momentum of the system is conserved, thus forming the basis for the optical method of producing spatial anisotropy of the distribution of the angular momenta of the ensemble of particles, i.e. its optical polarization . In terms of quantum concepts, spatial anisotropy means that in an ensemble of particles a non-equilibrium population of magnetic sublevels m j of angular momenta is created. We make a distinction between the alignment of momenta, for instance in the absorption of linear polarized light, when there is no difference between the population of ± m j -sublevels, and orientation , when such a difference exists. Anisotropic distribution of angular momenta in an excited state, as produced in absorption, manifests itself directly in the polarization of fluorescence. It is rather likely that understanding of the anisotropic distribution of the angular momenta of atoms was enhanced by Hanle's [184] discovery in 1924.