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Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences

Optical angular momentum and atoms

Sonja Franke‐Arnold

Published Jan 9, 2017• 103 citations
Publisher

Abstract

Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'.

DOI
10.1098/rsta.2015.0435

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Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'.
The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly 25 years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter. Furthermore, the use of OAM in quantum information has generated a lot of excitement, as it allows for encoding large amounts of information on a single photon. Here, we explain the intuition that led to the first quantum experiment with OAM 15 years ago. We continue by reviewing some key experiments investigating fundamental questions on photonic OAM and the first steps to applying these properties in novel quantum protocols. At the end, we identify several interesting open questions that could form the subject of future investigations with OAM.This article is part of the themed issue 'Optical orbital angular momentum'.
Light contains both spin and orbital angular momentum. Despite contributing equally to the total photonic angular momentum, these components derive from quite different parts of the electromagnetic field profile, namely its polarization and spatial variation, respectively, and therefore do not always share equal influence in light–matter interactions. With the growing interest in utilizing light’s orbital angular momentum to practice added control in the study of atomic systems, it becomes increasingly important for students and researchers to understand the subtlety involved in these interactions. In this article, we present a review of the fundamental concepts and recent experiments related to the interaction of beams containing orbital angular momentum with atoms. An emphasis is placed on understanding light’s angular momentum from the perspective of both classical waves and individual photons. We then review the application of these beams in recent experiments, namely single- and few-photon transitions, strong-field ionization, and high-harmonic generation, highlighting the role of light’s orbital angular momentum and the atom’s location within the beam profile within each case.
Angular momentum plays a central role in quantum mechanics, recurring in every length scale from the microscopic interactions of light and matter to the macroscopic behavior of superfluids. Vortex beams, carrying intrinsic orbital angular momentum (OAM), are now regularly generated with elementary particles such as photons and electrons. Thus far, the creation of a vortex beam of a nonelementary particle has never been demonstrated experimentally. We present vortex beams of atoms and molecules, formed by diffracting supersonic beams of helium atoms and dimers off transmission gratings. This method is general and could be applied to most atomic and molecular gases. Our results may open new frontiers in atomic physics, using the additional degree of freedom of OAM to probe collisions and alter fundamental interactions.
The exchange of orbital angular momentum between a Laguerre-Gaussian beam of light and the center-of-mass motion of an atom or molecule is well known. We show that the orbital angular momentum of light can also be transferred to the internal electronic or rotational motion of an atom or a molecule provided the internal and center-of-mass motions are coupled. However, this transfer does not happen directly to the internal motion, but via center-of-mass motion. If atoms or molecules are cooled down to the recoil limit, then an exchange of angular momentum between the quantized center-of-mass motion and the internal motion is possible during the interaction of cold atoms or molecules with the Laguerre-Gaussian beam. The orientation of the exchanged angular momentum is determined by the sign of the winding number of the Laguerre-Gaussian beam. We present selective results of numerical calculations for the quadrupole transition rates in the interaction of the Laguerre-Gaussian beam with an atomic Bose-Einstein condensate to illustrate the underlying mechanism of light orbital angular momentum transfer. We discuss how the alignment of diatomic molecules will facilitate exploration of the effects of light orbital angular momentum on the electronic motion of molecules.
The angular momentum of light is a useful resource for many applications. In specific physical architectures it can be considered as the sum of two independent terms, the spin and the orbital components, in analogy to particle systems. The spin angular momentum is related to the polarization of the optical beam, that is the direction of the oscillating electric field, whereas the orbital angular momentum is associated with the spatial distribution of the field. Being independent, spin and orbital angular momenta have been discovered and explored in separate contexts for many years, while only recently it has been considered the possibility to address both quantities on the same beam (or individual photons). The interaction between these two quantities gives rise to complex structures of the electromagnetic field, or to the so called classical entanglement in the domain of single photons. The research presented in this work aimed to show that combining spin and orbital angular momenta in light beams or single photons may be a useful tool for a variety of applications, with particular interest to the case of architectures characterized by spin-orbit interaction. This concept was made concrete through the design and the realization of several experiments, in the framework of singular optics, foundations of quantum mechanics, quantum information theory and quantum simulation.
This Chapter presents a review of the quantum mechanical properties of spatially structured light fields, specifically those fields carrying orbital angular momentum (OAM). This review is concerned both with the conceptual understanding of the quantum features of these light fields and with the use of these features for applications. We describe how to produce spatially entangled light fields by means of the nonlinear optical process of parametric downconversion. We ask and provide a tentative answer to the question of how much information can be encoded into a single photon. As an example, we review a recent experiment that demonstrated the ability to discriminate among four target objects using only one photon for illumination. We also present a description of the concept of the OAM of light, and we describe means to generate and detect OAM. We then present a brief survey of some recent studies of the fundamental quantum properties of structured light beams. Much of this work is aimed at studying the nature of entanglement for the complementary variables of angular position and OAM. Finally, as a realworld application, we describe a secure communication system based on quantum key distribution (QKD). This key distribution system makes use of encoding information in the OAM modes of light and hence is able to transmit more than one bit of information per photon. These keywords were added by machine and not by the authors. This process is experimental and the keywords may be updated as the learning algorithm improves.