Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Physical Review B

Subpicosecond adiabatic rapid passage on a single semiconductor quantum dot: Phonon-mediated dephasing in the strong-driving regime

Reuble Mathew, Eric Dilcher, Angela Gamouras, Ajan P. Ramachandran, Hong Yi Shi Yang, Sabine Freisem, DENNIS GLENN DEPPE, Kimberley C. Hall

Published Jul 25, 2014• 44 citations
Publisher

Abstract

We demonstrate adiabatic rapid passage on a subpicosecond time scale in a single semiconductor quantum dot, enabling the exploration of a regime of strong (and rapidly varying) Rabi energies for optical control of excitons. An observed dependence of the exciton inversion efficiency on the sign of the pulse chirp demonstrates the dominance of phonon-mediated dephasing, which is suppressed for positive chirp at low temperature. Our findings will support the realization of dynamical decoupling strategies and suggest that multiphonon emission and/or non-Markovian effects should be taken into account.

DOI
10.1103/physrevb.90.035316

Related papers

Subpicosecond adiabatic rapid passage in a single InGaAs quantum dot: Role of phonons in dephasing

Reuble Mathew, Eric Dilcher, Angela Gamouras +4 more

Robust excitation of an exciton state via adiabatic rapid passage is demonstrated in a single InGaAs quantum dot using subpicosecond optical pulses. A chirp sign dependence of the transfer efficiency indicates dephasing tied to phonons.

Journal of International Crisis and Risk Communication Research•Jan 1, 2014•0 citations

Demonstrating the decoupling regime of the electron-phonon interaction in a quantum dot using chirped optical excitation

Timo Kaldewey, Sebastian Lüker, Andreas V. Kuhlmann +7 more

Excitation of a semiconductor quantum dot with a chirped laser pulse allows excitons to be created by rapid adiabatic passage. In quantum dots this process can be greatly hindered by the coupling to phonons. Here we add a high chirp rate to ultrashort laser pulses and use these pulses to excite a single quantum dot. We demonstrate that we enter a regime where the exciton-phonon coupling is effective for small pulse areas, while for higher pulse areas a decoupling of the exciton from the phonons occurs. We thus discover a reappearance of rapid adiabatic passage, in analogy to the predicted reappearance of Rabi rotations at high pulse areas. The measured results are in good agreement with theoretical calculations.

arXiv:1701.01304•Physical review. B./Physical review. B•Jun 26, 2017•42 citations

Dephasing in the adiabatic rapid passage in quantum dots: the role of phonon-assisted biexciton generation

Krzysztof Gawarecki, Sebastian Lüker, Doris E. Reiter +5 more

We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and moderate pulse areas.

arXiv:1209.2675•Sep 12, 2012•0 citations

Influence of acoustic phonons on the optical control of quantum dots driven by adiabatic rapid passage

Sebastian Lüker, Krzysztof Gawarecki, Doris E. Reiter +4 more

The role of phonons for adiabatic rapid passage in semiconductor quantum dots is studied theoretically. While in an ideal system adiabatic rapid passage results in a full inversion of the quantum dot occupation, phonons hamper this behavior drastically. We show that the transitions between the adiabatic states lead to a temperature-dependent decrease of the final exciton occupation. In contrast to the ideal evolution, the phonon-related perturbation induces dependencies on the pulse power and on the sign of the chirp.

Physical Review B•Mar 15, 2012•65 citations

Dephasing in the adiabatic rapid passage in quantum dots: Role of phonon-assisted biexciton generation

Krzysztof Gawarecki, Sebastian Lüker, Doris E. Reiter +5 more

We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, then the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps, and moderate pulse areas.

Physical Review B•Dec 3, 2012•22 citations

Applications of femtosecond pulse engineering in the control of excitons in quantum dots

Reuble Mathew, Angela Gamouras, Eric Dilcher +5 more

Pulse shaping techniques are used to demonstrate quantum control of exciton qubits in InAs quantum dots. Linearly chirped laser pulses are used to demonstrate adiabatic rapid passage in a single quantum dot on a subpicosecond timescale. The observed dependence of the exciton inversion efficiency on the sign of the pulse chirp identifies phonons as the dominant source of dephasing, which can be suppressed for positive chirp at low temperatures. The use of optimal quantum control theory to engineer a single optical pulse to implement simultaneous π and 2π single qubit gates in two uncoupled quantum dots is demonstrated. This work will support the use of pulse shaping in solid-state quantum hardware.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Aug 28, 2014•0 citations
We demonstrate adiabatic rapid passage on a subpicosecond time scale in a single semiconductor quantum dot, enabling the exploration of a regime of strong (and rapidly varying) Rabi energies for optical control of excitons. An observed dependence of the exciton inversion efficiency on the sign of the pulse chirp demonstrates the dominance of phonon-mediated dephasing, which is suppressed for positive chirp at low temperature. Our findings will support the realization of dynamical decoupling strategies and suggest that multiphonon emission and/or non-Markovian effects should be taken into account.
Excitation of a semiconductor quantum dot with a chirped laser pulse allows excitons to be created by rapid adiabatic passage. In quantum dots this process can be greatly hindered by the coupling to phonons. Here we add a high chirp rate to ultrashort laser pulses and use these pulses to excite a single quantum dot. We demonstrate that we enter a regime where the exciton-phonon coupling is effective for small pulse areas, while for higher pulse areas a decoupling of the exciton from the phonons occurs. We thus discover a reappearance of rapid adiabatic passage, in analogy to the predicted reappearance of Rabi rotations at high pulse areas. The measured results are in good agreement with theoretical calculations.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps and moderate pulse areas.
The role of phonons for adiabatic rapid passage in semiconductor quantum dots is studied theoretically. While in an ideal system adiabatic rapid passage results in a full inversion of the quantum dot occupation, phonons hamper this behavior drastically. We show that the transitions between the adiabatic states lead to a temperature-dependent decrease of the final exciton occupation. In contrast to the ideal evolution, the phonon-related perturbation induces dependencies on the pulse power and on the sign of the chirp.
We study the evolution of an exciton confined in a quantum dot adiabatically controlled by a frequency-swept (chirped) laser pulse in the presence of carrier-phonon coupling. We focus on the dynamics induced by a linearly polarized beam and analyze the decoherence due to phonon-assisted biexciton generation. We show that if the biexciton state is shifted down by a few meV, as is typically the case, then the resulting decoherence is strong even at low temperatures. As a result, efficient state preparation is restricted to a small parameter area corresponding to low temperatures, positive chirps, and moderate pulse areas.
Pulse shaping techniques are used to demonstrate quantum control of exciton qubits in InAs quantum dots. Linearly chirped laser pulses are used to demonstrate adiabatic rapid passage in a single quantum dot on a subpicosecond timescale. The observed dependence of the exciton inversion efficiency on the sign of the pulse chirp identifies phonons as the dominant source of dephasing, which can be suppressed for positive chirp at low temperatures. The use of optimal quantum control theory to engineer a single optical pulse to implement simultaneous π and 2π single qubit gates in two uncoupled quantum dots is demonstrated. This work will support the use of pulse shaping in solid-state quantum hardware.