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Applied Physics Letters

Rapid adiabatic passage in quantum dots: Influence of scattering and dephasing

K. Schuh, F. Jahnke, Michael Lorke

Published Jul 4, 2011• 12 citations
Publisher

Abstract

Theoretical investigations for the realization of population inversion of semiconductor quantum dot ground-state transitions by means of adiabatic passage with chirped optical pulses are presented. While the inversion due to Rabi oscillations depends sensitively on the resonance condition, the pulse area, as well as on the absence of carrier scattering and dephasing, we find that adiabatic passage is surprisingly insensitive to the excitation conditions and carrier scattering effects. Quantum kinetic models for the interaction of quantum-dot carriers with longitudinal optical phonons are used to describe carrier scattering and dephasing in the corresponding simulations and allow to quantify the conditions to simultaneously invert an ensamble of quantum dots.

DOI
10.1063/1.3609016

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Theoretical investigations for the realization of population inversion of semiconductor quantum dot ground-state transitions by means of adiabatic passage with chirped optical pulses are presented. While the inversion due to Rabi oscillations depends sensitively on the resonance condition, the pulse area, as well as on the absence of carrier scattering and dephasing, we find that adiabatic passage is surprisingly insensitive to the excitation conditions and carrier scattering effects. Quantum kinetic models for the interaction of quantum-dot carriers with longitudinal optical phonons are used to describe carrier scattering and dephasing in the corresponding simulations and allow to quantify the conditions to simultaneously invert an ensamble of quantum dots.
We demonstrate adiabatic rapid passage on a subpicosecond time scale in a single semiconductor quantum dot, enabling the exploration of a regime of strong (and rapidly varying) Rabi energies for optical control of excitons. An observed dependence of the exciton inversion efficiency on the sign of the pulse chirp demonstrates the dominance of phonon-mediated dephasing, which is suppressed for positive chirp at low temperature. Our findings will support the realization of dynamical decoupling strategies and suggest that multiphonon emission and/or non-Markovian effects should be taken into account.
The eect of acoustic phonons on dierent light-induced excitations of a semiconductor quantum dot is investigated.Resonant excitation of the quantum dot leads to the Rabi oscillations, which are damped due to the phonon interaction.When the excitation frequency is detuned, an occupation can only occur due to phonon absorption or emission processes.For frequency-swept excitations a population inversion is achieved through adiabatic rapid passage, but the inversion is also damped by phonons.For all three scenarios the inuence of the phonons depends non-monotonically on the pulse area.
Preparation of a specific quantum state is a required step for a variety of proposed quantum applications. We report an experimental demonstration of optical quantum state inversion in a single semiconductor quantum dot using adiabatic rapid passage. This method is insensitive to variation in the optical coupling in contrast with earlier work based on Rabi oscillations. We show that when the pulse power exceeds a threshold for inversion, the final state is independent of power. This provides a new tool for preparing quantum states in semiconductor dots and has a wide range of potential uses.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, then the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps, and moderate pulse areas.