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Physical Review Letters

Population Inversion in Optical Adiabatic Rapid Passage with Phase Relaxation

Yōsuke Kayanuma

Published May 11, 1987• 39 citations
Publisher

Abstract

The transition probability $P$ in the optical adiabatic rapid passage is calculated for a two-level model with dephasing. In the limit $\frac{{T}_{2}}{{\ensuremath{\tau}}_{p}}\ensuremath{\rightarrow}0$, where ${T}_{2}$ is the dephasing time and ${\ensuremath{\tau}}_{p}$ is the time scale of passage through the resonance region, $P$ is given by $P=\frac{[1\ensuremath{-}\mathrm{exp}(\ensuremath{-}\frac{\ensuremath{\pi}{\ensuremath{\chi}}^{2}}{|\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}|})]}{2}$ in which $\ensuremath{\chi}$ is the Rabi flopping frequency at resonance and $\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}$ is the time derivative of the offset angular frequency. Generally, $P$ takes its maximum value at an intermediate $\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}$ for fixed $\ensuremath{\chi}$ and is bounded by the above formula and by $P=1\ensuremath{-}\mathrm{exp}(\ensuremath{-}\frac{\ensuremath{\pi}{\ensuremath{\chi}}^{2}}{2|\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}|})$, which gives the asymptotic value in the limit $\frac{{T}_{2}}{{\ensuremath{\tau}}_{p}}\ensuremath{\rightarrow}\ensuremath{\infty}$.

DOI
10.1103/physrevlett.58.1934

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The transition probability PPP in the optical adiabatic rapid passage is calculated for a two-level model with dephasing. In the limit T2\ensuremathτp\ensuremath→0\frac{{T}_{2}}{{\ensuremath{\tau}}_{p}}\ensuremath{\rightarrow}0\ensuremathτp​T2​​\ensuremath→0, where T2{T}_{2}T2​ is the dephasing time and \ensuremathτp{\ensuremath{\tau}}_{p}\ensuremathτp​ is the time scale of passage through the resonance region, PPP is given by P=[1\ensuremath−exp(\ensuremath−\ensuremathπ\ensuremathχ2∣\ensuremathω\ifmmode˙\else˙\fi∣)]2P=\frac{[1\ensuremath{-}\mathrm{exp}(\ensuremath{-}\frac{\ensuremath{\pi}{\ensuremath{\chi}}^{2}}{|\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}|})]}{2}P=2[1\ensuremath−exp(\ensuremath−∣\ensuremathω\ifmmode˙\else˙\fi​∣\ensuremathπ\ensuremathχ2​)]​ in which \ensuremathχ\ensuremath{\chi}\ensuremathχ is the Rabi flopping frequency at resonance and \ensuremathω\ifmmode˙\else˙\fi\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}\ensuremathω\ifmmode˙\else˙\fi​ is the time derivative of the offset angular frequency. Generally, PPP takes its maximum value at an intermediate \ensuremathω\ifmmode˙\else˙\fi\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}\ensuremathω\ifmmode˙\else˙\fi​ for fixed \ensuremathχ\ensuremath{\chi}\ensuremathχ and is bounded by the above formula and by P=1\ensuremath−exp(\ensuremath−\ensuremathπ\ensuremathχ22∣\ensuremathω\ifmmode˙\else˙\fi∣)P=1\ensuremath{-}\mathrm{exp}(\ensuremath{-}\frac{\ensuremath{\pi}{\ensuremath{\chi}}^{2}}{2|\stackrel{\ifmmode \dot{}\else \.{}\fi{}}{\ensuremath{\omega}}|})P=1\ensuremath−exp(\ensuremath−2∣\ensuremathω\ifmmode˙\else˙\fi​∣\ensuremathπ\ensuremathχ2​), which gives the asymptotic value in the limit T2\ensuremathτp\ensuremath→\ensuremath∞\frac{{T}_{2}}{{\ensuremath{\tau}}_{p}}\ensuremath{\rightarrow}\ensuremath{\infty}\ensuremathτp​T2​​\ensuremath→\ensuremath∞.
Theoretical investigations for the realization of population inversion of semiconductor quantum dot ground-state transitions by means of adiabatic passage with chirped optical pulses are presented. While the inversion due to Rabi oscillations depends sensitively on the resonance condition, the pulse area, as well as on the absence of carrier scattering and dephasing, we find that adiabatic passage is surprisingly insensitive to the excitation conditions and carrier scattering effects. Quantum kinetic models for the interaction of quantum-dot carriers with longitudinal optical phonons are used to describe carrier scattering and dephasing in the corresponding simulations and allow to quantify the conditions to simultaneously invert an ensamble of quantum dots.
This work explores the effect of phase relaxation on the population transfer efficiency in stimulated Raman adiabatic passage (STIRAP). The study is based on the Liouville equation, which is solved analytically in the adiabatic limit. The transfer efficiency of STIRAP is found to decrease exponentially with the dephasing rate; this effect is stronger for shorter pulse delays and weaker for larger delays, since the transition time is found to be inversely proportional to the pulse delay. Moreover, it is found that the transfer efficiency of STIRAP in the presence of dephasing does not depend on the peak Rabi frequencies at all, as long as they are sufficiently large to enforce adiabatic evolution; hence increasing the field intensity cannot reduce the dephasing losses. It is shown also that for any dephasing rate, the final populations of the initial state and the intermediate state are equal. For strong dephasing all three populations tend to 13\frac{1}{3}31​.
This Letter reports the first experimental observation of population inversion of a two-photon transition in NH3{\mathrm{H}}_{3}H3​ using the adiabatic rapid-passage technique. The population inversion was demonstrated by the observation of stimulated two-photon gain and emission. By use of this technique, the two-photon population relaxation time T1{T}_{1}T1​ was measured.
I report the observation of population inversion by optical adiabatic rapid passage. These observations, on an NH3{\mathrm{NH}}_{3}NH3​ infrared transition with all the relevant parameters known, agree with theoretical expectations. The pressure dependence of T1{T}_{1}T1​, obtained by this technique, makes possible the first estimate of the collision-induced rotational lifetime of NH3{\mathrm{NH}}_{3}NH3​ in an excited band, which is significantly longer than the rotational lifetime in the ground vibrational band.