Light contains both spin and orbital angular momentum. Despite contributing equally to the total photonic angular momentum, these components derive from quite different parts of the electromagnetic field profile, namely its polarization and spatial variation, respectively, and therefore do not always share equal influence in light–matter interactions. With the growing interest in utilizing light’s orbital angular momentum to practice added control in the study of atomic systems, it becomes increasingly important for students and researchers to understand the subtlety involved in these interactions. In this article, we present a review of the fundamental concepts and recent experiments related to the interaction of beams containing orbital angular momentum with atoms. An emphasis is placed on understanding light’s angular momentum from the perspective of both classical waves and individual photons. We then review the application of these beams in recent experiments, namely single- and few-photon transitions, strong-field ionization, and high-harmonic generation, highlighting the role of light’s orbital angular momentum and the atom’s location within the beam profile within each case.
Light contains both spin and orbital angular momentum. Despite contributing equally to the total photonic angular momentum, these components derive from quite different parts of the electromagnetic field profile, namely its polarization and spatial variation, respectively, and therefore do not always share equal influence in light–matter interactions. With the growing interest in utilizing light’s orbital angular momentum to practice added control in the study of atomic systems, it becomes increasingly important for students and researchers to understand the subtlety involved in these interactions. In this article, we present a review of the fundamental concepts and recent experiments related to the interaction of beams containing orbital angular momentum with atoms. An emphasis is placed on understanding light’s angular momentum from the perspective of both classical waves and individual photons. We then review the application of these beams in recent experiments, namely single- and few-photon transitions, strong-field ionization, and high-harmonic generation, highlighting the role of light’s orbital angular momentum and the atom’s location within the beam profile within each case.
The angular momentum of light is a useful resource for many applications. In specific physical architectures it can be considered as the sum of two independent terms, the spin and the orbital components, in analogy to particle systems. The spin angular momentum is related to the polarization of the optical beam, that is the direction of the oscillating electric field, whereas the orbital angular momentum is associated with the spatial distribution of the field. Being independent, spin and orbital angular momenta have been discovered and explored in separate contexts for many years, while only recently it has been considered the possibility to address both quantities on the same beam (or individual photons). The interaction between these two quantities gives rise to complex structures of the electromagnetic field, or to the so called classical entanglement in the domain of single photons. The research presented in this work aimed to show that combining spin and orbital angular momenta in light beams or single photons may be a useful tool for a variety of applications, with particular interest to the case of architectures characterized by spin-orbit interaction. This concept was made concrete through the design and the realization of several experiments, in the framework of singular optics, foundations of quantum mechanics, quantum information theory and quantum simulation.
The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly 25 years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter. Furthermore, the use of OAM in quantum information has generated a lot of excitement, as it allows for encoding large amounts of information on a single photon. Here, we explain the intuition that led to the first quantum experiment with OAM 15 years ago. We continue by reviewing some key experiments investigating fundamental questions on photonic OAM and the first steps to applying these properties in novel quantum protocols. At the end, we identify several interesting open questions that could form the subject of future investigations with OAM.This article is part of the themed issue 'Optical orbital angular momentum'.
The physics of optical vortices, also known as twisted light, is now a well-established and a growing branch of optical physics with a number of important applications and significant interdisciplinary connections.Optical vortex fields of widely varying forms and degrees of complexity can be realised in the laboratory by a host of different means.The interference between such beams with designated orbital angular momenta and optical spins (the latter is associated with wave polarisations) can be structured to conform to various geometrical arrangements.The focus of this review is on how such tailored forms of light can exert a controllable influence on atoms with which they interact.The main physical effects involve atoms in motion due to application of optical forces.The now mature area of atom optics has had notable successes both of fundamental nature and in applications such as atom lasers, atom guides and Bose-Einstein condensates.The concepts in atom optics encompass not only atomic beams interacting with light, but atomic motion in general as influenced by optical and other fields.Our primary concern in this review is on atoms in structured light where, in particular, the twisted nature of the light is made highly complex with additional features due to wave polarisation.These features bring to the fore a variety of physical phenomena not realisable in the context of atomic motion in more conventional forms of laser light.Atoms near resonance with such structured light fields become subject to electromagnetic fields with complex polarisation and phase distributions, as well as intricately structured intensity gradients and radiative forces.From the combined effect of optical spin and orbital angular momenta, atoms may also experience forces and torques involving an interplay between the internal and centre of mass degrees of freedom.Such interactions lead to new forms of processes including scattering, trapping and rotation and, as a result, they exhibit characteristic new features at the micro-scale and below.A number of distinctive properties involving angular momentum exchange between the light and the atoms are highlighted, and prospective applications are discussed.Comparison is made between the theoretical predictions in this area and the corresponding experiments that have been reported to date.
Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'.
Photons are an ideal candidate for encoding both classical and quantum information. Besides spin angular momentum associated with circular polarization, single photon can also carry other fundamentally new degree of freedom of orbital angular momentum related to the spiral phase structure of light. The key significance of orbital angular momentum lies in its potential in realizing a high-dimensional Hilbert space and in encoding a high-dimensional quantum information. Since Allen et al. [Allen L, Beijersbergen M W, Spreeuw R J C, Woerdman J P 1992 Phys. Rev. A 45 8185] recognized the physical reality of photon orbital angular momentum in 1992, rapidly growing interest has been aroused in orbital angular momentum (OAM) from both classical and quantum points of view. Here we present an overall review on the high-order orbital angular momentum of photon, including its preparation and manipulation based on some specific techniques and also its applications. The spatial light modulator is a commercial device that has been widely employed to generate the OAM beams. We make and identify the optical OAM superposition with very high quantum numbers up to l=360. Recently, the metallic spiral phase mirrors were also developed to produce high-order OAM beams up to l=5050. In addition, the Q-plates made of anisotropic and inhomogeneous liquid crystals were invented to generate high-order OAM beams in a polarization-controllable manner, and the OAM superposition of l=± 50 were achieved. Owing to high rotational symmetry, these high OAM beams have been found to have more and more important applications in the fields of high-sensitivity sensing and high-precision measurements. Two fascinating examples are discussed in detail. The first example is that the research group led by Prof. Zeilinger has prepared and observed the quantum entanglement of high orbital angular momenta up to l=±300 by the technique of polarization-OAM entanglement swapping, and they demonstrated that the angular resolution could be significantly improved by a factor of l. Their result was the first step for entangling and twisting even macroscopic, spatially separated objects in two different directions. The second example is that the research group led by Prof. Padgett has demonstrated an elegant experiment of rotational Doppler effects for visible light with l=±20 OAM superposition. They showed that a spinning object with an optically rough surface might induce a Doppler effect in light reflected from the direction parallel to the rotation axis, and the frequency shift was proportional to both the disk's angular speed and the optical OAM. The potential applications in noncontact measurement of angular speed and in significant improvement of angular resolution for remote sensing will be particularly fascinating.
Angular momentum plays an iniport,aiit role in both classical and quantum physics. Historically the angular momentum content of a photon was divided into spin or polarization angular momentum (PAM), which relies in the vectorial structure of the field, and orbital angular momentum (OAM), which is usually related with the spatial structure of the beam. It has been experimeiitally demonstrated that, under the paraxial approximation, one can manipulate independently the PAM and the OAM. While the former is a classical tool in quantum information experiments, only recently the potential of the OAM has been explored. In particular, it was demonstrated recently that the idler and signal photons produced in the process of spontaneous parametxic downconversion constitute an entangled state of OAM [l]. The experiment showed that when the beam that pumps the nonlinear crystal is an eigenstate of the OAM, the quantum state of the down converted photons can in principle be described as IQ