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arXiv:1403.2881 · Physical Review A

Angular momentum transfer in interaction of Laguerre-Gaussian beams with atoms and molecules

Pradip Kumar Mondal, Bimalendu Deb, Sonjoy Majumder

Published Jun 26, 2014• 92 citations
arXivHTMLPDF

Abstract

The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.

DOI
10.1103/physreva.89.063418

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The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.
We derive the interaction Hamiltonian between a diatomic molecule and a Laguerre-Gaussian beam under the assumption of a small spread of the center of mass wave function of the molecule in comparison with the beam waist. Considering the dynamical variables of the center of mass, vibrational, rotational, and electronic motion, we show that, within the electronic dipole approximation, the orbital angular momentum of the field couples with the rotational and electronic motion. The changes in the transition probabilities and selection rules induced by the field orbital angular momentum and the applicability of the derived interaction mechanisms for polyatomic molecules are discussed.
In the interaction of molecules with light endowed with orbital angular momentum, an exchange of orbital angular momentum in an electric dipole transition occurs only between the light and the center of mass motion; i.e., internal "electronic-type" motion does not participate in any exchange of orbital angular momentum in a dipole transition. A quadrupole transition is the lowest electric multipolar process in which an exchange of orbital angular momentum can occur between the light, the internal motion, and the center of mass motion. This rules out experiments seeking to observe exchange of orbital angular momentum between light beams and the internal motion in electric dipole transitions.
The interaction of atoms and molecules with structured light, specifically laser light endowed with the property of orbital angular momentum, such as Laguerre-Gaussian light, is discussed. The primary effects of interest here are the influence of the light on the gross motion of atoms and molecules and the possibilities this motion provides for particle manipulation in cooling, heating and trapping experiments. It turns out that, in addition to the possibility of modifying translational motion, suitably structured light can facilitate the manipulation of rotational motion. The latter possibility arises from a light-induced torque that is directly attributable to the orbital angular momentum property of the light. We outline the physics responsible for these effects and consider applications to typical cases in which atoms and ions are subject to near resonant Laguerre-Gaussian beams, leading to characteristic trajectories and eventual trapping in specific regions. Details are given for optical molasses configurations based on twisted light beams arranged in one-, two- and three-dimensional counter-propagating pairs. We extend consideration to the case of liquid crystals, subject to Laguerre-Gaussian light tuned far off-resonance, and show how this leads to the twisting of the directors in the liquid crystal, coinciding with the intensity distribution of the light.
An analysis of superradiant scattering of light by ultracold atoms is presented in which the pump and scattered light consist of hollow counterrotating Laguerre-Gaussian beams possessing orbital angular momentum. It is shown that the interaction between the Laguerre-Gaussian beams and the atoms can give rise to a superradiant instability in which orbital angular momentum is transferred to the atoms and the probe field is amplified. In the case where the atoms constitute a dilute Bose-Einstein condensate (BEC) that is trapped in a one-dimensional ring geometry, the transfer of orbital angular momentum to the BEC during the instability means that the BEC spontaneously develops rotation in the ring.
We derive the interaction Hamiltonian of a Laguerre–Gaussian beam with a simple atomic system, under the assumption of a small spread of the centre of mass wavefunction in comparison with the waist of the Laguerre–Gaussian beam and taking into account the centre of mass motion of the atomic system. Using the properties of regular spherical harmonics the internal and centre of mass dynamical variables are separated without making any multipolar expansion. The features of angular momentum exchange process assisted by Laguerre–Gaussian beams and the influence of their winding number on the selection rules and transition probability of internal and centre of mass motion are discussed.
We generated orbital angular momentum in atoms with a spin degree of freedom and coherently transferred it to a light field, which resulted in the generation of a Laguerre-Gaussian (LG) beam. In this method, atoms obtain orbital angular momentum through Larmor precession around the quadrupole field. Successive operations of quadrupole and homogeneous magnetic fields lead to a change of sign in the LG beam or even generation of superposition states of the LG beam with different indexes in real time. Possible applications to control orbital angular momentum of arbitrary photons are also discussed.